Robust and high-fidelity control of electron spins in solids is the cornerstone for facilitating applications of solid-state spins in quantum information processing and quantum sensing. However, precise control of spin systems is always challenging due to the presence of a variety of noises originating from the environment and control fields. Herein, noise-resilient quantum gates, designed with robust optimal control (ROC) algorithms, are demonstrated experimentally with nitrogen-vacancy (NV) centers in diamond to realize tailored robustness against detunings and Rabi errors simultaneously. In the presence of both 10% off-resonant detuning and deviation of a Rabi frequency, we achieve an average single-qubit gate fidelity of up to 99.97%. Our experiments also show that, ROCbased multipulse quantum sensing sequences can suppress spurious responses resulting from finite widths and imperfections of microwave pulses, which provides an efficient strategy for enhancing the performance of existing multipulse quantum sensing sequences.
Coherent manipulation of interacting electron qubitson solid neon
Harvard University（哈佛大学）；Argonne National Laboratory（阿贡国家实验室）；University of Chicago（芝加哥大学）；National High Magnetic Field Laboratory（国家高磁场实验室）；Florida State University（佛罗里达州立大学）；University of Notre Dame（圣母大学）
We propose fast phase-gates of single nuclear spins interacting with single electron spins. The gate operation utilizes geometric phase shifts of the electron spin induced by fast/slow rotating fields; the path difference depending on nuclear spin states enables nuclear phase shifts. The gate time is inversely proportional to the frequency of the slow rotating field. As an example, we use nitrogen-vacancy centers in diamond, and show the phase-gate time orders of magnitude shorter than previously reported. We also show the robustness of the gate against decoherence and systematic errors.
We demonstrate fast and accurate control of the evolution of collective atomic coherences in an Erbium doped solid using external electric fields. This is achieved by controlling the inhomogeneous broadening of Erbium ions emitting at 1536 nm using an electric field gradient and the linear Stark effect. The manipulation of atomic coherence is characterized with the collective spontaneous emission (optical free induction decay) emitted by the sample after an optical excitation, which does not require any previous preparation of the atoms. We show that controlled dephasing and rephasing of the a…
A coupled system of a superconducting transmission line resonator with a semiconductor double quantum dot is analyzed. We simulate the phase shift of the microwave signal in the resonator, which is sensitive to the quantum dot qubit state and manipulation. The measurement quality is sufficiently high and the results demonstrate a solid-state quantum processor based on this type of circuit can be envisioned.
We describe laser systems for photoionization, Doppler cooling and quantum state manipulation of beryllium ions. For photoionization of neutral beryllium, we have developed a continuous-wave 235 nm source obtained by two stages of frequency doubling from a diode laser at 940 nm. The system delivers up to 400 mW at 470 nm and 28 mW at 235 nm. For control of the beryllium ion, three laser wavelengths at 313 nm are produced by sum-frequency generation and second-harmonic generation from four infrared fiber lasers. Up to 7.2 W at 626 nm and 1.9 W at 313 nm are obtained using two pump beams at 1051…
We provide a scheme for quantum computation in lattice systems via global but periodic manipulation, in which only effective periodic magnetic fields and global nearest neighbor interaction are required. All operations in our scheme are attainable in optical lattice or solid state systems. We also investigate universal quantum operations and quantum simulation in 2 dimensional lattice. We find global manipulations are superior in simulating some nontrivial many body Hamiltonians.
Coherent control of quantum states is at the heart of implementing solid-state quantum processors and testing quantum mechanics at the macroscopic level. Despite significant progress made in recent years in controlling single- and bi-partite quantum systems, coherent control of quantum wave function in multipartite systems involving artificial solid-state qubits has been hampered due to the relatively short decoherence time and lacking of precise control methods. Here we report the creation and coherent manipulation of quantum states in a tripartite quantum system, which is formed by a superco…
The phase relation between quantum states represents an essential resource for the storage and processing of quantum information. While quantum phases are commonly controlled dynamically by tuning energetic interactions, utilizing geometric phases that accumulate during cyclic evolution may offer superior robustness to noise. To date, demonstrations of geometric phase control in solid-state systems rely on microwave fields that have limited spatial resolution. Here, we demonstrate an all-optical method based on stimulated Raman adiabatic passage to accumulate a geometric phase, the Berry phase…
We show that it is possible to initialize and manipulate in a deterministic manner protected qubits using time varying Hamiltonians. Taking advantage of the symmetries of the system, we predict the effect of the noise during the initialization and manipulation. These predictions are in good agreement with numerical simulations. Our study shows that the topological protection remains efficient under realistic experimental conditions.
