Optical control of Dirac surface states (SS) in topological insulators (TI) remains one of the most challenging problems governing their potential applications in novel electronic and spintronic devices. Here, using visible-range transient absorption spectroscopy exploiting ~340 nm (~3.65 eV) pumping, we provide evidence for dynamic opening of a gap in Dirac SS of the thin-film 3D TI Bi2Se3, which has been induced by the dynamic Rashba effect occurring in the film bulk with increasing optical pumping power (photoexcited carrier density). The observed effect appears through the transient absorption band associated with inverse-bremsstrahlung-type free carrier absorption in the gapped Dirac SS. We have also recognized experimental signatures of the existence of the higher energy Dirac SS in the 3D TI Bi2Se3 (in addition to those known as SS1 and SS2) with energies of ~2.7 and ~3.9 eV (SS3 and SS4). It is evidenced that the dynamic gap opening has the same effect on the Dirac SS occurring at any energy.
We propose a model of three-dimensional topological insulators consisting of weakly coupled electron- and hole-gas layers with Rashba spin-orbit interaction stacked along a given axis. We show that in the presence of strong electron-electron interactions the system realizes a fractional strong topological insulator, where the rotational symmetry and condensation energy arguments still allow us to treat the problem as quasi-one-dimensional with bosonization techniques. We also show that if Rashba and Dresselhaus spin-orbit interaction terms are equally strong, by doping the system with magnetic…
Thanks to its unique symmetry, the unidirectional spin Hall and Rashba-Edelstein magnetoresistance (USRMR) is of great fundamental and practical interest, particularly in the context of reading magnetization states in two-terminal spin-orbit torque switching memory and logic devices. Recent studies show that topological insulators could improve USRMR amplitude. However, the topological insulator device configurations studied so far in this context, namely ferromagnetic metal/topological insulator bilayers and magnetically doped topological insulators, suffer from current shunting by the metall…
The effects of Rashba interaction and electromagnetic field on the edge states of a two-dimensional topological insulator are investigated in a non-perturbative way. We show that the electron dynamics is equivalent to a problem of massless Dirac fermions propagating with an inhomogeneous velocity, enhanced by the Rashba profile with respect to the bare Fermi value $v_F$. Despite the inelastic and time-reversal breaking processes induced by the electromagnetic field, no backscattering occurs without interaction. The photoexcited electron densities are explicitly obtained in terms of the electri…
In addition to the topologically protected linear dispersion, a band-bending-confined two-dimensional electron gas with tunable Rashba spin-splitting (RSS) was found to coexist with the topological surface states on the surface of topological insulators (TIs). Here, we report the observation of large bilinear magnetoresistance (BMR) in Bi2Se3 films decorated with transition metal atoms. The magnitude of the BMR sensitively depends on the type and amount of atoms deposited, with a maximum achieved value close to those of strong Rashba semiconductors. Our first-principles calculations reproduce …
We study a generic topological Kondo insulator system by performing a mean-field theoretic calculation within the frame-work of slave-boson protocol. We assume infinite Hubbard-type interaction among the localized electrons. The difference between the bulk metallic and insulating phases of the insulator is in the sign of nearest neighbor hopping of localized electrons. The hopping amplitude is positive for the metallic and negative for the insulating phase. The surface metallicity together with bulk insulation, however, requires very strong f electron localization. Furthermore, we find that th…
This paper considers a model consisting of a kinetic term, Rashba spin-orbit coupling and short-range Coulomb interaction at zero-temperature. The Coulomb interaction is decoupled by a mean-field approximation in the spin channel using field theory methods. The results feature a first-order phase transition for any finite value of the chemical potential and quantum criticality for vanishing chemical potential. The Hall conductivity is also computed using Kubo formula in a mean-field effective Hamiltonian. In the limit of infinite mass the kinetic term vanishes and all the phase transitions are…
