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arXiv 2104.09385physics.optics
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极紫外飞秒脉冲在单原子材料中的非线性自驱动光谱调谐

Non-linear self-driven spectral tuning of Extreme Ultraviolet Femtosecond Pulses in monoatomic materials

Carino Ferrante, Emiliano Principi, Andrea Marini, Giovanni Batignani, Giuseppe Fumero, Alessandra Virga, Laura Foglia, Riccardo Mincigrucci, Alberto Simoncig, … 展开作者

Carino Ferrante, Emiliano Principi, Andrea Marini, Giovanni Batignani, Giuseppe Fumero, Alessandra Virga, Laura Foglia, Riccardo Mincigrucci, Alberto Simoncig, Carlo Spezzani, Claudio Masciovecchio, Tullio Scopigno

摘要:

自作用非线性是一个关键方面-无论是作为一个基本要素或有害因素-的一些光学光谱和光子器件。超连续谱产生、波长转换器和啁啾脉冲放大只是几个例子。最近自由电子激光(FEL)的出现促进了非线性的发展,提出了新的概念,并扩展了极紫外(EUV)和X射线的光波长范例。然而,在如此短的波长下,没有关于脉冲内动力学的证据,在这种情况下,光与物质的相互作用由核心电子的尖锐吸收边决定。在这里,我们提供了飞秒自由电子激光脉冲的自相位调制的实验证据,我们利用精细的自驱动光谱可调谐性与选定的单原子材料的亚微米箔的相互作用。将脉冲波长移过吸收边,光谱轮廓从非线性光谱蓝移变为红移加宽。这些发现是合理的占超快电离和延迟的热响应的高度激发的电子高于和低于阈值,分别。

英文摘要:

Self-action nonlinearity is a key aspect -- either as a foundational element or a detrimental factor -- of several optical spectroscopies and photonic devices. Supercontinuum generation, wavelength converters and chirped pulse amplification are just a few examples. The recent advent of Free Electron Lasers (FEL) fostered building on nonlinearity to propose new concepts and extend optical wavelengths paradigms for extreme ultraviolet (EUV) and X-ray regimes. No evidence for intrapulse dynamics, however, has been reported at such short wavelengths, where the light-matter interactions are ruled by the sharp absorption edges of core-electrons. Here, we provide experimental evidence for self-phase modulation of femtosecond FEL pulses, which we exploit for fine self-driven spectral tunability by interaction with sub-micrometric foils of selected monoatomic materials. Moving the pulse wavelength across the absorption edge, the spectral profile changes from a non-linear spectral blue-shift to a red-shifted broadening. These findings are rationalized accounting for ultrafast ionization and delayed thermal response of highly excited electrons above and below threshold, respectively.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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