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arXiv 2107.08161cond-mat.mtrl-scicond-mat.str-el
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核自旋Seebeck效应的观测

Observation of nuclear-spin Seebeck effect

T. Kikkawa, D. Reitz, H. Ito, T. Makiuchi, T. Sugimoto, K. Tsunekawa, S. Daimon, K. Oyanagi, R. Ramos, S. Takahashi, Y. Shiomi, Y. Tserkovnyak, E. Saitoh

摘要:

热电效应已经应用于发电机和将废热转换成电的温度传感器。然而,这些效应仅限于电子发生,并且由于电子熵淬灭而在低温下不可避免地消失。在这里,我们报告热电发电所造成的核自旋固体:核自旋塞贝克效应。样品是磁性有序材料MnCO $_{3}$,其具有$^{55}$ Mn核的大核自旋($I = 5/2$)和强超精细耦合,具有Pt接触。在该系统中,我们观察到低温热电信号下降到100 mK由于核自旋激发。我们的理论计算中,考虑了界面Korringa过程定量再现的结果。核热电效应为超低温下的热电科学和技术的探索提供了一条途径。

英文摘要:

Thermoelectric effects have been applied to power generators and temperature sensors that convert waste heat into electricity. The effects, however, have been limited to electrons to occur, and inevitably disappear at low temperatures due to electronic entropy quenching. Here, we report thermoelectric generation caused by nuclear spins in a solid: nuclear-spin Seebeck effect. The sample is a magnetically ordered material MnCO$_{3}$ having a large nuclear spin ($I = 5/2$) of $^{55}$Mn nuclei and strong hyperfine coupling, with a Pt contact. In the system, we observe low-temperature thermoelectric signals down to 100 mK due to nuclear-spin excitation. Our theoretical calculation in which interfacial Korringa process is taken into consideration quantitatively reproduces the results. The nuclear thermoelectric effect demonstrated here offers a way for exploring thermoelectric science and technologies at ultralow temperatures.

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