The recent discovery of materials featuring strong Rashba spin-orbit coupling (RSOC) and strong electronic correlation raises questions about the interplay of Mott and Rashba physics. In this work, we employ cluster perturbation theory to investigate the spectral properties of the two-dimensional Hubbard model in the presence of a significant or large RSOC. We show that RSOC strongly favors metallic phases and competes with Mott localization, leading to an unconventional scenario for the Mott transition which is no longer controlled by the ratio between the Hubbard $U$ and an effective bandwid…
Topological insulators are bulk insulators with exotic surface states, protected under time-reversal symmetry, that hold promise in observing many exciting condensed-matter phenomena. In this report, we show that by having a topological insulator (Bi$_2$Se$_3$) in proximity to a magnetic insulator (EuS), a metal-to-insulator transition in the surface state, attributed to opening of an exchange gap, can be observed whose properties are tunable using bottom gate voltage and external magnetic field. Our study provides evidence of gate-controlled enhanced interface magnetism with the signature of …
We consider a system of stacked tunnel-coupled two-dimensional electron- and hole-gas layers with Rashba spin-orbit interactions subjected to a staggered Zeeman field. The interplay of different intra-layer tunnel couplings results in a phase transition to a topological insulator phase in three dimensions hosting gapless surface states. The staggered Zeeman field further enriches the topological phase diagram by generating a second-order topological insulator phase hosting gapless hinge states. The emergence of the topological phases is proven analytically in the regime of small Zeeman field a…
Topological insulators represent a new class of quantum phase defined by invariant symmetries and spin-orbit coupling that guarantees metallic Dirac excitations at its surface. The discoveries of these states have sparked the hope of realizing nontrivial excitations and novel effects such as a magnetoelectric effect and topological Majorana excitations. Here we develop a theoretical formalism to show that a three dimensional topological insulator can be designed artificially via stacking bilayers of two-dimensional Fermi gases with opposite Rashba-type spin-orbit coupling on adjacent layers, a…
We study the helical edge states of a two-dimensional topological insulator without axial spin symmetry due to the Rashba spin-orbit interaction. Lack of axial spin symmetry can lead to so-called generic helical edge states, which have energy-dependent spin orientation. This opens the possibility of inelastic backscattering and thereby nonquantized transport. Here we find analytically the new dispersion relations and the energy dependent spin orientation of the generic helical edge states in the presence of Rashba spin-orbit coupling within the Bernevig-Hughes-Zhang model, for both a single is…
Rashba spin-orbit coupling and a magnetic field perpendicular to the Rashba axis have been predicted to open a partial gap ("helical gap") in the energy spectrum of noninteracting or weakly interacting one-dimensional quantum wires. By comparing kinetic energy and Coulomb energy we show that this gap opening typically occurs at low electron densities where the Coulomb energy dominates. To address this strongly correlated limit, we investigate Rashba wires using Wigner crystal theory. We find that the helical gap exists even in the limit of strong interactions but its dependence on electron den…
The critical current of a superconductor can depend on the direction of current flow due to magnetochiral anisotropy when both inversion and time-reversal symmetry are broken, an effect known as the superconducting (SC) diode effect. Here, we consider one-dimensional (1D) systems in which superconductivity is induced via the proximity effect. In both topological insulator and Rashba nanowires, the SC diode effect due to a magnetic field applied along the spin-polarization axis and perpendicular to the nanowire provides a measure of inversion symmetry breaking in the presence of a superconducto…
Erratum: Engineering a p+ip Superconductor: Comparison of Topological Insulator and Rashba Spin-Orbit Coupled Materials [Phys. Rev. B 83, 184520 (2011)]
In this work we have investigated the effect of Rashba splitting on the RKKY interaction in TI thin film both at finite and zero chemical potential. We find that the spin susceptibility of Rashba materials including TI thin film is strongly dependent on the direction of distance vector. Moreover, we find another term in the off-diagonal terms of the spin-susceptibility tensor which in contrast to the well-known DM-like term is symmetric. We show how one can tune the RKKY interaction by using electric field applied perpendicularly to the surface plane and by small chemical doping giving rise to…