We analyze approximate transformations of pure entangled quantum states by local operations and classical communication, finding explicit conversion strategies which optimize the fidelity of transformation. These results allow us to determine the most faithful teleportation strategy via an initially shared partially entangled pure state. They also show that procedures for entanglement manipulation such as entanglement catalysis [Jonathan and Plenio, Phys. Rev. Lett. 83, 3566 (1999)] are robust against perturbation of the states involved, and motivate the notion of non-local fidelity, which qua…
Superconducting quantum systems are promising candidates for quantum information processing due to their scalability and design flexibility. However, the existence of defects, fluctuations, and inaccuracies is unavoidable for practical superconducting quantum circuits. In this paper, a sampling-based learning control (SLC) method is used to guide the design of control fields for manipulating superconducting quantum systems. Numerical results for one-qubit systems and coupled two-qubit systems show that the "smart" fields learned using the SLC method can achieve robust manipulation of supercond…
The limitations for the coherent manipulation of neutral atoms with fabricated solid state devices, so-called `atom chips', are addressed. Specifically, we examine the dominant decoherence mechanism, which is due to the magnetic noise originating from the surface of the atom chip. It is shown that the contribution of fluctuations in the chip wires at the shot noise level is not negligible. We estimate the coherence times and discuss ways to increase them. Our main conclusion is that future advances should allow for coherence times as long as one second, a few micrometers away from the surface.
High-fidelity control of quantum systems is crucial for quantum information processing, but is often limited by perturbations from the environment and imperfections in the applied control fields. Here, we investigate the combination of dynamical decoupling (DD) and robust optimal control (ROC) to address this problem. In this combination, ROC is employed to find robust shaped pulses, wherein the directional derivatives of the controlled dynamics with respect to control errors are reduced to a desired order. Then, we incorporate ROC pulses into DD sequences, achieving a remarkable improvement o…
We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in diamond, we demonstrate control of a proximal $^{14}$N nuclear spin via an all-optical Raman technique. We evaluate the extent to which the intrinsic physical properties of the NV center limit the performance of coherent control, and find that it is ultimately constrained by the relative rates of transverse hyperfine coupling and radiative decay in the NV cen…
In this paper we study robust pulse design for electron shuttling in solid state devices. This is crucial for many practical applications of coherent quantum mechanical systems. Our objective is to design control pulses that can transport an electron along a chain of donors, and also make this process robust to parameter uncertainties. We formulate it as a set of optimal control problems on the special unitary group SU(n), and derive explicit expressions for the gradients of the aggregate transfer fidelity. Numerical results for a donor chain of ionized phosphorus atoms in bulk silicon demonst…
We demonstrate a synchronized readout (SR) technique for spectrally selective detection of oscillating magnetic fields with sub-millihertz resolution, using coherent manipulation of solid state spins. The SR technique is implemented in a sensitive magnetometer (~50 picotesla/Hz^(1/2)) based on nitrogen vacancy (NV) centers in diamond, and used to detect nuclear magnetic resonance (NMR) signals from liquid-state samples. We obtain NMR spectral resolution ~3 Hz, which is nearly two orders of magnitude narrower than previously demonstrated with NV based techniques, using a sample volume of ~1 pic…
We discuss the operational definition of decoherence in various solid state systems. In particular, we review, in the context of spin-based solid state quantum computation, the introduction of $T_1$ and $T_2$ to describe decoherence in a two level system. We provide a perspective on recent experiments involving the manipulation of spin coherence in semiconductors, and discuss specific decoherence and dephasing issues in electron spin-based quantum dot quantum computer architectures.
We investigate creation, manipulation, and steering of entanglement in spin chains from the viewpoint of quantum communication between distant parties. We demonstrate how global parametric driving of the spin-spin coupling and/or local time-dependent Zeeman fields produce a large amount of entanglement between the first and the last spin of the chain. This occurs whenever the driving frequency meets a resonance condition, identified as "entanglement resonance". Our approach marks a promising step towards an efficient quantum state transfer or teleportation in solid state system. Following the …
Solid-state electronic spin systems such as nitrogen-vacancy (NV) color centers in diamond are promising for applications of quantum information, sensing, and metrology. However, a key challenge for such solid-state systems is to realize a spin coherence time that is much longer than the time for quantum spin manipulation protocols. Here we demonstrate an improvement of more than two orders of magnitude in the spin coherence time ($T_2$) of NV centers compared to previous measurements: $T_2 \approx 0.5$ s at 77 K, which enables $\sim 10^7$ coherent NV spin manipulations before decoherence. We …
We experimentally demonstrate a robust dynamical decoupling protocol with bounded controls using long soft pulses, eliminating a challenging requirement of strong control pulses in conventional implementations. This protocol is accomplished by designing the decoupling propagators to go through a Eulerian cycle of the coupler group [Phys. Rev. Lett. 90, 037901(2003)]. We demonstrate that this Eulerian decoupling scheme increases the coherence time by two orders of magnitude in our experiment under either dephasing or a universal noise environment.
