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arXiv 2207.04861cond-mat.mtrl-sci
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电荷密度波的莫尔调制

Moiré Modulation of Charge Density Waves

Zachary A. H. Goodwin, Vladimir I. Fal'ko

AI总结:

本文研究了扭转金属性TMD同质双层中莫尔畴结构与不同周期电荷密度波的相互作用,揭示了不同CDW周期和扭转角下的传播、相位破坏及畴结构形成规律,为实验验证提供了理论预测。

摘要:

本文研究了单层固有的电荷密度波(CDW)在构建扭转范德华结构时受到的影响。以金属性过渡金属二硫族化合物(TMDs)同质双层为例,在小扭转角下存在显著原子重构,用于研究莫尔畴结构与不同周期CDW之间的相互作用。对于$\sqrt{3}\times\sqrt{3}$ CDW,不存在几何约束阻止CDW在整个莫尔结构中传播。而对于$2\times2$ CDW,为确保各层中的CDW在畴内具有最有利的相互作用,CDW相位必须在连接畴壁处被破坏。对于扭转角接近180度的$3\times3$ CDW,可形成莫尔尺度的三角形结构;而接近0度时,则出现莫尔尺度的二聚体畴。研究发现大卫之星CDW($\sqrt{13}\times\sqrt{13}$)仅在畴内容纳CDW,因为与$2\times2$ CDW类似,只存在一种低能堆叠构型。这些预测为在承载CDW的扭转双层金属性TMDs中进行实验验证提供了依据,我们希望这将促进对莫尔超晶格与组成二维材料固有CDW相之间相互作用的进一步研究。

英文摘要:

Here we investigate how charge density waves (CDW), inherent to a monolayer, are effected by creating twisted van der Waals structures. Homobilayers of metallic transition metal dichalcogenides (TMDs), at small twist angles where there is significant atomic reconstruction, are utilised as an example to investigate the interplay between the moiré domain structure and CDWs of different periods. For $\sqrt{3}\times\sqrt{3}$ CDWs, there is no geometric constraint to prevent the CDWs from propagating throughout the moiré structure. Whereas for $2\times2$ CDWs, to ensure the CDWs in each layer have the most favourable interactions in the domains, the CDW phase must be destroyed in the connecting domain walls. For $3\times3$ CDWs with twist angles close to 180 degree, moiré-scale triangular structures can form; while close to 0 degree, moiré-scale dimer domains occur. The star-of-David CDW ($\sqrt{13}\times\sqrt{13}$) is found to host CDWs in the domains only, since there is one low energy stacking configuration, similar to $2\times2$ CDWs. These predictions are offered for experimental verification in twisted bilayer metallic TMDs which host CDWs, and we hope this will stimulate further research on the interplay between the moiré supperlattice and CDW phases intrinsic to the comprising 2D materials.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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