Strong photon-magnon coupling using a lithographically defined organic ferrimagnet
Qin Xu, Hil Fung Harry Cheung, Donley S. Cormode, Tharnier O. Puel, Huma Yusuf, Michael Chilcote, Michael E. Flatté, Ezekiel Johnston-Halperin, Gregory D. Fuchs
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31 pages preprint format with supplementary materials
We demonstrate a hybrid quantum system composed of superconducting resonator photons and magnons hosted by the organic-based ferrimagnet vanadium tetracyanoethylene (V[TCNE]$_x$). Our work is motivated by the challenge of scalably integrating an arbitrarily-shaped, low-damping magnetic system with planar superconducting circuits, thus enabling a host of quantum magnonic circuit designs that were previously inaccessible. For example, by leveraging the inherent properties of magnons, one can enable nonreciprocal magnon-mediated quantum devices that use magnon propagation rather than electrical current. We take advantage of the properties of V[TCNE]$_x$, which has ultra-low intrinsic damping, can be grown at low processing temperatures on arbitrary substrates, and can be patterned via electron beam lithography. We demonstrate the scalable, lithographically integrated fabrication of hybrid quantum magnonic devices consisting of a thin-film superconducting resonator coupled to a low-damping, thin-film V[TCNE]$_x$ microstructure. Our devices operate in the strong coupling regime, with a cooperativity as high as 1181(44) at T$\sim$0.4 K, suitable for scalable quantum circuit integration. This work paves the way for the exploration of high-cooperativity hybrid magnonic quantum devices in which magnonic circuits can be designed and fabricated as easily as electrical wires.
We propose a stabilizing mechanism for the Bose-Einstein condensation (BEC) of interacting magnons in ferrimagnets and ferromagnets. By studying the effects of the magnon-magnon interaction on the stability of the magnon BEC in a ferrimagnet and two ferromagnets, we show that the magnon BEC remains stable even in the presence of the magnon-magnon interaction in the ferrimagnet and ferromagnet with a sublattice structure, whereas it becomes unstable in the ferromagnet without a sublattice structure. This indicates that the existence of a sublattice structure is the key to stabilizing the BEC of…
Quantum fluctuations are the key concepts of quantum mechanics. Quantum fluctuations of quantum fields induce a zero-point energy shift under spatial boundary conditions. This quantum phenomenon, called the Casimir effect, has been attracting much attention beyond the hierarchy of energy scales, ranging from elementary particle physics to condensed matter physics together with photonics. However, the application of the Casimir effect to spintronics has not yet been investigated enough, particularly to ferrimagnetic thin films, although yttrium iron garnet (YIG) is one of the best platforms for…
Quantum entanglement in the motion of macroscopic objects is of significance to both fundamental studies and quantum technologies. Here we show how to entangle the mechanical vibration modes of two massive ferrimagnets that are placed in the same microwave cavity. Each ferrimagnet supports a magnon mode and a low-frequency vibration mode coupled by the magnetostrictive force. The two magnon modes are, respectively, coupled to the microwave cavity by the magnetic dipole interaction. We first generate a stationary nonlocal entangled state between the vibration mode of the ferrimagnet-1 and the m…
Recent studies show that hybrid quantum systems based on magnonics provide a new and promising platform for generating macroscopic quantum states involving a large number of spins. Here we show how to entangle two magnon modes in two massive yttrium-iron-garnet (YIG) spheres using cavity optomagnonics, where magnons couple to high-quality optical whispering gallery modes supported by the YIG sphere. The spheres can be as large as 1 mm in diameter and each sphere contains more than $10^{18}$ spins. The proposal is based on the asymmetry of the Stokes and anti-Stokes sidebands generated by the m…
We experimentally investigate magnon-polaritons, arising in ferrimagnetic resonance experiments in a microwave cavity with a tuneable quality factor. To his end, we simultaneously measure the electrically detected spin pumping signal and microwave reflection (the ferrimagnetic resonance signal) of a yttrium iron garnet (YIG) / platinum (Pt) bilayer in the microwave cavity. The coupling strength of the fundamental magnetic resonance mode and the cavity is determined from the microwave reflection data. All features of the magnetic resonance spectra predicted by first principle calculations and a…
We present a scheme to entangle two magnon modes in a cavity magnomechanical system. The two magnon modes are embodied by collective motions of a large number of spins in two macroscopic ferrimagnets, and couple to a single microwave cavity mode via magnetic dipole interaction. We show that by activating the nonlinear magnetostrictive interaction in one ferrimagnet, realized by driving the magnon mode with a strong red-detuned microwave field, the two magnon modes can be prepared in an entangled state. The entanglement is achieved by exploiting the nonlinear magnon-phonon coupling and the line…
