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arXiv 2106.01358cond-mat.mes-hall
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Kekulé序石墨烯中的自能动力学与模式特异性声子阈值效应

Self-energy dynamics and mode-specific phonon threshold effect in a Kekulé-ordered graphene

Hongyun Zhang, Changhua Bao, Michael Schüler, Shaohua Zhou, Qian Li, Laipeng Luo, Wei Yao, Zhong Wang, Thomas P. Devereaux, Shuyun Zhou

AI总结:

针对石墨烯弛豫动力学中特定声子模式作用难以直接明确的问题,通过对Kekulé序石墨烯开展时间-角分辨光电子能谱测量,解析了两种声子耦合的自能效应及时域变化,证实模式特异性声子的主导作用。

摘要:

电子-声子相互作用及相关自能是固体平衡性质与非平衡弛豫动力学的基础。尽管各类时间分辨测量已表明电子-声子相互作用对石墨烯的弛豫动力学至关重要,但由于缺乏能量和动量分辨的自能动力学研究,无法直接明确特定声子模式在弛豫动力学中的作用。本文通过对Γ点处存在折叠狄拉克锥的Kekulé序石墨烯开展时间-角分辨光电子能谱测量,成功解析了电子与Ω₁=177 meV和Ω₂=54 meV这两个声子耦合所产生的自能效应,并揭示了其在时域内的动态变化。此外,这些强耦合声子定义了能量阈值,将层级弛豫动力学划分为超快、快速与慢速三个阶段,从而为模式特异性声子在弛豫动力学中的主导作用提供了直接实验证据。

英文摘要:

Electron-phonon interaction and related self-energy are fundamental to both the equilibrium properties and non-equilibrium relaxation dynamics of solids. Although electron-phonon interaction has been suggested by various time-resolved measurements to be important for the relaxation dynamics of graphene, the lack of energy- and momentum-resolved self-energy dynamics prohibits direct identification of the role of specific phonon modes in the relaxation dynamics. Here by performing time- and angle-resolved photoemission spectroscopy measurements on a Kekulé-ordered graphene with folded Dirac cones at the $Γ$ point, we have succeeded in resolving the self-energy effect induced by coupling of electrons to two phonons at $Ω_1$ = 177 meV and $Ω_2$ = 54 meV and revealing its dynamical change in the time domain. Moreover, these strongly coupled phonons define energy thresholds, which separate the hierarchical relaxation dynamics from ultrafast, fast to slow, thereby providing direct experimental evidence for the dominant role of mode-specific phonons in the relaxation dynamics

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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