arXivDaily arXiv每日学术速递 周一至周五更新
arXiv周末暂无论文更新,休息一下吧,周末愉快~~
arXiv 2203.04265cond-mat.str-elcond-mat.supr-con
收藏

高电荷$T_c$铜氧化物La $_{1.875}$ Ba $_{0.125}$ NMR $_{4}$中晶格、电荷和自旋动力学之间相互作用的研究

$^{139}$La NMR investigation of the interplay between the lattice, charge, and spin dynamics in charge ordered high $T_c$ cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$

P. M. Singer, A. Arsenault, T. Imai, M. Fujita

摘要:

本文基于对$^{139}$ La核自旋-晶格弛豫速率$1/T_1$的逆拉普拉斯变换(ILT)分析,研究了电荷有序高$T_c$铜氧化物La $_{1.875}$ Ba $_{0.125}$ CuO $_{4}$($T_{c} =4$ ~K)中晶格、电荷和自旋动力学之间的相互作用. ILTT $_{1}$分析的一个主要推动力是可以推导出分布式$1/T_1$的概率密度函数$P(1/T_1)$。我们证明,$1/T_{1}^{lm}$,定义为$P(1/T_1)$的对数平均值(即在对数尺度上的重心),可以很好地近似由$1/T_{1}^{str}$推导出的唯象拉伸拟合,然而,$P(1/T_1)$可以提供更丰富的洞察力,晶格,电荷和自旋的波动及其分布的发展附近和以下的长程电荷秩序在$T_{charge} \sim 54$ ~K。当进入电荷有序态时,$1/T_{1}^{lm}$朝着$T_{spin}^{μSR} \simeq 35$ ~K处的自旋有序的发散增加伴随着$P(1/T_1)$的不对称加宽。即使在电荷有序状态的深处,随着温度的降低,$1/T_{1}$在$^{139}$ La位点的分数逐渐减少,继续减慢,正如对没有增强的自旋波动的规范超导CuO $_2$平面所预期的那样。这种典型的$^{139}$ La位的分数几乎消失的$\simeq 40$ ~K。与此相反,在LaPDMATHABNC SrPDMATHABND CuOPDMATHABMP($T_{charge} \simeq 80$ ~K)中,近一半的$^{139}$ La位甚至在其$T_{c} = 31$ ~K附近仍表现出没有增强自旋涨落的正则行为.这些对比行为解释了为什么超导电性在La $_{1.875}$ Ba $_{0.125}$ CuO $_{4}$更强烈地抑制比在La $_{1.885}$ Sr $_{0.115}$ CuO $_{4}$尽管较低的起始温度的电荷顺序。

英文摘要:

We investigate the interplay between the lattice, charge, and spin dynamics in charge ordered high $T_c$ cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ ($T_{c} =4$~K) based on the inverse Laplace transform (ILT) analysis of the $^{139}$La nuclear spin-lattice relaxation rate $1/T_1$ (dubbed ILTT$_{1}$ analysis here after). A major thrust of the ILTT$_{1}$ analysis is that one can deduce the probability density function $P(1/T_1)$ of distributed $1/T_1$. We demonstrate that $1/T_{1}^{lm}$, defined as the log-mean (i.e. the center of gravity on a logarithmic scale) of $P(1/T_1)$, can be well approximated by $1/T_{1}^{str}$ deduced from the phenomenological stretched fit, however, $P(1/T_1)$ can provide much richer insight into how the lattice, charge, and spin fluctuations and their distribution develop near and below the long range charge order at $T_{charge} \sim 54$~K. Upon entering the charge ordered state, a divergent increase of $1/T_{1}^{lm}$ toward the spin ordering at $T_{spin}^{μSR} \simeq 35$~K is accompanied by an asymmetric broadening of $P(1/T_1)$. Even deep inside the charge ordered state, $1/T_{1}$ at a gradually diminishing fraction of $^{139}$La sites continues to slow down as temperature is lowered, as expected for canonical superconducting CuO$_2$ planes without enhanced spin fluctuations. The fraction of such canonical $^{139}$La sites almost disappears by $\simeq 40$~K. In contrast, nearly a half of the $^{139}$La sites in La$_{1.885}$Sr$_{0.115}$CuO$_{4}$ ($T_{charge} \simeq 80$~K) still exhibits the canonical behavior without enhanced spin fluctuations even near its $T_{c} = 31$~K. These contrasting behaviors explain why superconductivity in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ is more strongly suppressed than in La$_{1.885}$Sr$_{0.115}$CuO$_{4}$ despite the lower onset temperature of the charge order.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