We show how to create quantum squeezed states of magnons and phonons in a cavity magnomechanical system. The magnons are embodied by a collective motion of a large number of spins in a macroscopic ferrimagnet, and couple to cavity microwave photons and phonons (vibrational modes of the ferrimagnet) via the magnetic dipole interaction and magnetostrictive interaction, respectively. The cavity is driven by a weak squeezed vacuum field generated by a flux-driven Josephson parametric amplifier, which is essential to get squeezed states of the magnons and phonons. We show that the magnons can be pr…
We present a scheme to entangle two microwave fields by using the nonlinear magnetostrictive interaction in a ferrimagnet. The magnetostrictive interaction enables the coupling between a magnon mode (spin wave) and a mechanical mode in the ferrimagnet, and the magnon mode simultaneously couples to two microwave cavity fields via the magnetic dipole interaction. The magnon-phonon coupling is enhanced by directly driving the ferrimagnet with a strong red-detuned microwave field, and the driving photons are scattered onto two sidebands induced by the mechanical motion. We show that two cavity fie…
We present a theoretical approach to use ferro- or ferrimagnetic nanoparticles as microwave nanomagnonic cavities to concentrate microwave magnetic fields into deeply subwavelength volumes $\sim 10^{-13}$ mm$^3$. We show that the field in such nanocavities can efficiently couple to isolated spin emitters (spin qubits) positioned close to the nanoparticle surface reaching the single magnon-spin strong-coupling regime and mediate efficient long-range quantum state transfer between isolated spin emitters. Nanomagnonic cavities thus pave the way towards magnon-based quantum networks and magnon-med…
The axion provides a solution for the strong CP problem and is one of the leading candidates for dark matter. This paper proposes an axion detection scheme based on quantum nondemolition detection of magnon, i.e., quanta of collective spin excitations in solid, which is expected to be excited by the axion-electron interaction predicted by the Dine-Fischer-Srednicki-Zhitnitsky (DFSZ) model. The prototype detector is composed of a ferrimagnetic sphere as an electronic spin target and a superconducting qubit. Both of these are embedded inside a microwave cavity, which leads to a coherent effectiv…
Hybrid quantum devices expand the tools and techniques available for quantum sensing in various fields. Here, we experimentally demonstrate quantum sensing of the steady-state magnon population in a magnetostatic mode of a ferrimagnetic crystal. Dispersively coupling the magnetostatic mode to a superconducting qubit allows the detection of magnons using Ramsey interferometry with a sensitivity on the order of $10^{-3}$ $\text{magnons}/\sqrt{\text{Hz}}$. The protocol is based on dissipation as dephasing via fluctuations in the magnetostatic mode reduces the qubit coherence proportionally to the…
We present a scheme to implement a steady lightwave-photon-and-magnon entanglement in a hybrid photon-magnon system by adiabatically eliminating the auxiliary microwave cavity and effectively laser cooling a delocalized Bogoliubov mode. The system consists of magnons, lightwave and microwave photons, and phonons. The magnons are embodied by a collective motion of a large number of spins in a macroscopic ferrimagnet. To achieve an entangling interaction between magnons and lightwave photons, we drive optical cavity and magnon at the red and blue sideband associated with the mechanical resonator…
When there is a certain amount of field inhomogeneity, the biased ferrimagnetic crystal will exhibit the higher-order magnetostatic (HMS) mode in addition to the uniform-precession Kittel mode. In cavity magnonics, we show both experimentally and theoretically the cross-Kerr-type interaction between the Kittel mode and HMS mode. When the Kittel mode is driven to generate a certain number of excitations, the HMS mode displays a corresponding frequency shift and vice versa. The cross-Kerr effect is caused by an exchange interaction between these two spin-wave modes. Utilizing the cross-Kerr effe…
A photon-magnon hybrid system can be realised by coupling the electron spin resonance of a magnetic material to a microwave cavity mode. The quasiparticles associated with the system dynamics are the cavity magnon polaritons, which arise from the mixing of strongly coupled magnons and photons. We illustrate how these particles can be used to probe the magnetisation of a sample with a remarkable sensitivity, devising suitable spin-magnetometers which ultimately can be used to directly assess oscillating magnetic fields. Specifically, the capability of cavity magnon polaritons of converting magn…
The spin resonance of electrons can be coupled to a microwave cavity mode to obtain a photon-magnon hybrid system. These quantum systems are widely studied for both fundamental physics and technological quantum applications. In this article, the behavior of a large number of ferrimagnetic spheres coupled to a single cavity is put under test. We use second-quantization modeling of harmonic oscillators to theoretically describe our experimental setup and understand the influence of several parameters. The magnon-polariton dispersion relation is used to characterize the system, with a particular …
