In this work, we established a novel theory for the dynamics of oscillating bubbles such as cavitation bubbles, underwater explosion bubbles, and air bubbles. For the first time, we proposed bubble dynamics equations that can simultaneously take into consideration the effects of boundaries, bubble interaction, ambient flow field, gravity, bubble migration, fluid compressibility, viscosity, and surface tension while maintaining a unified and elegant mathematical form. The present theory unifies different classical bubble equations such as the Rayleigh-Plesset equation, the Gilmore equation, and the Keller-Miksis equation. Furthermore, we validated the theory with experimental data of bubbles with a variety in scales, sources, boundaries, and ambient conditions and showed the advantages of our theory over the classical theoretical models, followed by a discussion on the applicability of the present theory based on a comparison to simulation results with different numerical methods. Finally, as a demonstration of the potential of our theory, we modeled the complex multi-cycle bubble interaction with wide ranges of energy and phase differences and gained new physical insights into inter-bubble energy transfer and coupling of bubble-induced pressure waves.
Water-immersed gold nanoparticles irradiated by a laser can trigger the nucleation of plasmonic bubbles after a delay time of a few microseconds [Wang et al., Proc. Natl. Acad. Sci. USA 122, 9253,(2018)]. Here we systematically investigated the light-vapor conversion efficiency, η, of these plasmonic bubbles as a function of the ambient pressure. The efficiency of the formation of these initial-phase and mainly water-vapor containing bubbles, which is defined as the ratio of the energy that is required to form the vapor bubbles and the total energy dumped in the gold nanoparticles before nucle…
Using a nonlinear sound wave equation for a bubbly liquid in conjunction with an equation for bubble pulsation, we predict and experimentally demonstrate the appearance of a gap in the frequency spectrum of a sound wave propagating in a cavitation cloud comprising bubbles. For bubbles with an ambient radius of 100 μm, the calculations revealed that this gap corresponds to the phenomenon of sound wave localization. For bubbles with an ambient radius of 120 μm, this spectral gap relates to a forbidden band of the sound wave. In the experiment, we observed the predicted gap in the frequency spect…
We present a direct numerical simulation (DNS) study of buoyancy driven bubbly flows in two-dimensions. We employ volume of fluid (VOF) method to track the bubble interface. To investigate spectral properties of the flow, we derive the scale-by-scale energy budget equation. We show that the Galilei number (Ga) controls different scaling regimes in the energy spectrum. For high Galilei numbers, we find the presence of an inverse energy cascade. Our study indicates that the density ratio of the bubble with the ambient fluid or the presence of coalescence between the bubbles does not alter the sc…
We consider the collapse behavior of cavitation bubbles near walls under high ambient pressure conditions. Generic configurations with different stand-off distances are investigated by numerical simulation using a fully compressible two-phase flow solver including phase change. The results show that the stand-off distance has significant effects on collapse dynamics, micro-jet formation, rebound, and maximum wall pressure. A relation between cavitation induced material damage and corresponding collapse mechanisms is obtained from pressure-impact data at the wall. We analyze the resolution depe…
In many environmental and industrial applications, the mass transfer of gases in liquid solvents is a fundamental process during the generation of bubbles for specific purposes or, vice versa, the removal of entrapped bubbles. We address the growth dynamics of a trapped slug bubble in a vertical glass cylinder under a water barrier. In the studied process, the ambient air atmosphere is replaced by a CO$_2$ atmosphere at the same or higher pressure. The asymmetric exchange of the gaseous solutes between the CO$_2$-rich water barrier and the air-rich bubble always results in net bubble growth. W…
A small, spherical bubble of high internal pressure is inserted into water at constant ambient pressure as a model of a laser-induced bubble. Its subsequent dynamics near a flat solid boundary is studied in dependence on the distance of the bubble to the boundary by numerically solving the Navier-Stokes equations with the help of the open source software environment OpenFOAM. Implemented is the finite volume method for discretization of the equations of motion and the volume of fluid method for capturing the interface between the bubble interior and exterior. The bubble contains a small amount…