Rare-earth ion doped crystals have proven to be solid platforms for implementing quantum memories. Their potential use for integrated photonics with large multiplexing capability and unprecedented coherence times is at the core of their attractiveness. The best performances of these ions are however usually obtained when subject to a dc magnetic field, but consequences of such fields on the quantum memory protocols have only received little attention. In this article, we focus on the effect of a dc bias magnetic field on the population manipulation of non-Kramers ions with nuclear quadrupole s…
The inhomogeneity of an electron spin ensemble as well as fluctuating environment acting upon individual spins drastically shorten the spin coherence time $T_2$ and hinder coherent spin manipulation. We show that this problem can be solved by the simultaneous application of a radiofrequency (rf) field, which stimulates coherent spin precession decoupled from an inhomogeneous environment, and periodic optical pulses, which amplify this precession. The resulting resonance, taking place when the rf field frequency approaches the laser pulse repetition frequency, has a width determined by the spin…
We apply an invariant-based inverse engineering method to control by time-dependent electric fields electron spin dynamics in a quantum dot with spin-orbit coupling in a weak magnetic field. The designed electric fields provide a shortcut to adiabatic processes that flips the spin rapidly, thus avoiding decoherence effects. This approach, being robust with respect to the device-dependent noise, can open new possibilities for the spin-based quantum information processing.
As a qubit usually has a limited lifetime, its manipulation should be as fast as possible, and thus non-adiabatic operation is more preferable. Moreover, as a qubit inevitably interacts with its surrounding environment, robust operations are of great significance. Here, we propose a scheme for quantum manipulation of the polariton qubit in circuit QED using non-adiabatic holonomy, which is inherently fast and robust. In particularly, the polariton qubit is shown to be robust against arbitrary low-frequency noise due to its near symmetric spectrum, which can also be convenient manipulated by ex…
The study of individual quantum systems in solids, for use as quantum bits (qubits) and probes of decoherence, requires protocols for their initialization, unitary manipulation, and readout. In many solid-state quantum systems, these operations rely on disparate techniques that can vary widely depending on the particular qubit structure. One such qubit, the nitrogen-vacancy (NV) center spin in diamond, can be initialized and read out through its special spin selective intersystem crossing, while microwave electron spin resonance (ESR) techniques provide unitary spin rotations. Instead, we demo…
Manipulation of solid-state spin coherence is an important paradigm for quantum information processing. Current systems either operate at very low temperatures or are difficult to scale-up. Developing low-cost, scalable materials whose spins can be coherently manipulated at room temperature is thus highly-attractive for a sustainable future of quantum information science. Here we report ambient-condition all-optical initialization, manipulation and readout of single-hole spins in an ensemble of solution-grown CsPbBr3 perovskite QDs. Single-hole spins are obtained by sub-picosecond electron sca…
We review progress on the use of electron spins to store and process quantum information, with particular focus on the ability of the electron spin to interact with multiple quantum degrees of freedom. We examine the benefits of hybrid quantum bits (qubits) in the solid state that are based on coupling electron spins to nuclear spin, electron charge, optical photons, and superconducting qubits. These benefits include the coherent storage of qubits for times exceeding seconds, fast qubit manipulation, single qubit measurement, and scalable methods for entangling spatially separated matter-based…
Nonlinear Electro-Optic Visible Photonic Circuits for Solid-State Quantum Defects
Korea Institute of Science and Technology (KIST)（韩国科学技术院）；Korea University（高丽大学）；Sejong University（世宗大学）；KIST School, Korea University of Science and Technology（韩国科学技术院KIST学院）
Control over electron-spin states, such as coherent manipulation, filtering and measurement promises access to new technologies in conventional as well as in quantum computation and quantum communication. In this paper, we review recent theoretical proposal of using electron spins in quantum confined structures as qubits. We also present a theoretical proposal for testing Bell's inequality in nano-electronics devices. We show that the entanglement of two electron spins can be detected in the spin filter effect in the nanostructure semiconductor / ferromagnetic semiconductor / semiconductor jun…
Lattice Gauge Theories form a very successful framework for studying nonperturbative gauge field physics, in particular in Quantum Chromodynamics. Recently, their quantum simulation on atomic and solid-state platforms has been discussed, aiming at overcoming some of the difficulties still faced by the conventional approaches (such as the sign problem and real time evolution). While the actual implementations of a lattice gauge theory on a quantum simulator may differ in terms of the simulating system and its properties, they are all directed at studying similar physical phenomena, requiring th…
Realization of Quantum information and communications technologies requires robust, stable solid state single photon sources. However, most existing sources cease to function above cryogenic or room temperature due to thermal ionization or strong phonon coupling which impede their emissive and quantum properties. Here we present an efficient single photon source based on a defect in a van der Waals crystal that is optically stable and operates at elevated temperatures of up to 800 K. The quantum nature of the source and the photon purity are maintained upon heating to 800 K and cooling back to…