A dielectric body couples with electromagnetic fields through radiation pressure and electrostrictive forces, which mediate phonon-photon coupling in cavity optomechanics. In a magnetic medium, according to Korteweg-Helmholtz formula, magnetostrictive forces should arise and lead to phonon-magnon interaction. Here we report such a coupled phonon-magnon system based on ferrimagnetic spheres, which we term as cavity magnomechanics, by analogy to cavity optomechanics. Coherent phonon-magnon interactions, including electromagnetically induced transparency and absorption, are demonstrated. Exciting…
We show how to generate tripartite entanglement in a cavity magnomechanical system which consists of magnons, cavity microwave photons, and phonons. The magnons are embodied by a collective motion of a large number of spins in a macroscopic ferrimagnet, and are driven directly by an electromagnetic field. The cavity photons and magnons are coupled via magnetic dipole interaction, and the magnons and phonons are coupled via magnetostrictive (radiation pressure-like) interaction. We show optimal parameter regimes for achieving the tripartite entanglement where magnons, cavity photons, and phonon…
We study the parity-symmetry-breaking quantum phase transition (QPT) in a cavity magnonic system driven by a parametric field, where the magnons in a ferrimagnetic yttrium-iron-garnet sphere strongly couple to a microwave cavity. With appropriate parameters, this cavity magnonic system can exhibit a rich phase diagram, including the parity-symmetric phase, parity-symmetry-broken phase, and bistable phase. When increasing the drive strength beyond a critical threshold, the cavity magnonic system undergoes either a first- or second-order nonequilibrium QPT from the parity-symmetric phase with mi…
We show how a quantum state in a microwave cavity mode can be transferred to and stored in a phononic mode via an intermediate magnon mode in a magnomechanical system. For this we consider a ferrimagnetic yttrium iron garnet (YIG) sphere inserted in a microwave cavity, where the microwave and magnon modes are coupled via a magnetic-dipole interaction and the magnon and phonon modes in the YIG sphere are coupled via magnetostrictive forces. By modulating the cavity and magnon detunings and the driving of the magnon mode in time, a Stimulated Raman Adiabatic Passage (STIRAP)-like coherent transf…
We show how to prepare a steady-state entangled state between magnons and optical photons in an opto-magnomechanical configuration, where a mechanical vibration mode couples to a magnon mode in a ferrimagnet by the dispersive magnetostrictive interaction, and to an optical cavity by the radiation pressure. We find that, by appropriately driving the magnon mode and the cavity to simultaneously activate the magnomechanical Stokes and the optomechanical anti-Stokes scattering, a stationary optomagnonic entangled state can be created. We further show that, by activating the magnomechanical state-s…
A quantum network consisting of magnonic and mechanical nodes connected by light is proposed. Recent years have witnessed a significant development in cavity magnonics based on collective spin excitations in ferrimagnetic crystals, such as yttrium iron garnet (YIG). Magnonic systems are considered to be a promising building block for a future quantum network. However, a major limitation of the system is that the coherence time of the magnon excitations is limited by their intrinsic loss (typically in the order of 1 $μ$s for YIG). Here, we show that by coupling the magnonic system to a mechanic…
The generation and manipulation of strong entanglement and Einstein-Podolsky-Rosen (EPR) steering in macroscopic systems are outstanding challenges in modern physics. Especially, the observation of asymmetric EPR steering is important for both its fundamental role in interpreting the nature of quantum mechanics and its application as resource for the tasks where the levels of trust at different parties are highly asymmetric. Here, we study the entanglement and EPR steering between two macroscopic magnons in a hybrid ferrimagnet-light system. In the absence of light, the two types of magnons on…
Anticrossing behavior between magnons in a non-collinear chiral magnet Cu$_2$OSeO$_3$ and a two-mode X-band microwave resonator was studied in the temperature range 5-100K. In the field-induced ferrimagnetic phase, we observed a strong coupling regime between magnons and two microwave cavity modes with a cooperativity reaching 3600. In the conical phase, cavity modes are dispersively coupled to a fundamental helimagnon mode, and we demonstrate that the magnetic phase diagram of Cu$_2$OSeO$_3$ can be reconstructed from the measurements of the cavity resonance frequency. In the helical phase, a …
Enhancing ground-state cooling of center-of-mass motions via quantum squeezing from magnon nonlinearity
Hangzhou Dianzi University（杭州电子科技大学）；Zhejiang Key Laboratory of Quantum State Control and Optical Field Manipulation, Hangzhou Dianzi University（杭州量子态控制与光场调控浙江省重点实验室）
