Collective spontaneous emission occurs when multiple quantum emitters decay into common radiation modes, resulting in enhanced or suppressed emission. Here, we find the quantum state of light collectively emitted from emitters exhibiting quantum correlations. We unveil under what conditions the quantum correlations are not lost during the emission but are instead transferred to the output light. Under these conditions, the inherent nonlinearity of the emitters can be tailored to create desired photonic states in the form of traveling single-mode pulses, such as Gottesman-Kitaev-Preskill and Schrödinger-cat states. To facilitate such predictions, our work reveals the multi-mode nature of collective spontaneous emission, capturing the role of the emitters' positions, losses, interactions, and beyond-Markov dynamics on the emitted quantum state of light. We present manifestations of these effects in different physical systems, with examples in cavity-QED, waveguide-QED, and atomic arrays. Our findings suggest new paths for creating and manipulating multi-photon quantum light for bosonic codes in continuous-variable-based quantum computation, communications, and sensing.
The q-deformation of a single quantized radiation mode interacting with a collection of two level atoms is introduced, analysing its effects on the cooperative behavior of the system.
We explore the spontaneous generation and decay of quantum correlations between two identical atoms coupled to a common Markovian environment in the presence of electromagnetic field modes. For this purpose, we analyze the dynamics of quantum correlations by employing the concurrence, the trace quantum discord and the local quantum uncertainty, for collective Dicke states. It is shown that the collective damping and dipole-dipole interaction plays a key role in enhancing non-classical correlations during the process of intrinsic decoherence. The quantum correlations can be maintained over a lo…
We describe an experimentally straightforward method for preparing an entangled W state of up to 100 qubits. Our repeat-until-success protocol relies on detection of single photons from collective spontaneous emission in free space. Our method allows entanglement preparation in a wide range of qubit implementations that lack entangling qubit-qubit interactions. We give detailed numerical examples for entanglement of neutral atoms in optical lattices and of nitrogen-vacancy centres in diamond. The simplicity of our method should enable preparation of mesoscopic entangled states in a number of p…
A universal and fault tolerant scheme for quantum computation is proposed which utilizes a class of error correcting codes that is based on the detection of spontaneous emission (of, e.g., photons, phonons, and ripplons). The scheme is compatible with a number of promising solid-state and quantum-optical proposals for quantum computer implementations, such as quantum dots in cavities, electrons on helium, and trapped ions.
Considering the paradigmatic case of a cloud of two-level atoms interacting through common vacuum modes, we show how cooperative spontaneous emission, which is at the origin of superradiance, leads the system to long-lived entangled states at late times. These subradiant modes are characterized by an entanglement between all particles, independently of their geometrical configuration. While there is no threshold on the interaction strength necessary to entangle all particles, stronger interactions lead to longer-lived entanglement.
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
The creation of single collective excitations in atomic ensembles via spontaneous Raman emission plays a key role in several quantum communication protocols, starting with the seminal DLCZ protocol [L.-M.Duan, M.D. Lukin, J.I. Cirac, and P. Zoller, Nature {\bf 414}, 413 (2001).] This process is usually analyzed theoretically under the assumptions that the write laser pulse inducing the Raman transition is far off-resonance, and that the atomic ensemble is only homogeneously broadened. Here we study the impact of near-resonance excitation for inhomogeneously broadened ensembles on the collectiv…
Recent work has shown that collective single photon emission from an ensemble of resonate two-level atoms, i.e. single photon superradiance, is a rich field of study. The present paper addresses the flip side of superradiance, i.e. subradiance. Single photon subradiant states are potentially stable against collective spontaneous emission and can have ultrafast readout. In particular it is shown how many atom collective effects provide a new way to control spontaneous emission by preparing and switching between subradiant and superradiant states.
