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arXiv 2210.11202cond-mat.mtrl-sci
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钙钛矿半导体中载流子和激子自旋翻转的共振拉曼散射理论

Theory of resonant Raman scattering due to spin-flips of resident charge carries and excitons in perovskite semiconductors

A. V. Rodina, E. L. Ivchenko

摘要:

我们发展了一个拉曼散射理论,在共振激子区的光激发下,半导体钙钛矿晶体中的局域电子和空穴以及非平衡局域激子的单自旋和双自旋翻转。研究了局域激子、双激子和激子极化激元作为中间态的散射机制,极化激元的自旋翻转拉曼散射是一种新的机制。导出的方程中的不变形式允许一个分析的依赖性的初始和散射光的偏振和外部磁场的方向上的散射效率。

英文摘要:

We have developed a theory of Raman scattering with single and double spin flips of localized resident electrons and holes as well as nonequilibrium localized excitons in semiconductor perovskite crystals under optical excitation in the resonant exciton region. Scattering mechanisms involving localized excitons, biexcitons and exciton polaritons as intermediate states has been examined, the spin-flip Raman scattering by polaritons being a novel mechanism. The derived equations are presented in the invariant form allowing one for the analysis of the dependence of scattering efficiency on the polarization of the initial and scattered light and on the orientation of the external magnetic field.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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