We provide a systemic theory to entangle excitons with microcavity photons. This is realized by adopting an exciton-optomechanics system and introducing a nonlinear dispersive interaction with a mechanical oscillator. We show that when either the exciton and cavity modes in the weak-coupling regime, or the two exciton-polariton modes in the strong-coupling regime, are respectively resonant with the optomechanical Stokes and anti-Stokes sidebands, entanglement between excitons and cavity photons, or between two exciton polaritons, can be established. The entanglement is in the steady state and can potentially be achievable at room temperature. In both cases, genuine tripartite entanglement is shown to be present.
We present two novel schemes to generate photon polarization entanglement via single electron spins confined in charged quantum dots inside microcavities. One scheme is via entangled remote electron spins followed by negatively-charged exciton emissions, and another scheme is via a single electron spin followed by the spin state measurement. Both schemes are based on giant circular birefringence and giant Faraday rotation induced by a single electron spin in a microcavity. Our schemes are deterministic and can generate an arbitrary amount of multi-photon entanglement. Following similar procedu…
Semiconductor quantum dots (known as artificial atoms) hold great promise for solid-state quantum networks and quantum computers. To realize a quantum network, it is crucial to achieve light-matter entanglement and coherent quantum-state transfer between light and matter. Here we present a robust photon-spin entangling gate with high fidelity and high efficiency (up to 50 percent) using a charged quantum dot in a double-sided microcavity. This gate is based on giant circular birefringence induced by a single electron spin, and functions as an optical circular polariser which allows only one ci…
We study the hybrid exciton-polaritons in a bad microcavity containing the organic and inorganic quantum wells. The corresponding polariton states are given. The analytical solution and the numerical result of the stationary spectrum for the cavity field are finished
In this work we have studied the quantum statistical properties of the photon emitted from a driven microcavity embedded with a single armchair-edged graphene nanoribbon (GNR). The system is coherently pumped with weak laser amplitude. Analytical expressions are derived in both strong and weak coupling regimes and the nonclassical proprieties of the emitted field have been investigated. Furthermore, it is concluded that this excitonic system presents several statistical similarities to the atomic system, in particular for the bad-cavity and good-cavity limits in the weak laser amplitude regime…
We present experimental observations of a non-resonant dynamic Stark shift in strongly coupled microcavity quantum well exciton-polaritons - a system which provides a rich variety of solid-state collective phenomena. The Stark effect is demonstrated in a GaAs/AlGaAs system at 10K by femtosecond pump-probe measurements, with the blue shift approaching the meV scale for a pump fluence of 2 mJcm^-2 and 50 meV red detuning, in good agreement with theory. The energy level structure of the strongly coupled polariton Rabi-doublet remains unaffected by the blue shift. The demonstrated effect should al…
We investigate exciton emission of quantum well embedded in a semiconductor microcavity. The analytical expressions of the light intensity for the cases of excitonic number state and coherent state are presented by using secular approximation. Our results show that the effective exciton-exciton interaction leads to the appearance of collapse and revival of the light intensity. The revival time is twice compared the coherent state case with that of the number state. The dissipation of the exciton-polariton lowers the revival amplitude but does not alter the revival time. The influences of the d…
A novel, optimized numerical method of modeling of an exciton-polariton superfluid in a semiconductor microcavity was proposed. Exciton-polaritons are spin-carrying quasiparticles formed from photons strongly coupled to excitons. They possess unique properties, interesting from the point of view of fundamental research as well as numerous potential applications. However, their numerical modeling is challenging due to the structure of nonlinear differential equations describing their evolution. In this paper, we propose to solve the equations with a modified Runge--Kutta method of 4th order, fu…
In this paper we introduce and analyze a new system design for quantum-dot-based qubits that simultaneously supports scalable one-qubit and two-qubit gates, and single-shot qubit measurement. All three key processes (one-qubit gates, two-qubit gates, and qubit measurement) rely on the interaction between the electron in each quantum dot and exciton-polaritons formed in a quantum well situated near the quantum dots. A key novel feature of our proposed system is the use of polariton traps, which we show enhances the quantum-dot--quantum-well interaction by a factor of 10 and consequently results…
We report on the observation of the strong coupling regime between a single GaAs quantum dot and a microdisk optical mode. Photoluminescence is performed at various temperatures to tune the quantum dot exciton with respect to the optical mode. At resonance, we observe an anticrossing, signature of the strong coupling regime with a well resolved doublet. The Vacuum Rabi splitting amounts to 400 μeV and is twice as large as the individual linewidths.