The effective Hamiltonian describing resonant interaction of an ensemble of identical quantum particles with a photon-free vacuum electromagnetic field has been obtained with allowance for the second-order terms over the coupling constant (the Stark interaction) by means of the perturbation theory on the basis of the unitary transformation of the system quantum state. It has been shown that in the Markov approximation the effective Hamiltonian terms of the first-order coupling constant are represented as the quantum Wiener process, whereas the second-order terms are expressed by the quantum Po…
We derive a markovian master equation for the internal dynamics of an ensemble of two-level atoms including all effects related to the quantization of their motion. Our equation provides a unifying picture of the consequences of recoil and indistinguishability of atoms beyond the Lamb-Dicke regime on both their dissipative and conservative dynamics, and applies equally well to distinguishable and indistinguishable atoms. We give general expressions for the decay rates and the dipole-dipole shifts for any motional states, and we find closed-form formulas for a number of relevant states (Gaussia…
We consider spontaneous emission of two two-level atoms interacting with vacuum fluctuations. We study the process of disentanglement in this system and show the possibility of changing disentanglement time by local operations.
We study the collective radiative decay of a system of two two-level emitters coupled to a one-dimensional waveguide in a regime where their separation is comparable to the coherence length of a spontaneously emitted photon. The electromagnetic field propagating in the cavity-like geometry formed by the emitters exerts a retarded backaction on the system leading to strongly non-Markovian dynamics. The collective spontaneous emission rate of the emitters exhibits an enhancement or inhibition beyond the usual Dicke super- and sub-radiance due to a self-consistent coherent time-delayed feedback.
The local-field renormalization of the spontaneous emission rate in a dielectric is explicitly obtained from a fully microscopic quantum-electrodynamical, many-body derivation of Langevin-Bloch operator equations for two-level atoms embedded in an absorptive and dispersive, linear dielectric host. We find that the dielectric local-field enhancement of the spontaneous emission rate is smaller than indicated by previous studies.
Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a π-pulse, resulting in amplified spontaneous emission. The application of a second π-pulse leads to a coherent echo of the amplified spontaneous emission that is correlated in both amplitude and phase. For small optical thicknesses, we see evidence that the amplified spontaneous emission and its echo are entangled.
As one of the central topics in quantum optics, collective spontaneous emission such as superradiance has been realized in a variety of systems. This work proposes an innovative scheme to coherently control collective emission rates via a self-interference mechanism in a nonlinear waveguide setting. The self-interference is made possible by photon backward scattering incurred by quantum scatterers in a waveguide working as quantum switches. Whether the interference is constructive or destructive is found to depend strongly on the distance between the scatterers and the emitters. The interferen…
The detrimental effect of spontaneous emission on the performance of control schemes designed to achieve population inversion between the ground state and a highly excited atomic state are studied using computer simulations.
We demonstrate how spontaneous emission in a cavity can be controlled by the application of a dc field. The method is specially suitable for Rydberg atoms. We present a simple argument for the control of emission.
Two recent experiments studying the potential effect of entanglement on the emission properties of excited atoms produced in molecular photodissociation have been interpreted in conflicting ways. We present a theoretical analysis of the problem, showing that the experimental results can be explained by a combination of three processes: entanglement, exchange effects associated with the identical nature of the atoms and disentanglement by spontaneous emission. According to our approach these experiments provide the first verification of the phenomenon of disentanglement by spontaneous emission.
Amplified spontaneous emission is usually treated as an incoherent noise process. Recent theoretical and experimental work using rephasing optical pulses has shown that rephased amplified spontaneous emission (RASE) is a potential source of wide bandwidth time-delayed entanglement. Due to poor echo efficiency the plain RASE protocol doesn't in theory achieve perfect entanglement. Experiments done to date show a very small amount of entanglement at best. Here we show that rephased amplified spontaneous emission can, in principle, produce perfect multimode time-delayed two mode squeezing when th…
We study quantum teleportation via two two-level atoms coupled collectively to a multimode vacuum field and prepared initially in different atomic states. We concentrated on influence of the spontaneous emission, collective damping and dipole-dipole interaction of the atoms on fidelity dynamics of quantum teleportation and obtained the region of spatial distance between the two atoms over which the state can be teleported nonclassically. Moreover, we showed through concrete examples that entanglement of the channel state is the prerequisite but not the only essential quantity for predicting th…
