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arXiv 2203.06129cond-mat.mtrl-scicond-mat.str-elphysics.optics
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范德华磁体中的自旋关联激子-极化激元

Spin-correlated exciton-polaritons in a van der Waals magnet

Florian Dirnberger, Rezlind Bushati, Biswajit Datta, Ajesh Kumar, Allan H. MacDonald, Edoardo Baldini, Vinod M. Menon

AI总结:

本文在范德华反铁磁体NiPS3中实现了自旋关联激子与微腔光子的强耦合,发现了一类新型极化激元准粒子,为通过腔量子电动力学设计和控制关联电子系统提供了新途径。

摘要:

光与元激发之间的强耦合正成为调控固态系统性质的有力工具。与光学腔产生强耦合的自旋关联激发有望实现对磁相变等集体量子现象的控制,但尚未找到其合适的电子共振。我们在NiPS3中报告了强光-物质耦合,这是一种具有高度关联电子自由度的范德华反铁磁体。其自旋关联激子与微腔内的光子发生强耦合,产生了一类此前未被观测到的极化激元准粒子。结合微观理论的详细光谱分析,为这些奇异的磁性耦合激发的起源和相互作用提供了独特见解。我们的工作将范德华磁体引入强光-物质物理领域,并为通过腔量子电动力学设计和控制关联电子系统提供了途径。

英文摘要:

Strong coupling between light and elementary excitations is emerging as a powerful tool to engineer the properties of solid-state systems. Spin-correlated excitations that couple strongly to optical cavities promise control over collective quantum phenomena such as magnetic phase transitions, but their suitable electronic resonances have yet to be found. Here we report strong light-matter coupling in $\textrm{NiPS}_3$, a van der Waals antiferromagnet with highly correlated electronic degrees of freedom. A previously unobserved class of polaritonic quasiparticles emerges from the strong coupling between its spin-correlated excitons and the photons inside a microcavity. Detailed spectroscopic analysis in conjunction with a microscopic theory provides unique insights into the origin and interactions of these exotic magnetically coupled excitations. Our work introduces van der Waals magnets to the field of strong light-matter physics and provides a path towards the design and control of correlated electron systems via cavity quantum electrodynamics.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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