arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2402.00869cond-mat.supr-concond-mat.str-el
收藏

扭转双层石墨烯超导中的分子配对

Molecular Pairing in Twisted Bilayer Graphene Superconductivity

Yi-Jie Wang, Geng-Dong Zhou, Shi-Yu Peng, Biao Lian, Zhi-Da Song

AI总结:

本文提出魔角扭转双层石墨烯中声子介导的分子配对机制,证明掺杂关联绝缘体中重整化局域相互作用必存在配对通道,并分析了向列d波单重态配对对称性。

摘要:

我们提出了一种理论,解释弱的声子介导相互作用($J_{\rm A}\\!=\\!1\\!\sim\\!4$meV)如何战胜被禁止的库仑排斥($U\\!=\\!30\\!\sim\\!60$meV),并在魔角扭转双层石墨烯(MATBG)中导致超导。我们发现其配对机制类似于A$_3$C$_{60}$族分子超导体中的机制:MATBG的每个AA堆叠区域类似于一个C$_{60}$分子,其中光学声子可以动态地解除莫尔轨道的简并,类似于动态Jahn-Teller效应。这种诱导的$J_{\rm A}$具有谷间反洪特耦合的形式,并且在莫特绝缘体附近受到近藤屏蔽的抑制程度比$U$小。此外,我们还考虑了源于碳原子在位排斥的轨道内洪特耦合$J_{\rm H}$。在现实模型的合理近似下,我们证明在掺杂关联绝缘体中,准粒子之间的重整化局域相互作用在$ν=\pm(2+δν)$处必须具有配对(负)通道,尽管裸相互作用是正定的。该证明是非微扰的,并基于Ward恒等式所施加的顶点函数的精确渐近行为。我们预测了超导存在一个最优的$U$。我们还分析了配对对称性。在$J_{\rm A}$、$J_{\rm H}$参数空间的大片区域内,基态具有向列$d$波单重态配对,然而由于费米面上的Berry相位(或欧拉阻碍),这种配对可能导致类似$p$波的节点结构。

英文摘要:

We propose a theory for how the weak phonon-mediated interaction ($J_{\rm A}\!=\!1\!\sim\!4$meV) wins over the prohibitive Coulomb repulsion ($U\!=\!30\!\sim\!60$meV) and leads to a superconductor in magic-angle twisted bilayer graphene (MATBG). We find the pairing mechanism akin to that in the A$_3$C$_{60}$ family of molecular superconductors: Each AA stacking region of MATBG resembles a C$_{60}$ molecule, in that optical phonons can dynamically lift the degeneracy of the moiré orbitals, in analogy to the dynamical Jahn-Teller effect. Such induced $J_{\rm A}$ has the form of an inter-valley anti-Hund's coupling and is less suppressed than $U$ by the Kondo screening near a Mott insulator. Additionally, we also considered an intra-orbital Hund's coupling $J_{\rm H}$ that originates from the on-site repulsion of a carbon atom. Under a reasonable approximation of the realistic model, we prove that the renormalized local interaction between quasi-particles must have a pairing (negative) channel in a doped correlated insulator at $ν=\pm(2+δν)$, albeit the bare interaction is positive definite. The proof is non-perturbative and based on exact asymptotic behaviors of the vertex function imposed by Ward identities. Existence of an optimal $U$ for superconductivity is predicted. We also analyzed the pairing symmetry. In a large area of the parameter space of $J_{\rm A}$, $J_{\rm H}$, the ground state has a nematic $d$-wave singlet pairing, which, however, can lead to a $p$-wave-like nodal structure due to the Berry's phase on Fermi surfaces (or Euler obstruction).

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