Two-dimensional topological insulators (TIs) host gapless helical edge states that are predicted to support a quantized two-terminal conductance. Quantization is protected by time-reversal symmetry, which forbids elastic backscattering. Paradoxically, the current-carrying state itself breaks the time-reversal symmetry that protects it. Here we show that the combination of electron-electron interactions and momentum-dependent spin polarization in helical edge states gives rise to feedback through which an applied current opens a gap in the edge state dispersion, thereby breaking the protection …
We report the observation of ferromagnetic resonance-driven spin pumping signals at room temperature in three-dimensional topological insulator thin films -- Bi2Se3 and (Bi,Sb)2Te3 -- deposited by molecular beam epitaxy on yttrium iron garnet thin films. By systematically varying the Bi2Se3 film thickness, we show that the spin-charge conversion efficiency, characterized by the inverse Rashba-Edelstein effect length (lambda_IREE), increases dramatically as the film thickness is increased from 2 quintuple layers, saturating above 6 quintuple layers. This suggests a dominant role of surface stat…
Achieving combination of spin and valley polarized states with topological insulating phase is pregnant to promote the fantastic integration of topological physics, spintronics and valleytronics. In this work, a spin-valley-coupled quantum spin Hall insulator (svc-QSHI) is predicted in Janus monolayer $\mathrm{CSb_{1.5}Bi_{1.5}}$ with dynamic, mechanical and thermal stabilities. The inequivalent valleys have opposite Berry curvature and spin moment, which can produce a spin-valley Hall effect. In the center of Brillouin zone, a Rashba-type spin splitting can be observed due to missing horizont…
We report the observation of efficient charge-to-spin conversion in the three-dimensional topological insulator (TI) Bi2Se3 and Ag bilayer by the spin-torque ferromagnetic resonance technique. The spin orbit torque ratio in the Bi2Se3/Ag/CoFeB heterostructure shows a significant enhancement as the Ag thickness increases to ~2 nm and reaches a value of 0.5 for 5 nm Ag, which is ~3 times higher than that of Bi2Se3/CoFeB at room temperature. The observation reveals the interfacial effect of Bi2Se3/Ag exceeds that of the topological surface states (TSS) in the Bi2Se3 layer and plays a dominant rol…
Topological Flat Minibands and Fractional Chern Insulators in Rashba Systems with Tunable Superlattice Potentials
University of Science and Technology of China（中国科学技术大学）；International Center for Quantum Design of Functional Materials (ICQD), Hefei National Research Center for Physical Sciences at Microscale, University of Science and Technology of China（中国科学技术大学合肥微尺度物质科学国家研究中心量子功能材料国际中心）；Hefei National Laboratory, University of Science and Technology of China（中国科学技术大学合肥国家实验室）
Three-dimensional topological insulators (TIs) exhibit time-reversal symmetry protected, linearly dispersing Dirac surface states. Band bending at the TI surface may also lead to coexisting trivial two-dimensional electron gas (2DEG) states with parabolic energy dispersion that exist as spin-split pairs due to Rashba spin-orbit coupling (SOC). A bias current is expected to generate spin polarization in both systems arising from their helical spin-momentum locking. However, their induced spin polarization is expected to be different in both magnitude and sign. Here, we compare spin potentiometr…
Three-dimensional topological insulators protected by both the time reversal (TR) and mirror symmetries were recently predicted and observed. Two-dimensional materials featuring this property and their potential for device applications have been less explored. We find that in these systems, the spin-polarization of edge states can be controlled with an external electric field breaking the mirror symmetry. This symmetry requires that the spin-polarization is perpendicular to the mirror plane, therefore, the electric field induces spin-polarization components parallel to the mirror plane. Since …
In the quest for topological insulators with large band gaps, heterostructures with Rashba spin-orbit interactions come into play. Transition metal oxides with heavy ions are especially interesting in this respect. We discuss the design principles for stacking oxide Rashba layers. Assuming a single layer with a two-dimensional electron gas (2DEG) on both interfaces as a building block, a two-dimensional topological insulating phase is present when negative coupling between the 2DEGs exists. When stacking multiple building blocks, a two-dimensional or three-dimensional topological insulator is …
We theoretically consider spin pumping in a junction between a ferromagnetic insulator (FI) and a two-dimensional electron gas (2DEG) in which the Rashba and Dresselhaus spin-orbit interactions coexist. Using second-order perturbation theory, we derive an increase in linewidth in the case of an interfacial exchange coupling in a ferromagnetic resonance (FMR) experiment. We clarify how the enhancement of Gilbert damping depends on the resonant frequency and spin orientation of the FI. We show that this setup of an FMR experiment can provide information on the spin texture of 2DEG at the Fermi s…