We present a detailed analysis of exciton-photon interaction in a microcavity made out of a photonic crystal slab. Here we have analyzed a disk-like quantum dot where an exciton is formed. Excitonic eigen-functions in addition to their eigen-energies are found through direct matrix diagonalization, while wave functions corresponding to unbound electron and hole are chosen as the basis set for this procedure. In order to evaluate these wave functions precisely, we have used Luttinger Hamiltonian in the case of hole while ignoring bands adjacent to conduction band for electron states. After anal…
We investigate the possibility of creating X-waves, or localized wave packets, in resonantly excited exciton-polariton superfluids. We demonstrate the existence of X-wave traveling solutions in the coupled exciton-photon system past the inflection point, where the effective mass of lower polaritons is negative in the direction perpendicular to the wavevector of the pumping beam. Contrary to the case of bright solitons, X-waves do not require nonlinearity for sustaining their shape. Nevertheless, we show that nonlinearity is important for their dynamics, as it allows for their spontaneous forma…
We analyze the entanglement between two matter modes in a hybrid quantum system consists of a microcavity, a quantum well, and a mechanical oscillator. Although the exciton mode in the quantum well and the mechanical oscillator are initially uncoupled, their interaction through the microcavity field results in an indirect exciton-mode--mechanical-mode coupling. We show that this coupling is a Fano-Agarwal-type coupling induced by the decay of the exciton and the mechanical modes caused by the leakage of photons through the microcavity to the environment. Using experimental parameters and for s…
We propose and characterize a two-photon emitter in a highly polarised, monochromatic and directional beam, realized by means of a quantum dot embedded in a linearly polarized cavity. In our scheme, the cavity frequency is tuned to half the frequency of the biexciton (two excitons with opposite spins) and largely detuned from the excitons thanks to the large biexciton binding energy. We show how the emission can be Purcell enhanced by several orders of magnitude into the two-photon channel for available experimental systems.
Controlled non-local energy and coherence transfer enables light harvesting in photosynthesis and non-local logical operations in quantum computing. The most relevant mechanism of coherent coupling of distant qubits is coupling via the electromagnetic field. Here, we demonstrate the controlled coherent coupling of spatially separated excitonic qubits via the photon mode of a solid state microresonator. This is revealed by two-dimensional spectroscopy of the sample's coherent response, a sensitive and selective probe of the coherent coupling. The experimental results are quantitatively describe…
We consider a semiconductor quantum well in a microcavity driven by coherent light and coupled to a squeezed vacuum reservoir. By systematically solving the pertinent quantum Langevin equations in the strong coupling and low excitation regimes, we study the effect of exciton-photon detuning, external coherent light, and the squeezed vacuum reservoir on vacuum Rabi splitting and on quantum statistical properties of the light emitted by the quantum well. We show that the exciton-photon detuning leads to a shift in polariton resonance frequencies and a decrease in fluorescence intensity. We also …
We show theoretically that entangled photon pairs can be produced on demand through the biexciton decay of a quantum dot strongly coupled to the modes of a photonic crystal. The strong coupling allows to tune the energy of the mixed exciton-photon (polariton) eigenmodes, and to overcome the natural splitting existing between the exciton states coupled with different linear polarizations of light. Polariton states are moreover well protected against dephasing due to their lifetime ten to hundred times shorter than that of a bare exciton. Our analysis shows that the scheme proposed can be achiev…
Excitonic transitions offer a possible route to ultrafast optical spin manipulation in coupled nanostructures. We perform here a detailed study of the three principal exciton-mediated decoherence channels for optically-controlled electron spin qubits in coupled quantum dots: radiative decay of the excitonic state, exciton-phonon interactions, and Landau-Zener transitions between laser-dressed states. We consider a scheme to produce an entangling controlled-phase gate on a pair of coupled spins which, in its simplest dynamic form, renders the system subject to fast decoherence rates associated …
We study the photon emission from a quantum dot embedded in a microcavity. Incoherent pumping of its excitons and biexciton provokes the emission of leaky and cavity modes. By solving a master equation we obtain the correlation functions required to compute the spectrum and the relative efficiency among the emission of pairs and single photons. A quantum regime appears for low pumping and large rate of emission. By means of a post-selection process, a two beams experiment with different linear polarizations could be performed producing a large polarization entanglement visibility precisely in …
We investigate the strong coupling regime of a self-assembled quantum dot in a tunable microcavity with dark-field laser spectroscopy. The high quality of the spectra allows the lineshapes to be analyzed revealing subtle quantum interferences. Agreement with a model calculation is achieved only by including exciton dephasing which reduces the cooperativity from a bare value of 9.0 to the time-averaged value 5.5. In the pursuit of high cooperativity, besides a high-Q and low mode-volume cavity, we demonstrate that equal efforts need to be taken towards lifetime-limited emitter linewidths.