The production of single photons using rephased amplified spontaneous emission is examined. This process produces single photons on demand with high efficiency by detecting the spontaneous emission from an atomic ensemble, then applying a population-inverting pulse to rephase the ensemble and produce a photon echo of the spontaneous emission events. The theoretical limits on the efficiency of the production are determined for several variants of the scheme. For an ensemble of uniform optical density, generating the initial spontaneous emission and its echo using transitions of different streng…
We investigate the quantum dynamics of a driven two-level system under spontaneous emission and its application in clock frequency estimation. By using a Lindblad equation to describe the system, we analytically obtain its exact solutions, which show three different regimes: Rabi oscillation, damped oscillation and overdamped decay. From the analytical solutions, we explore how the spontaneous emission affects the clock frequency estimation. We find that, under a modest spontaneous emission rate, the transition frequency can still be inferred from the Rabi oscillation. Our results provide pote…
Modification of spontaneous decay in space and time is a central topic of quantum physics. It has been predominantly investigated in the context of cavity quantum electrodynamics (QED), gaining new interest recently in the domain of nano-optics. Beyond cavity-QED, spontaneous emission may be modified also in free space due to correlations among the photon emitters, a phenomenon known as super- and sub-radiance. Correlations may stem either from direct interactions between the particles, from long-range exchange of photons, or by measuring single photons in a common mode. Yet, the genuine spati…
We study the generation of spin-squeezing in arrays of long-lived dipoles subject to collective emission, coherent drive, elastic interactions, and spontaneous emission. Counter-intuitively, it is found that the introduction of spontaneous emission leads to an enhancement of the achievable spin-squeezing, relative to that which emerges in the steady-state of the purely collective dynamics for the same model parameters. This behavior is connected to the dynamical self-tuning of the system through a dissipative phase transition that is present in the collective system alone. Our findings will be…
We present a dissipative protocol to engineer two $^{87}Rb$ atoms into a form of three-dimensional entangled state via spontaneous emission. The combination of coupling between ground states via microwave fields and dissipation induced by spontaneous emission make the current scheme deterministic and a stationary entangled state can always be achieved without state initialization. Moreover, this scheme can be straightforwardly generalized to preparation of an $N$-dimensional entangled state in principle.
An electronically excited atom or molecule located outside but near a planar optical waveguide can decay by spontaneous emission of a photon into a guided mode of the waveguide. We outline a QED theory for calculating the probability for this process and describe general physical insights from that theory. A couple of representative examples are discussed in detail.
We study evolution of entanglement of two two-level atoms in the presence of dissipation caused by spontaneous emission. We find explicit fromulas for the amount of entanglement as a function of time, in the case of destruction of the initial entanglement and possible creation of a transient entanglement between atoms. We also discuss how spontaneous emission influences nonlocality of states expressed by violation of Bell - CHSH inequality. It is shown that evolving system very quickly becomes local, even if entanglement is still present or produced.
It has been shown that strong Stark interaction of a quantum particle with a vacuum electromagnetic field reduces the speed of the one-quantum spontaneous radiation and leads to additional shift of frequency of radiation transition.
We show that under the influence of pure vacuum noise two entangled qubits become completely disentangled in a finite time, and in a specific example we find the time to be given by $\ln \Big(\frac{2 +\sqrt 2}{2}\Big)$ times the usual spontaneous lifetime.
We investigate the spontaneous emission from an inverted Y-type atomic system coupled by three coherent fields. We use the Schrödinger equation to calculate the probability amplitudes of the wave function of the system and derive an analytical expression of the spontaneous emission spectrum to trace the origin of the spectral features. Quantum interference effects, such as the spectral line narrowing, spectrum splitting and dark resonance are observed. The number of spectral components, the spectral linewidth, and relative heights can be very different depending on the physical parameters. A v…
We study two distinct multi-level atomic models in which one transition is coupled to a Markovian reservoir, while another linked transition is coupled to a non-Markovian reservoir. We show that by choosing appropriately the density of modes of the non-Markovian reservoir the spontaneous emission to the Markovian reservoir is greatly altered. The existence of `dark lines' in the spontaneous emission spectrum in the Markovian reservoir due to the coupling to specific density of modes of the non-Markovian reservoir is also predicted.
Quasi-stationary states of the quantum system in the driving resonant field are considered without rotating wave approximation. Conditions under which the spontaneous emission could be suppressed in this system are investigated in the special case when the frequency of the driving field is essentially less than the frequency of spontaneous emission. It is shown that the characteristic parameters of the effect are substantially changed in comparison with the results corresponding to RWA. The real physical system for which the considered effects could be observed is described.
