The short timescale spin dynamics in antiferromagnets is an attractive feature from the standpoint of ultrafast spintronics. Yet generating highly polarized spin currents at room temperature remains a fundamental challenge for antiferromagnets. We propose a spin circular photogalvanic effect (spin-CPGE), in which circularly polarized light can produce a spin current without net charge current at room temperature, through an "injection-current-like" mechanism in parity-time(PT)-symmetric antiferromagnetic (AFM) insulators. We demonstrate this effect by first-principles simulations of bilayer CrI3 and room-temperature AFM hematite. Our calculations show that the spin-CPGE is significant, and the magnitude of spin photo-current is comparable with the widely observed charge photocurrent in ferroelectric materials. Interestingly, this spin photocurrent is not sensitive to spin-orbit interactions, which were regarded as fundamental mechanisms for generating spin current. Given the fast response of light-matter interactions, large energy scale, and insensitivity to spin-orbit interactions, our work gives hope to realizing a fast-dynamic and temperature-robust pure spin current in a wide range of PT-symmetric AFM materials, including weak-relativistic magnetic insulators and topological axion insulators.
Interface-Controlled Antiferromagnetic Tunnel Junctions based on a metallic van der Waals A-type Antiferromagnet
Hefei University of Technology(合肥工业大学);University of Science and Technology of China(中国科学技术大学);Agency for Science Technology and Research (A*STAR)(科学与技术研究局);Anhui University(安徽大学);RMIT University(皇家墨尔本理工大学)
Spectrally Programmable Spin-Polarized Photocurrents in WSe$_2$-NiPS$_3$ Magnetic van der Waals Heterostructures
Bar-Ilan University(巴伊兰大学);Technical University of Darmstadt(达姆施塔特工业大学);Technische Universität Dresden(德累斯顿工业大学);Center for Advanced Systems Understanding, CASUS, HZDR(先进系统理解中心,CASUS,HZDR);Yonsei University(延世大学)
Disentangling magnetic and optical contributions in ultrafast dynamics of antiperovskite non-collinear antiferromagnets
Charles University(查理大学);University of Cambridge(剑桥大学);University of Glasgow(格拉斯哥大学);Czech Technical University(捷克理工大学);LoMaRe Technologies Ltd.(洛玛雷科技有限公司);Jiangsu LoMaRe Chip Technology Co., Ltd.(江苏洛玛雷芯片技术有限公司)
Magnetic and crystal electric field excitations in a spin-orbit coupled frustrated hyperkagome magnet Nd$_3$Li$_3$W$_2$O$_{12}$
Indian Institute of Science Education and Research Thiruvananthapuram(印度科学教育研究所特里凡得琅分校);Technical University of Denmark(丹麦技术大学);Forschungszentrum Jülich GmbH(于利希研究中心有限公司);RWTH Aachen(亚琛工业大学);ISIS Neutron and Muon Source, Science and Technology Facilities Council, Rutherford Appleton Laboratory(ISIS中子与μ子源,英国科学与技术设施委员会,卢瑟福阿普顿实验室)