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arXiv 2402.01347cond-mat.supr-concond-mat.dis-nn
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三维 MoTiN 超导薄膜中的量子格里菲斯奇异性

Quantum Griffiths singularity in three-dimensional MoTiN superconducting films

Zi-Xiao Wang, Tian-Yu Jing, Zi-Yan Han, Kuang-Hong Gao, Song-Ci Li, Zhi-Qing Li

AI总结:

本文在三维 MoTiN 超导薄膜场致超导-金属转变附近观测到量子格里菲斯奇异性,通过磁电阻标度分析证实其存在,为三维超导体中 QGS 提供了实验证据。

摘要:

量子格里菲斯奇异性(QGS)已在一系列二维(2D)超导体系中被实验观测到。尽管理论上认为 QGS 也存在于三维(3D)超导体中,但该理论预测几乎缺乏实验支持。本文中,我们在厚度约 80 nm 的 Mo$_{0.8}$Ti$_{0.2}$N$_x$($0.84 \lesssim x \lesssim 1.12$)超导薄膜系列中,在场驱动的超导-金属转变(SMT)附近观测到了 QGS 的出现。这些薄膜具有 NaCl 结构,且就超导电性而言属于三维体系。对每一薄膜,在磁场垂直于或平行于薄膜平面的条件下测得的低温磁电阻等温线并不相交于单一点,而是在一个清晰的宽区域内相交。通过分析相关磁电阻等温线得到的动力学临界指数 $zν_{\perp}$(垂直场)和 $zν_{\parallel}$(平行场)随温度降低而增大,并趋于在 $T\rightarrow 0$ K 时发散。此外,SMT 附近垂直场和平行场的有效电阻率数据均遵从基于随机横场 Ising 模型的激活标度律。我们还在低氮分压下制备了具有面心立方结构的约 80 nm 厚 (Mo$_{0.8}$Ti$_{0.2}$)$_2$N$_{1.06}$ 超导薄膜。研究发现,垂直(平行)场的低温磁电阻等温线相交于单一点,且场致 SMT 附近垂直(平行)场的电阻率数据遵从由脏玻色子模型导出的幂律标度。我们的结果为三维超导体中 QGS 的存在提供了明确的实验证据。

英文摘要:

Quantum Griffiths singularity (QGS) has been experimentally observed in a range of two-dimensional (2D) superconducting systems. Although it is theoretically suggested that the QGS also exists in three-dimensional (3D) superconductors, there is almost no experimental support to the theoretical prediction. In the present paper, we observe the occurrence of QGS in a series of $\sim$80-nm-thick Mo$_{0.8}$Ti$_{0.2}$N$_x$ ($0.84 \lesssim x \lesssim 1.12$) superconducting films near the field-driven superconductor-metal transition (SMT). These films have a NaCl structure and are 3D with respect to the superconductivity. For each film, the low-temperature magnetoresistance isotherms, measured at magnetic fields being perpendicular or parallel to the film plane, do not cross at a single point but at a clear wide region. The dynamical critical exponents $zν_{\perp}$ (for perpendicular field) and $zν_{\parallel}$ (for parallel field) obtained by analyzing the related magnetoresistance isotherms increase with decreasing temperature and tend to diverge as $T\rightarrow 0$ K. In addition, the effective resistivity data for the perpendicular and parallel field in the vicinity of the SMTs both obey an activated scaling based on the random transverse-field Ising model. We also fabricate a $\sim$80-nm-thick (Mo$_{0.8}$Ti$_{0.2}$)$_2$N$_{1.06}$ superconducting film with face-centered cubic structure at low nitrogen partial pressure. It is found that the low-temperature magnetoresistance isotherms for the perpendicular (parallel) field cross at a single point and the resistivity data for the perpendicular (parallel) field in the vicinity of the field-induced SMT obey the power-law scaling deduced from the dirty-boson model. Our results provide unambigous experimental evidence for the existence of QGS in 3D superconductors.

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