Dipolar Spin Liquid Ending with Quantum Critical Point in a Gd-based Triangular Magnet
Junsen Xiang, Cheng Su, Ning Xi, Zhendong Fu, Zhuo Chen, Hai Jin, Ziyu Chen, Zhao-Jun Mo, Yang Qi, Jun Shen, Long Zhang, Wentao Jin, Wei Li, Peijie Sun, Gang Su
备注：
7 pages and 4 figures in main text, 5 pages and 4 figures in Supplementary Materials
By performing experiment and model studies on a triangular-lattice dipolar magnet KBaGd(BO$_3$)$_2$ (KBGB), we find the highly frustrated magnet with a planar anisotropy hosts a strongly fluctuating dipolar spin liquid (DSL), which originates from the intriguing interplay between dipolar and Heisenberg interactions. The DSL constitutes an extended regime in the field-temperature phase diagram, which gets lowered in temperature as field increases and eventually ends with an unconventional quantum critical point (QCP) at $B_c\simeq 0.75$~T. Based on dipolar Heisenberg model calculations, we identify the DSL as a Berezinskii-Kosterlitz-Thouless (BKT) phase with emergent U(1) symmetry. Due to the tremendous entropy accumulation that can be related to the strong BKT and quantum fluctuations, unprecedented magnetic cooling effects are observed in the DSL regime and particularly near the QCP, making KBGB a superior dipolar coolant to commercial Gd-based refrigerants. We establish the phase diagram for triangular-lattice dipolar quantum magnets where emergent symmetry plays an essential role, and provide a basis and opens an avenue for their applications in sub-Kelvin refrigeration.
Switching magnetic texture via in-plane magnetic field in noncentrosymmetric dipolar magnets: From skyrmions to antiskyrmions and nontopological magnetic bubbles