Entanglement generation in microcavity exciton-polaritons is an interesting application of the peculiar properties of these half-light/half-matter quasiparticles. In this paper we theoretically investigate their luminescence dynamics and entanglement formation in single, double, and triple cavities. We derive general expressions and selection rules for polariton-polariton scattering. We evaluate a number of possible parametric scattering schemes in terms of entanglement, and identify the ones that are experimentally most promising.
Exciton-polariton solitons are strongly nonlinear quasiparticles composed of coupled exciton-photon states due to the interaction of light with matter. In semiconductor microcavity systems such as semiconductor micro and nanowires, polaritons are characterized by a negative mass which when combined with the repulsive nonlinear exciton-exciton interaction, leads to the generation of bright polariton solitons. In this work we investigate the dynamics of bright exciton-polariton solitons in a finite-size microcavity waveguide, for which radiative losses are assumed balanced by the external pumpin…
Two-photon absorption (TPA) allows accessing dark states of matter otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA driven condensation of strongly-coupled light-matter exciton-polaritons can enable new solid-state quantum simulations of dark state-condensate interactions, and was predicted to stimulate THz emission. Here, we report the first observation of two-photon pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the…
We investigate theoretically two-photon processes in a microcavity containing one quantum dot in the strong coupling regime. The cavity mode can be tuned to resonantly drive the two-photon transition between the ground and the biexciton states, while the exciton states are far-off resonance due to the biexciton binding energy. We study the steady state of the quantum dot and cavity field in presence of a continuous incoherent pumping. We identify the regime where the system acts as two-photon emitter and discuss the feasibility and performance of realistic single quantum dot devices for two-ph…
We discuss the generation of two-atom entanglement inside a resonant microcavity under stimulated emission (STE) interaction. The amount of entanglement is shown based on different atomic initial state. For each kind of intial state, we obtain the entanglement period and the entanglement critical point, which are found to deeply depend on driving field density. In case of atomic state $| ee >$, the entanglement can be induced due to STE. In case of atomic state $| eg >$, there is a competition between driving field indued entanglement and STE induced entanglement. When two atoms are initially …
Narrow dark resonances associated with electromagnetically induced transparency play a key role in enhancing photon-photon interactions. The schemes realized to date relied on the existence of long-lived atomic states with strong van der Waals interactions. Here, we show that by placing an atomically thin semiconductor with ultra-fast radiative decay rate inside a \textcolor{black}{0D} cavity, it is possible to obtain narrow dark or bright resonances in transmission whose width could be much smaller than that of the cavity and bare exciton decay rates. While breaking of translational invarianc…
We propose a quantum non-demolition method - giant Faraday rotation - to detect a single electron spin in a quantum dot inside a microcavity where negatively-charged exciton strongly couples to the cavity mode. Left- and right-circularly polarized light reflected from the cavity feels different phase shifts due to cavity quantum electrodynamics and the optical spin selection rule. This yields giant and tunable Faraday rotation which can be easily detected experimentally. Based on this spin-detection technique, a scalable scheme to create an arbitrary amount of entanglement between two or more …
We study the evolution of quantum entanglement during exciton energy transfer (EET) in a network model of the Fenna-Matthews-Olson (FMO) complex, a biological pigment-protein complex involved in the early steps of photosynthesis in sulphur bacteria. The influence of Markovian, as well as spatially and temporally correlated (non-Markovian) noise on the generation of entanglement across distinct chromophores (site entanglement) and different excitonic eigenstates (mode entanglement) is studied for different injection mechanisms, including thermal and coherent laser excitation. Additionally, we s…