To investigate the intrinsic mechanism for mixing enhancement by variable density behaviour, a canonical variable density (VD) mixing extracted from a supersonic streamwise vortex protocol, shock bubble interaction (SBI), is numerically studied and compared with a counterpart of passive scalar (PS) mixing. It is meaningful to observe that the maximum concentration decays much faster in VD SBI than in PS SBI regardless of the shock Mach number (Ma = 1.22 ~ 4). The quasi-Lamb-Oseen type velocity distribution in the PS SBI is found by analyzing the azimuthal velocity that stretches the bubble. Me…
Dynamics of vapor bubble train in flow boiling heat transfer in microchannels
State Key Laboratory of Engines, Tianjin University（天津大学内燃机燃烧学国家重点实验室）；National Industry-Education Platform of Energy Storage, Tianjin University（天津大学国家储能产教融合创新平台）
Interdisciplinary Centre of Energy Sciences, Indian Institute of Science（印度科学学院交叉能源科学中心）；Department of Mechanical Engineering, Indian Institute of Science（印度科学学院机械工程系）
Cloud cavitation causes nontrivial energy concentration and acoustic shielding in liquid, and its control is a long-standing challenge due to complex dynamics of bubble clouds. We present a new framework to study closed-loop control of cavitation through acoustic feedback. While previous approaches used empirical thresholding, we employ model-based state estimation of coherent bubble dynamics based on theory and high-performance computing. Using a pulsed ultrasound setup, we demonstrate set-point control of the pulse repetition frequency (PRF) to modulate acoustic cavitation near a solid targe…
During the operation of a seismic airgun source, a certain amount of compressed high-pressure air is released from the airgun chamber into the surrounding water, generating an expanding toroidal bubble attached to the airgun-body. The subsequent oscillations of the bubble generate low-frequency pressure waves, which are used to map the ocean subbottom, e.g., to locate oil and gas reserves. The bubble dynamic behavior and the emitted pressure waves are inevitably influenced by the airgun-body. However, the bubble-airgun-body interaction is far from well understood. This paper investigates the s…
A variety of approaches have been used to model the dynamics of a single, isolated bubble nucleated by a microsecond length high-amplitude ultrasound pulse (e.g., a histotripsy pulse). Until recently, the lack of single--bubble experimental radius vs. time data for bubble dynamics under a well-characterized driving pressure has limited model validation efforts. This study uses radius vs. time measurements of single, spherical histotripsy-nucleated bubbles in water [Wilson et al., Phys. Rev. E, 2019, 99, 043103] to quantitatively compare and validate a variety of bubble dynamics modeling approa…
Bubbles in complex fluids are often desirable, and sometimes simply inevitable, in the processing of formulated products. Bubbles can rise by buoyancy, grow or dissolve by mass transfer, and readily respond to changes in pressure, thereby applying a deformation to the surrounding complex fluid. The deformation field around a stationary, spherical bubble undergoing a change in radius is simple and localised, thus making it suitable for rheological measurements. This article reviews emerging approaches to extract information on the rheology of complex fluids by analysing bubble dynamics. The foc…
Understanding the dynamics of the micro-sized surface bubbles produced by plasmonic heating can benefit a wide range of applications like microfluidics, catalysis, micro-patterning and photo-thermal energy conversion. Usually, surface plasmonic bubbles are generated on plasmonic nano-structures pre-deposited on the surface subject to laser heating. In our studies, we have investigated the growth dynamics and movement mechanism of surface microbubbles generated in plasmonic nanoparticle (NP) suspension. In the first section, we observe much faster bubble growth rates compared to those in pure w…
Bridging scales in multiscale bubble growth dynamics with correlated fluctuations using neural operator learning
Artificial Intelligence Innovation and Incubation Institute, Fudan University（复旦大学人工智能创新与孵化研究院）；Division of Applied Mathematics, Brown University（布朗大学应用数学系）；Department of Mechanical Engineering, Clemson University（克莱姆森大学机械工程系）
Bubble dynamics and luminol emissions of cavitation in sub-millimeter-sized PFA flow tubes, submerged in an ultrasonic bath reactor, are studied at 27 kHz driving frequency. Nucleation of cavitation inside the tubes only takes place via a free interface, realized here in form of an alternating water-air slug flow. High-speed recordings show that cavitation bubbles in the water slugs often develop localized structures in form of clusters or bubble plugs, and that such structures can be seeded via a single pinch-off from the free interface. Within the structures, bubbles strongly interact and fr…
Recently, an asymptotic solution of the Rayleigh equation for an empty bubble in $N$ dimensions has been obtained. Here we give the closed--from general analytical solution of this equation. We also find the general solution of the Rayleigh equation in $N$ dimensions for the case of a gas--filled hyperspherical bubble. In addition, we include a surface tension into consideration.
