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arXiv 2106.04017cond-mat.str-elcond-mat.mtrl-sci
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一维共角铜氧化物动力学自旋和电荷结构因子中的粒子-空穴不对称性

Particle-hole asymmetry in the dynamical spin and charge structure factors of the corner-shared one-dimensional cuprates

Shaozhi Li, Alberto Nocera, Umesh Kumar, Steven Johnston

摘要:

掺杂铜氧化物的集体自旋和电荷激发及其与超导性的关系尚未完全理解,特别是在电荷激发的情况下。本文采用数值精确方法研究了一维角共享自旋链铜氧化物单轨道和多轨道模型中掺杂相关的自旋和电荷结构因子。我们发现单带哈伯德模型可以描述$pd$模型在低能区的自旋和电荷激发,包括自旋响应中的粒子-空穴不对称性。然而,我们的结果也表明,铜和O轨道之间的轨道间自旋激发的重量是可比的两个铜轨道之间的自旋激发的重量。这一发现阐明了一维铜氧化物中自旋激发的微观本质,并揭示了其他氧化物的自旋性质。重要的是,我们发现了一个粒子-空穴不对称的轨道分辨的电荷激发,这不能描述的单带哈伯德模型和相关的共振非弹性X射线散射实验。我们的研究结果意味着,明确列入氧自由度可能需要理解实验观察。

英文摘要:

The collective spin and charge excitations of doped cuprates and their relationship to superconductivity are not yet fully understood, particularly in the case of the charge excitations. Here, we study the doping-dependent dynamical spin and charge structure factors of single and multi-orbital models for the one-dimensional corner shared spin-chain cuprates using several numerically exact methods. We find that the singleband Hubbard model can describe the spin and charge excitations of the $pd$-model in the low-energy region, including the particle-hole asymmetry in the spin response. However, our results also reveal that the weight of the interorbital spin excitations between Cu and O orbitals is comparable to the weight of the spin excitations between two Cu orbitals. This finding elucidates the microscopic nature of the spin excitations in the 1D cuprates and sheds light on the spin properties of other oxides. Importantly, we find a particle-hole asymmetry in the orbital-resolved charge excitations, which cannot be described by the singleband Hubbard model and is relevant to resonant inelastic x-ray scattering experiments. Our results imply that the explicit inclusion of the oxygen degrees of freedom may be required to understand experimental observations.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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