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arXiv 2403.04136cond-mat.mes-hallcond-mat.supr-con
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光学探测原子级厚度Bi$_2$Sr$_2$Ca$_{0.92}$Y$_{0.08}$Cu$_2$O$_{8+δ}$中的非常规超导性

Optically Probing Unconventional Superconductivity in Atomically Thin Bi$_2$Sr$_2$Ca$_{0.92}$Y$_{0.08}$Cu$_2$O$_{8+δ}$

Yunhuan Xiao, Jingda Wu, Jerry I Dadap, Kashif Masud Awan, Dongyang Yang, Jing Liang, Kenji Watanabe, Takashi Taniguchi, Marta Zonno, Martin Bluschke, Hiroshi E… 展开作者

Yunhuan Xiao, Jingda Wu, Jerry I Dadap, Kashif Masud Awan, Dongyang Yang, Jing Liang, Kenji Watanabe, Takashi Taniguchi, Marta Zonno, Martin Bluschke, Hiroshi Eisaki, Martin Greven, Andrea Damascelli, Ziliang Ye

AI总结:

本研究利用光学泵浦-探测方法非侵入式研究原子级厚度Y-Bi2212的非常规超导性,发现其超导响应与块体相近、信号受介电环境影响显著,揭示了单层材料的环境敏感性及超导凝聚体的层内本质,明确了双面封装的作用。

摘要:

近期已制备出超导相变温度与块体材料相近的原子级厚度铜氧化物,但其器件制备仍存在挑战,限制了诸多新型研究与应用的潜力。本文采用光学泵浦-探测方法,非侵入式研究原子级厚度Bi$_2$Sr$_2$Ca$_{0.92}$Y$_{0.08}$Cu$_2$O$_{8+δ}$(Y-Bi2212)的非常规超导性。除发现其超导相变对应的光学响应与块体Y-Bi2212相似外,还观测到原子级厚度薄片中泵浦-探测信号的符号与幅度在不同介电环境下会随光激发性质发生显著变化。借助光学探针的空间分辨率,研究揭示了单层Y-Bi2212对环境的极高敏感性。该结果为Bi2212中超导凝聚体的层内本质提供了首个光学证据,同时凸显了双面封装在维持原子级厚度铜氧化物超导性方面的作用。

英文摘要:

Atomically thin cuprates exhibiting a superconducting phase transition temperature similar to bulk have recently been realized, although the device fabrication remains a challenge and limits the potential for many novel studies and applications. Here we use an optical pump-probe approach to noninvasively study the unconventional superconductivity in atomically thin Bi$_2$Sr$_2$Ca$_{0.92}$Y$_{0.08}$Cu$_2$O$_{8+δ}$ (Y-Bi2212). Apart from finding an optical response due to the superconducting phase transition that is similar to bulk Y-Bi2212, we observe that the sign and amplitude of the pump-probe signal in the atomically thin flake vary significantly in different dielectric environments depending on the nature of the optical excitation. By exploiting the spatial resolution of the optical probe, we uncover the exceptional sensitivity of monolayer Y-Bi2212 to the environment. Our results provide the first optical evidence for the intralayer nature of the superconducting condensate in Bi2212, and highlight the role of double-sided encapsulation in preserving superconductivity in atomically thin cuprates.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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