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arXiv 2107.00876cond-mat.str-el
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非掺杂Sr $_2$ IrO $_4$中斜反铁磁性和赝自旋电流的三维堆积:对称性分析和微观模型实现

Three-dimensional Stacking of Canted Antiferromagnetism and Pseudospin Current in Undoped Sr$_2$IrO$_4$: Symmetry Analysis and Microscopic Model Realization

Yun-Peng Huang, Jin-Wei Dong, Ziqiang Wang, Sen Zhou

摘要:

最近的光学二次谐波产生实验观察到未掺杂的自旋-轨道莫特绝缘体Sr $_2$ IrO $_4$中意外的空间对称性破缺,导致对其基态性质的激烈争论。我们认为它是一种具有循环交错赝自旋流隐序的倾斜反铁磁性。对称性分析表明,一个适当的$c$轴堆叠的倾斜反铁磁性和赝自旋电流导致磁电共存状态,打破了双重旋转,反转和时间反转对称性,与实验观察一致。我们构造了一个三维哈伯德模型,考虑了以Ir位为中心的5个定域5 $d$ Wannier轨道的自旋轨道耦合,并通过自洽Hartree-Fock和变分计算的结合证明了在宽的能带参数范围内所需共存态的微观实现.

英文摘要:

Recent optical second-harmonic generation experiments observed unexpected broken spatial symmetries in the undoped spin-orbit Mott insulator Sr$_2$IrO$_4$, leading to intensive debates on the nature of its ground state. We propose that it is a canted antiferromagnetism with a hidden order of circulating staggered pseudospin current. Symmetry analysis shows that a proper $c$-axis stacking of the canted antiferromagnetism and the pseudospin current lead to a magnetoelectric coexistence state that breaks the two-fold rotation, inversion, and time-reversal symmetries, consistent with experimental observations. We construct a three-dimensional Hubbard model with spin-orbit coupling for the five localized 5$d$ Wannier orbitals centered at Ir sites, and demonstrate the microscopic realization of the desired coexistence state in a wide range of band parameters via a combination of self-consistent Hartree-Fock and variational calculations.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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