Accelerating a free electron to high energy forms the basis for studying particle and nuclear physics. Here it is shown that wavefunction of such an energetic electron can be further manipulated with femtosecond intense lasers. During the scattering between a high-energy electron and a strong laser pulse, we find a regime where the enormous photon spin angular momenta can be efficiently transferred to the electron orbital angular momentum (OAM). The wavefunction of the scattered electron is twisted from its initial plane-wave state to quantum vortex state. Nonlinear quantum electrodynamics (QED) theory suggests that GeV-level electrons acquire average intrinsic OAM beyond 100 h-barat laser intensities of 10^20W/cm^2 with linear scaling. These electrons emit gamma photons with double-peaked spectrum, which sets them apart from ordinary electrons. The findings demonstrate a proficient method for generating relativistic leptons with quantum vortex wavefunctions based on existing laser technology, thereby fostering a novel source for particle and nuclear physics.
Intense few cycle terahertz pulses exhibit complex non-linear behavior under interaction with heavily n-doped Si. Fast increase in the transmission of a 700 fs pulse (central frequency 1.5 THz) through the Si sample (low field transmission of 0:02 %) saturates at 8 % for the external field of 5 MV/cm and then drops twofold at 20 MV/cm. An electro-optical sampling measurements revealed formation of a single cycle terahertz pulse at this field due to formation of a thin ionized layer by the first intense oscillation of the terahertz field.
We theoretically study the generation of terahertz (THz) radiation by two-color filamentation of ultrashort laser pulses with different wavelengths. We consider wavelengths in the range from 0.6 to 10.6 $μ$m, thus covering the whole range of existing and future powerful laser sources in the near, mid and far-infrared. We show how different parameters of two-color filaments and generated THz pulses depend on the laser wavelength. We demonstrate that there is an optimal laser wavelength for two-color filamentation that provides the highest THz conversion efficiency and results in generation of e…
Energy transfer processes from a high-intensity ultrashort laser pulse to electrons in simple dielectrics, silicon, diamond, and $α$-quartz are theoretically investigated by first-principles calculations based on time-dependent density functional theory (TDDFT). Dependences on frequency as well as intensity of the laser pulse are examined in detail, making a comparison with the Keldysh theory. Although the Keldysh theory reliably reproduces the main features of the TDDFT calculation, we find some deviations between results by the two theories. The origin of the differences is examined in detai…
The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses with center frequency tunable between 2-4 THz. The coherent THz light source with pulse energy of 1.2 microjoule can be generated from a low-cost crystalline quartz pumped by an ultrashort tilted wave-front pulse. Thanks to the wide transparent spectral window and high damage threshold, our theoretical analysis and experiment show that the optical rectification…
Giant self-induced transparency of intense few-cycle terahertz pulses in n-doped silicon
给出了在n型掺杂硅（载流子浓度为$8.7\times10^{16}$ cm $^{-3}$）上进行的高场太赫兹传输实验的结果。我们使用电场强度高达3.1 MV cm $^{-1}$和脉冲持续时间为700 fs的太赫兹脉冲。在1.5- 3.1 MV cm $^{-1}$范围内，随着太赫兹电场强度的增加，$\sim$的透过率增加了90倍。
The magnitude of the topological charge of the vortex of a ring-shaped pulse is found to be limited by the squared mean frequency of the pulse spectrum at the ring relative to its variance. This limitation implies a upper bound to the orbital angular momentum carried by a pulse, and a lower bound to the duration for a pulse to carry any orbital angular momentum.
