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arXiv 2210.00337cond-mat.soft
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剪切增稠悬浮液中的流动诱导刚性逾渗

Flow induced rigidity percolation in shear thickening suspensions

Abhay Goyal, Nicos S. Martys, Emanuela Del Gado

摘要:

不连续剪切增稠(DST)与悬浮液的粘度随施加的剪切速率的增加而急剧上升有关。DST的一个关键特征,在最近的研究中强调,是非常大的波动的测量应力作为悬浮液增厚。微观结构的发展和应力波动的急剧增加之间的明确联系尚未建立。为了确定这种行为的微观结构基础,我们进行模拟剪切致密悬浮液。通过分析颗粒接触网络,我们确定了一个子集的约束颗粒,直接有助于粘度的快速上升和大的应力波动。事实上,这两种现象都可以用约束粒子网络的生长和渗透来解释--直接类比于刚性渗透。一个有限尺寸标度分析证实这是一个渗流现象,并允许我们估计的临界指数。我们的研究结果揭示了特定的微观结构转变,DST的基础。

英文摘要:

Discontinuous shear thickening (DST) is associated with a sharp rise of a suspension's viscosity with increasing applied shear rate. A key signature of DST, highlighted in recent studies, is the very large fluctuations of the measured stress as the suspension thickens. A clear link between microstructural development and the dramatic increase of the stress fluctuations has not been established yet. To identify the microstructural underpinnings of this behavior, we perform simulations of sheared dense suspensions. By analyzing particle contact networks, we identify a subset of constrained particles that contribute directly to the rapid rise in viscosity and the large stress fluctuations. Indeed, both phenomena can be explained by the growth and percolation of constrained particle networks -- in direct analogy to rigidity percolation. A finite size scaling analysis confirms this is a percolation phenomenon and allows us to estimate the critical exponents. Our findings reveal the specific microstructural transition that underlies DST.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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