We report an interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms that are coherently excited by a short laser pulse. The ensembles are Erbium ions doped into two LiNbO3 crystals with channel waveguides, which are placed in the two arms of a Mach-Zehnder interferometer. The light that is spontaneously emitted after the excitation pulse shows first-order interference. By a strong collective enhancement of the emission, the atoms behave as ideal two-level quantum systems and no which-path information is left in the atomic ensembles after emissi…
We study theoretically the effects of dissipation on the performances of a variational quantum algorithm used to approximately solve a combinatorial optimization problem, the Maximum Independent Set, on a platform of neutral atoms. We take a realistic model of dissipation with spontaneous emission, and show numerically that the detrimental effects of these incoherent processes are spontaneously attenuated by the variational nature of the procedure. We furthermore implement an alternative optimization scheme recently proposed, where one uses the expected shortfall of the mean energy as the obje…
We present a quantum error correcting code that is invariant under the conditional time evolution between spontaneous emissions and which can correct for one general error. The code presented here generalizes previous error correction codes in that not all errors lead to different error syndromes. This idea may lead to shorter codes than previously expected.
We consider local time evolution given by spontaneous emission in the system of independent two-level atoms. It is shown that all classically correlated initial states are driven into the states with transient non-zero quantum discord. Thus local creation of genuine quantum correlations can be observed in a simple physical system of non-interacting atoms which are not completely isolated from the environment.
We propose two quantum error correction schemes which increase the maximum storage time for qubits in a system of cold trapped ions, using a minimal number of ancillary qubits. Both schemes consider only the errors introduced by the decoherence due to spontaneous emission from the upper levels of the ions. Continuous monitoring of the ion fluorescence is used in conjunction with selective coherent feedback to eliminate these errors immediately following spontaneous emission events, and the conditional time evolution between quantum jumps is removed by symmetrizing the quantum codewords.
Here we discuss an effect of dephasing induced by a weak gravitational field on the collective radiation dynamics of an atomic system in timed single-photon Dicke states. We show that a photon absorbed by the stationary system of randomly placed stationary atoms is no longer spontaneously emitted in the direction of the impinging photon. Gravity leads to broadening of the angular distribution of emission.
We derive spontaneous emission rate and line shift for two-level atoms coupled to the radiation field using causal perturbation theory. In this approach, employing the theory of distribution splitting prevents the occurrence of divergent integrals. Our method confirms the result for atomic decay rate but suggests that the cutoff frequency for the atomic line shift is determined by the atomic mass, rather than Bohr radius or electron mass.
We discuss a simple example demonstrating that spontaneous emission from "space-time-superposed" atomic center-of-mass wave packets is nontrivially and time-dependent modified with respect to the standard dipole-pattern typical of "space-superposed" wave packets. Our approach provides an approximate description of a nonsimultaneous interaction of electromagnetic field with different parts of a wave packet.
We compute the modification in the spontaneous emission rate for a two-level atom when it is located between two parallel plates of different nature: a perfectly conducting plate $(ε\to \infty)$ and an infinitely permeable one $(μ\to \infty)$. We also discuss the case of two infinitely permeable plates. We compare our results with those found in the literature for the case of two perfectly conducting plates.
We present a fully quantum mechanical treatment of optically rephased photon echoes. These echoes exhibit noise due to amplified spontaneous emission, however this noise can be seen as a consequence of the entanglement between the atoms and the output light. With a rephasing pulse one can get an "echo" of the amplified spontaneous emission, leading to light with nonclassical correlations at points separated in time, which is of interest in the context of building wide bandwidth quantum repeaters. We also suggest a wideband version of DLCZ protocol based on the same ideas.
The problem of spontaneous emission is studied by a direct computer simulation of the dynamics of a combined system: atom + radiation field. The parameters of the discrete finite model, including up to 20k field oscillators, have been optimized by a comparison with the exact solution for the case when the oscillators have equidistant frequencies and equal coupling constants. Simulation of the effect of multi-pulse sequence of phase kicks and emission by a pair of atoms shows that both the frequency and the linewidth of the emitted spectrum could be controlled.