We proposed that the simultaneous presence of both Rashba and band inversion can lead to a Rashba-like spin-splitting formed by two bands with the same in-plane helical spin texture. Because of this unconventional spin texture, the backscattering is forbidden in edge and bulk conductivity channels. We propose a new non-centrosymmetric honeycomb-lattice quantum spin Hall (QSH) insulator family formed by the IV, V, and VII elements with this property. The system formed by Bi, Pb and I atoms is mechanically stable and has both a large Rashba spin-splitting of 60 meV and a large nontrivial band ga…
Rashba spin-orbit interaction leads to a number of electromagnetic cross-correlation effects by inducing a mixing of electric and magnetic degrees of freedom. In this study, we investigate the optical properties of a magnetic Rashba conductor by deriving an effective Hamiltonian based on an imaginary-time path-integral formalism. We show that the effective Hamiltonian can be described in terms of toroidal and quadrupole moments, as has been argued in the case of insulator multiferroics. The toroidal moment turns out to coincide with the spin gauge field induced by the Rashba field. It causes D…
In materials lacking inversion symmetry, the spin-orbit coupling enables the direct connection between the electron's spin and its linear momentum, a phenomenon called inverse spin galvanic effect. In magnetic materials, this effect promotes current-driven torques that can be used to control the magnetization direction electrically. In this work, we investigate the current-driven inverse spin galvanic effect in a quantum well consisting in a magnetic material embedded between dissimilar insulators. Assuming the presence of Rashba spin-orbit coupling at the interfaces, we investigate the nature…
We investigate the change in the non-zero Chern number and out-of-plane spin polarization of the edge currents in a honeycomb lattice with the Haldane-Rashba interaction. This interaction breaks the time-reversal symmetry due to the Haldane phase caused by a current loop at site-I and -II atoms and also accounts for the Rashba-type spin-orbit interaction. The Rashba spin-orbit interaction increases the number of Dirac points and the band-touching phenomenon can be generated by tuning the on-site potential in the non-zero Haldane phase. By using the Pontryagin winding number and numerical Berry…
We propose an experimental realization of the Spin Hall effect in graphene by illuminating a graphene sheet on top of a substrate with circularly polarized monochromatic light. The substrate induces a controllable Rashba type spin-orbit coupling which breaks the spin-degeneracy of the Dirac cones but it is gapless. The circularly polarized light induces a gap in the spectrum and turns graphene into a Floquet topological insulator with spin dependent edge states. By analyzing the high and intermediate frequency regimes, we find that in both parameter limits, the spin-Chern number can be tuned b…
We discuss the transport properties of a quantum spin-Hall insulator with sizable Rashba spin-orbit coupling in a disk geometry. The presence of topologically protected helical edge states allows for the control and manipulation of spin polarized currents: when ferromagnetic leads are coupled to the quantum spin-Hall device, the ballistic conductance is modulated by the Rashba strength. Therefore, by tuning the Rashba interaction via an all-electric gating, it is possible to control the spin polarization of injected electrons.
In this work we analytically investigate the longitudinal optical conductivity of the C$_{2v}$ symmetric topological insulator. The conductivity expressions at $ T = 0 $ are derived using the Kubo formula and expressed as a function of the ratio of the Dresselhaus and Rashba parameters that characterize the low-energy Hamiltonian. We find that the longitudinal inter-band conductivity vanishes when Dresselhaus and Rashba parameters are equal in strength, also called the persistent spin helix state. The calculations are extended to obtain the frequency-dependent real and imaginary components of …
The inverse Rashba-Edelstein effect (IREE) is a spin conversion mechanism that recently attracts attention in spintronics and condensed matter physics. In this letter, we report an investigation of the IREE in Bi/Ag by using ferrimagnetic insulator yttrium iron garnet (YIG). We prepared two types of samples with opposite directions of the Rashba field by changing a stacking order of Bi and Ag. An electric current generated by the IREE was observed from both stacks, and an efficiency of spin conversion -characterized by the IREE length- was estimated by taking into account a number of contribut…
