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arXiv 2107.06508cond-mat.mtrl-sci
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$Y_{1.5}Gd_{1.5}Fe_{5}O_{12}$ 稀土铁石榴石中跨磁补偿温度的亚晶格自旋反转与场诱导 $Fe^{3+}$ 自旋倾斜

Sublattice spin reversal and field induced $Fe^{3+}$ spin-canting across the magnetic compensation temperature in $Y_{1.5}Gd_{1.5}Fe_{5}O_{12}$ rare-earth iron garnet

Manik Kuila, Jose Renato Linares Mardegan, Akhil Tayal, Sonia Francoual, V. Raghavendra Reddy

AI总结:

本研究利用穆斯堡尔谱和XMCD证实YGdIG中跨磁补偿温度的Fe³⁺与Gd³⁺亚晶格自旋反转及场诱导Fe³⁺自旋倾斜,实现单边分析提取双亚晶格信息,结果与体磁化数据吻合。

摘要:

本研究通过外加磁场下的 $^{57}Fe$ 穆斯堡尔谱测量,在多晶 $Y_{1.5}Gd_{1.5}Fe_{5}O_{12}$(YGdIG)中证实了跨磁补偿温度($T_{Comp}$)的 $Fe^{3+}$ 亚晶格自旋反转与 $Fe^{3+}$ 自旋倾斜现象。作为外加磁场下 $^{57}Fe$ 穆斯堡尔测量的佐证,硬X射线区的X射线磁圆二色(XMCD)测量也证实了 $Fe^{3+}$ 与 $Gd^{3+}$ 亚晶格的自旋反转。此外,通过外加磁场下的 $^{57}Fe$ 穆斯堡尔测量,对有效内超精细场($H_{eff}$)、六线谱中吸收线相对强度的估算与分析,明确揭示了跨 $T_{Comp}$ 时 $Fe^{3+}$ 自旋反转的特征、其连续转变过程以及场诱导的 $Fe^{3+}$ 亚晶格自旋倾斜。进一步发现,Fe K边(Gd $L_{3}$ 边)的XMCD信号包含额外的谱特征,这些特征源自 $Gd^{3+}$($Fe^{3+}$)的磁有序,使得我们能够通过单边分析提取两种亚晶格($Fe^{3+}$ 与 $Gd^{3+}$)的信息。从Fe K边或Gd $L_3$ 边提取的两种磁亚晶格的磁矩随温度的演化,与从YGdIG和YIG($Y_{3}Fe_{5}O_{12}$)的体磁化数据提取的值高度吻合。这些测量为研究此类复杂体系在补偿点附近的磁行为开辟了新途径。

英文摘要:

In the present work $Fe^{3+}$ sublattice spin reversal and $Fe^{3+}$ spin-canting across the magnetic compensation temperature ($T_{Comp}$) are demonstrated in polycrystalline $Y_{1.5}Gd_{1.5}Fe_{5}O_{12}$ (YGdIG) by means of in-field $^{57}Fe$ M$\ddot{o}$ssbauer spectroscopy measurements. Corroborating in-field $^{57}Fe$ M$\ddot{o}$ssbauer measurements, both $Fe^{3+}$ & $Gd^{3+}$ sublattice spin reversal has also been manifested with x-ray magnetic circular dichroism (XMCD) measurement in hard x-ray region. Moreover from in-field $^{57}Fe$ M$\ddot{o}$ssbauer measurements, estimation and analysis of effective internal hyperfine field ($H_{eff}$), relative intensity of absorption lines in a sextet elucidated unambiguously the signatures of $Fe^{3+}$ spin reversal, their continuous transition and field induced spin-canting of $Fe^{3+}$ sublattices across $T_{Comp}$. Further, Fe K- (Gd $L_{3}$-) edge XMCD signal is observed to consist of additional spectral features, those are identified from $Gd^{3+}$ ($Fe^{3+}$) magnetic ordering, enabling us the extraction of both the sublattices ($Fe^{3+}$ & $Gd^{3+}$) information from a single edge analysis. The evolution of the magnetic moments as a function of temperature for both magnetic sublattices extracted either at the Fe K- or Gd $L_3$-edge agree quite well with values that are extracted from bulk magnetization data of YGdIG and YIG ($Y_{3}Fe_{5}O_{12}$). These measurements pave new avenues to investigate how the magnetic behavior of such complex system acts across the compensation point.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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