arXivDaily arXiv每日学术速递 周一至周五更新
arXiv周末暂无论文更新,休息一下吧,周末愉快~~
arXiv 1702.02068cond-mat.soft
收藏

局部应力波动驱动稠密悬浮液中的剪切增稠

Localized Stress Fluctuations Drive Shear Thickening in Dense Suspensions

Vikram Rathee, Daniel L. Blair, Jeffery S. Urbach

摘要:

分散在牛顿流体中的固体颗粒的机械响应表现出广泛的非线性现象,包括粘度\cite{1-3}随着应力的增加而急剧增加。如果固相的体积分数是中等高的,悬浮液将经历连续剪切增稠(CST),其中悬浮液粘度随着施加的剪切应力平稳地增加;在更高的体积分数下,悬浮液可以显示不连续剪切增稠(DST),其中粘度在增加施加的应力时突然改变几个数量级。提出的模型来解释这种现象是基于两种不同类型的粒子相互作用,流体动力学\cite{2,4,5}和摩擦\cite{6-10}。在这两种情况下,体积粘度的增加归因于某种形式的局部聚集\cite{11,12}。然而,这些异质性的物理性质和动力学行为仍然不清楚。在这里,我们表明,连续的剪切增稠源于动态本地化定义良好的区域的颗粒具有高粘度,随着浓度迅速增加。此外,我们发现,这些区域的空间范围在很大程度上取决于剪切面之间的距离。我们的研究结果表明,连续剪切增稠产生越来越频繁的本地化的不连续过渡共存的低粘度和高粘度牛顿流体相之间。我们的研究结果提供了一个关键的物理联系之间的微观动力学过程,确定颗粒之间的相互作用和剪切增稠流体的体流变响应。

英文摘要:

The mechanical response of solid particles dispersed in a Newtonian fluid exhibits a wide range of nonlinear phenomena including a dramatic increase in the viscosity \cite{1-3} with increasing stress. If the volume fraction of the solid phase is moderately high, the suspension will undergo continuous shear thickening (CST), where the suspension viscosity increases smoothly with applied shear stress; at still higher volume fractions the suspension can display discontinuous shear thickening (DST), where the viscosity changes abruptly over several orders of magnitude upon increasing applied stress. Proposed models to explain this phenomenon are based in two distinct types of particle interactions, hydrodynamic\cite{2,4,5} and frictional\cite{6-10}. In both cases, the increase in the bulk viscosity is attributed to some form of localized clustering\cite{11,12}. However, the physical properties and dynamical behavior of these heterogeneities remains unclear. Here we show that continuous shear thickening originates from dynamic localized well defined regions of particles with a high viscosity that increases rapidly with concentration. Furthermore, we find that the spatial extent of these regions is largely determined by the distance between the shearing surfaces. Our results demonstrate that continuous shear thickening arises from increasingly frequent localized discontinuous transitions between coexisting low and high viscosity Newtonian fluid phases. Our results provide a critical physical link between the microscopic dynamical processes that determine particle interactions and bulk rheological response of shear thickened fluids.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