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arXiv 2104.08341cond-mat.mtrl-scicond-mat.mes-hallphysics.optics
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反铁磁绝缘体中PT对称性使能的自旋圆光电流效应

PT-symmetry enabled spin circular photogalvanic effect in antiferromagnetic insulators

Ruixiang Fei, Wenshen Song, Lauren Pusey-Nazzaro, Li Yang

摘要:

从超快自旋电子学的观点来看,反铁磁体中的短时间尺度自旋动力学是一个很有吸引力的特性。然而,在室温下产生高度极化的自旋电流仍然是反铁磁体的一个基本挑战。提出了一种自旋圆光电流效应(spin-circular photocalvanic effect,spin-CPGE),即圆偏振光在室温下通过“类注入电流”机制在宇称时间(parity-time,PT)对称反铁磁(antiferromagnetic,AFM)绝缘体中产生自旋电流而不产生净电荷电流.我们证明了这种效果的第一性原理模拟双层CrI 3和室温AFM赤铁矿。我们的计算表明,自旋CPGE是显着的,并且自旋光电流的大小与铁电材料中广泛观察到的电荷光电流相当。有趣的是,这种自旋光电流对自旋轨道相互作用不敏感,而自旋轨道相互作用被认为是产生自旋电流的基本机制。鉴于光-物质相互作用的快速响应,大的能量尺度,以及对自旋-轨道相互作用的不敏感性,我们的工作有望在广泛的PT对称AFM材料中实现快速动态和温度鲁棒的纯自旋电流,包括弱相对论磁性绝缘体和拓扑轴子绝缘体。

英文摘要:

The short timescale spin dynamics in antiferromagnets is an attractive feature from the standpoint of ultrafast spintronics. Yet generating highly polarized spin currents at room temperature remains a fundamental challenge for antiferromagnets. We propose a spin circular photogalvanic effect (spin-CPGE), in which circularly polarized light can produce a spin current without net charge current at room temperature, through an "injection-current-like" mechanism in parity-time(PT)-symmetric antiferromagnetic (AFM) insulators. We demonstrate this effect by first-principles simulations of bilayer CrI3 and room-temperature AFM hematite. Our calculations show that the spin-CPGE is significant, and the magnitude of spin photo-current is comparable with the widely observed charge photocurrent in ferroelectric materials. Interestingly, this spin photocurrent is not sensitive to spin-orbit interactions, which were regarded as fundamental mechanisms for generating spin current. Given the fast response of light-matter interactions, large energy scale, and insensitivity to spin-orbit interactions, our work gives hope to realizing a fast-dynamic and temperature-robust pure spin current in a wide range of PT-symmetric AFM materials, including weak-relativistic magnetic insulators and topological axion insulators.

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