Propagation of intense few-cycle laser pulse in a telecommunication-type optical fiber: analysis of the error introduced by the unidirectional approximation
Strong mid-infrared light-matter interaction has attracted extensive attention as it opens up new frontiers in nonlinear optics. Here we observe through simulations a novel aspect of mid-infrared pulse dynamics in a high-pressure gas-filled capillary, where a pulse with a power well below the critical power for Kerr self-focusing undergoes an astonishing rise of the peak intensity following an extremely efficient spectral broadening. This intensity enhancement is attributed to the Kerr-induced focusing of the supercontinuum. Our study provides an interesting perspective for controlling the las…
It has been recently shown that the orbital angular momentum (OAM) and temporal degrees of freedom in ultrafast (few-cycle) vortices are coupled. This coupling manifests itself with different effects in different parts of the vortex, as has been shown for the ring surrounding the vortex where the pulse energy is maximum, and also in the immediate vicinity of the vortex center. In may applications, however, the ring of maximum energy is not of primary interest, but that where the pulse peak intensity is maximum, which is particularly true in nonlinear optics applications such as the experiments…
In this paper we perform a fusion between two important theoretical methodologies, one related to the Frozen Wave beams, which are non-diffracting beams whose longitudinal intensity pattern can be chosen a priori in an medium (absorbing or not), and the other related to the Airy-Type pulses, which are pulses resistant to dispersion effects in dispersive materials. As a result, a new method emerges, capable of providing vortex pulses resistant to three concomitant effects, i.e.: diffraction, dispersion and attenuation; while concurrently the spatial variation of the wave intensity along its axi…
Using an affordable ytterbium laser with sub-mJ of energy combined with a novel pulse compression technique, we demonstrate an extremely competitive state-of-the-art terahertz (THz) source with 53 mW of average power and 310 kV/cm at focus from the tilted-pulse front pumping scheme in lithium niobate at room temperature. Key points of this demonstration include the use of a pump pulse duration of 280 fs in combination with an echelon mirror. Our results present unmatched combined characteristics and are highly competitive with the existing THz sources pumped at the mJ range. This demonstration…
Sources of intense, ultra-short electromagnetic pulses enable applications such as attosecond pulse generation, control of electron motion in solids and the observation of reaction dynamics at the electronic level. For such applications both high-intensity and carrier envelope phase~(CEP) tunability are beneficial, yet hard to obtain with current methods. In this work we present a new scheme for generation of isolated CEP-tunable intense sub-cycle pulses with central frequencies that range from the midinfrared to the ultraviolet. It utilizes an intense laser pulse which drives a wake in a plas…
Ionization is a fundamental process in intense laser-matter interactions, and is known to cause plasma defocusing and intensity clamping. Here, we investigate theoretically the propagation dynamics of an intense laser pulse in a helium gas jet in the ionization saturation regime, and we find that the pulse undergoes self-focusing and self-compression through ionization-induced reshaping, resulting in a manyfold increase in the laser intensity. This unconventional behavior is associated with the spatiotemporal frequency variation mediated by ionization and spatiotempral coupling. Our results il…
A new physical mechanism to achieve spin-to-orbital angular momentum conversion based on the interaction of an intense circularly polarized (CP) laser beam with a plane foil is presented and studied for the first time. It has been verified by both simulation and theoretical analysis that vortex harmonics carrying orbital angular momentum (OAM) are generated after a relativistic CP laser beam, even a Gaussian beam, impinges normally on a plane foil. The generation of this vortex harmonics is attributed to the vortex oscillation of the plasma surface driven harmonically by the vortex longitudina…
We propose a novel measurement technique capable of determining the temporal duration of an intense laser pulse directly in its focus at full intensity. We show that the electromagnetic radiation pattern emitted by an electron bunch with a temporal energy chirp colliding perpendicularly with the laser pulse exhibits a distinct dependence on the pulse's duration. As the electrons emit radiation into an angular region determined by the ratio of their instantaneous energy to the laser's local field strength, the temporal change of the electrons' energy imprints information about the laser's pulse…
We show theoretically that an intense femtosecond optical pulse incident normally on a metal surface tends to decay into a pair of counter-propagating surface plasmon-polaritons (SPPs). The interference field heats the medium periodically, which causes a periodic permittivity perturbation and resonantly amplifies the magnitudes of SPPs. The instability growth time is only 10-50 fs for typical metals at damaging laser fluences. This mechanism is promising for the interpretation of laser-induced periodic surface structures formation in a single-pulse pumping regime.
We have systematically investigated the spatial and temporal dynamics of crystallization that occurs in the phase-change material Ge2Sb2Te5 upon irradiation with an intense THz pulse. THz pump and optical probe spectroscopy revealed that Zener tunneling induces a nonlinear increase in the conductivity of the crystalline phase. This result indicates that the large electric field associated with the THz pulses causes a nonlinear increase only at the edge of the crystallized area. The electric field concentrating in this area causes a temperature increase via Joule heating, which in turn leads to…
Intense extreme-ultraviolet (XUV) pulses enable the investigation of XUV-induced nonlinear processes and are a prerequisite for the development of attosecond pump - attosecond probe experiments. While highly nonlinear processes in the XUV range have been studied at free-electron lasers (FELs), high-harmonic generation (HHG) has allowed the investigation of low-order nonlinear processes. Here we suggest a concept to optimize the HHG intensity, which surprisingly requires a scaling of the experimental parameters that differs substantially from optimizing the HHG pulse energy. As a result, we are…
Relativistic surface high harmonics have been considered a unique source for the generation of intense isolated attosecond pulses in the extreme ultra-violet (XUV) and X-ray spectral range. However, its experimental realization is still a challenging task requiring identification of the optimum conditions for the generation of isolated attosecond pulses as well as their temporal characterization. Here, we demonstrate measurements in both directions. Particularly, we have made a first step towards the temporal characterization of the emitted XUV radiation by adapting the attosecond streak camer…