We demonstrate strong confinement of the optical field by depositing a micron sized metallic disk on a planar interferential mirror. Zero dimensional Tamm plasmon modes are evidenced both experimentally and theoretically, with a lateral confinement limited to the disk area and strong coupling to TE polarized fields. Single quantum dots deterministically coupled to these modes are shown to experience acceleration of their spontaneous emission when spectrally resonant with the mode. For quantum dots spectrally detuned from the confined Tamm Plasmon mode, an inhibition of spontaneous emission by …
Non dispersive electronic Rydberg wave packets may be created in atoms illuminated by a microwave field of circular polarization. We discuss the spontaneous emission from such states and show that the elastic incoherent component (occuring at the frequency of the driving field) dominates the spectrum in the semiclassical limit, contrary to earlier predictions. We calculate the frequencies of single photon emissions and the associated rates in the "harmonic approximation", i.e. when the wave packet has approximately a Gaussian shape. The results agree well with exact quantum mechanical calculat…
We study an array of dissipative tunnel-coupled cavities, each interacting with an incoherently pumped two-level emitter. For cavities in the lasing regime, we find correlations between the light fields of distant cavities, despite the dissipation and the incoherent nature of the pumping mechanism. These correlations decay exponentially with distance for arrays in any dimension but become increasingly long ranged with increasing photon tunneling between adjacent cavities. The interaction-dominated and the tunneling-dominated regimes show markedly different scaling of the correlation length whi…
We have measured the variation of the spontaneous emission rate with polarization for self-assembled single quantum dots in two-dimensional photonic crystal membranes. We observe a maximum anisotropy factor of 6 between the decay rates of the two bright exciton states. This large anisotropy is attributed to the substantially different projected local density of optical states for differently oriented dipoles in the photonic crystal.
We study the probe spectrum of light generated by spontaneous emission into the mode of a cavity QED system. The probe spectrum has a maximum on-resonance when the number of inverted atoms for an input drive is maximal. For a larger number of atoms N, the maximum splits and develops into a doublet, but its frequencies are different from those of the so-called vacuum Rabi splitting.
We study the collective spontaneous emission of three identical two-level atoms initially prepared in the excited states by measuring Glauber's third-order photon correlation function. Assuming two atoms at sub-wavelength distance from each other such that they are subject to the dipole-dipole interaction while the third one is located several wavelengths away, we observe super- and subradiant decay alike, depending on the direction of observation. Unlike the case where no remote atom is introduced or no conditional measurements are performed, the spontaneous emission behavior of the condition…
We revisit the back-action of emitted photons on the motion of the relative position of two cold atoms. We show that photon recoil resulting from the spontaneous emission can induce the localization of the relative position of the two atoms through the entanglement between the spatial motion of individual atoms and their emitted photons. The result provides a more realistic model for the analysis of the environment-induced localization of a macroscopic object.
We present a very simple model of a spontaneous emission from a two-level atom, interacting with a field of a finite number of states. Such a process is often said to occur because of the large number of equally-probable states of environment. We show that in our model increasing the number of field states may and may not cause a practically permanent emission, depending on the details of the model. We also describe how irreversibility emerges with growing number of states. Mathematical tools are reduced to a necessary minimum and hopefully can be well understood by undergraduate students.
We investigate decoherence of quantum superpositions induced by gravitational time dilation and spontaneous emission between two atomic levels. It has been shown that gravitational time dilation can be an universal decoherence source. Here, we consider decoherence induced by gravitational time dilation only in the situation of spontaneous emission. Then, we obtain that the coherence of particle's position state depends on reference frame due to the time dilation changing the distinguishability of emission photon from two positions of particle. Changing the direction of light field can also res…
In a previous paper [B. Deb and G. S. Agarwal, Phys. Rev. A 90, 063417 (2014)], it was theoretically shown that, magneto-optical manipulation of low energy scattering resonances and atom-molecule transitions could lead to the formation of a bound state in continuum (BIC), provided there is no spontaneous emission. We find that even an exceedingly small spontaneous decay from exited molecular states can spoil the BIC. In this paper, we show how to circumvent the detrimental effect of spontaneous emission by making use of vacuum-induced coherence (VIC) which results in the cancellation or suppre…
