Cooper pairs featuring a nonzero center-of-mass crystal momentum ${\boldsymbol Q}=(π,π, \dots)$ and an off-diagonal long-range order ($η$-pairing states) constitute exact eigenstates of a Hubbard model [C. N. Yang, Phys. Rev. Lett. 63, 2144 (1989)]. Here we show that the $η$-pairing states are rendered dynamically unstable via coupling to dynamical electromagnetic fields. The instability is caused by "tachyonic" electromagnetic fields and unstable plasma modes for attractive and repulsive interactions, respectively. The typical time scale of the growth of the instability is of the order of femtoseconds for electron systems in solids, which places a strict bound on the lifetime of the $η$-pairing states. The decay of the $η$-pairing states leads to enhanced light emission with frequencies shifted from the Hubbard interaction strength for the repulsive case and unattenuated electromagnetic penetration for the attractive case.
Motivated by the surge in research activities on graphene, we investigate instabilities of electrons on the honeycomb lattice, interacting by onsite and nearest-neighbor terms, using a renormalization group scheme. Near half band-filling, critical minimal interaction strengths are required for instabilities toward antiferromagnetic or charge-density wave order. Away from half filling, f-wave triplet pairing and d+id singlet pairing instabilities are found to emerge out of density-wave regimes.
Electron pairing and ferromagnetism in various cluster geometries are studied with emphasis on tetrahedron and square pyramid under variation of interaction strength, electron doping and temperature. These exact calculations of charge and spin collective excitations and pseudogaps yield intriguing insights into level crossing degeneracies, phase separation and condensation. Criteria for spin-charge separation and reconciliation driven by interaction strength, next nearest coupling and temperature are found. Phase diagrams resemble a number of inhomogeneous, coherent and incoherent nanoscale ph…
There is growing evidence that the unconventional spatial inhomogeneities in the doped high-Tc superconductors are accompanied by the pairing of electrons, subsequent quantum phase transitions (QPTs), and condensation in coherent states. We show that these superconducting states can be obtained from phase separation instabilities near the quantum critical points. We examine electron coherent and incoherent pairing instabilities using our results on exact diagonalization in pyramidal and octahedron Hubbard-like clusters under variation of chemical potential (or doping), interaction strength, te…
Using a renormalization group approach, we determine the phase diagram of an extended quasi-one-dimensional electron gas model that includes interchain hopping, nesting deviations and both intrachain and interchain repulsive interactions. We find a close proximity of spin-density- and charge-density-wave phases, singlet d-wave and triplet f-wave superconducting phases. There is a striking correspondence between our results and recent puzzling experimental findings in the Bechgaard salts, including the coexistence of spin-density-wave and charge-density-wave phases and the possibility of a trip…
The interplay of non-Fermi liquid and superconductivity born out of strong dynamical interactions is at the heart of the physics of unconventional superconductivity. As a solvable platform of the strongly correlated superconductors, we study the pairing instabilities of the Yukawa-Sachdev-Ye-Kitaev (Yukawa-SYK) model, which describes spin-1/2 fermions coupled to bosons by the random, all-to-all, spin-independent and dependent Yukawa interactions. In contrast to the previously studied models, the random Yukawa couplings are sampled from a collection of Gaussian ensembles whose variances follow …
Using finite-temperature determinantal quantum Monte Carlo calculations, we re-examine the pairing susceptibilities in the Hubbard model on the honeycomb lattice, focusing on doping levels onto and away from the van Hove singularity (VHS) filling. For this purpose, electronic densities of $0.75$ (at the hole-doping VHS) and $0.4$ (well below the VHS) are considered in detail, where due to a severe sign problem at strong coupling strengths, we focus on the weak interaction region of the Hubbard model Hamiltonian. From analyzing the temperature dependence of pairing susceptibilities in various s…
Exact calculations of collective excitations and charge/spin (pseudo)gaps in an ensemble of bipartite and nonbipartite clusters yield level crossing degeneracies, spin-charge separation, condensation and recombination of electron charge and spin, driven by interaction strength, inter-site couplings and temperature. Near crossing degeneracies, the electron configurations of the lowest energies control the physics of electronic pairing, phase separation and magnetic transitions. Rigorous conditions are found for the smooth and dramatic phase transitions with competing stable and unstable inhomog…
We studied the electronic Raman spectra of (Li$_{1-x}$Fe$_x$)OHFeSe as a function of light polarization and temperature. In the B$_{1g}$ spectra alone we observe the redistribution of spectral weight expected for a superconductor and two well-resolved peaks below T$_c$. The nearly resolution-limited peak at 110 cm$^{-1}$ (13.6 meV) is identified as a collective mode. The peak at 190 cm$^{-1}$ (23.6 meV) is presumably another collective mode since the line is symmetric and its energy is significantly below the gap energy observed by single-particle spectroscopies. Given the experimental band st…
In the recently discovered Co-oxide superconductor Na_xCoO_2*yH_2O, the edge-shared CoO6 octahedra are trigonally contracted along the c-axis in the CoO2-plane. We study how this CoO6 distortion affects the magnetic properties and superconductivity in this compound by analyzing the multiorbital Hubbard model using the fluctuation-exchange approximation. It is shown that through generating the trigonal crystal field, the distortion pushes the Co e'g bands up and consequently gives rise to the hole-pocket Fermi surfaces, which have been predicted in the band calculations. As the distortion incre…
Spontaneous phase separation instabilities with the formation of various types of charge and spin pairing (pseudo)gaps in $U>0$ Hubbard model including the {\it next nearest neighbor coupling} are calculated with the emphasis on the two-dimensional (square) lattices generated by 8- and 10-site Betts unit cells. The exact theory yields insights into the nature of quantum critical points, continuous transitions, dramatic phase separation instabilities and electron condensation in spatially inhomogeneous systems. The picture of coupled anti-parallel (singlet) spins and paired charged holes sugges…
We use a novel temperature-flow renormalization group technique to analyze magnetic and superconducting instabilities in the two-dimensional t-t' Hubbard model for particle densities close to the van Hove filling as a function of the next-nearest neighbor hopping t'. In the one-loop flow at the van Hove filling, the characteristic temperature for the flow to strong coupling is suppressed drastically around t'_c approx. -0.33t, suggesting a quantum critical point between d-wave pairing at moderate t'>t'_c and ferromagnetism for t'<t'_c. Upon increasing the particle density in the latter regime …
Fluctuating local diamagnetic pairs of electrons, embedded in a Fermi sea, are candidates for non-phonon-mediated superconductors without the stringent conditions on Tc which arise in phonon-mediated BCS classical low-Tc superconductors. The local accumulations of charge, from which such diamagnetic fluctuations originate, are irrevocably coupled to local dynamical lattice instabilities and form composite charge-lattice excitations of the system. For a superconducting phase to be realized, such excitations must be itinerant spatially phase-coherent modes. This can be achieved by resonant pair …
The Bethe-Salpeter equation is combined with the temperature-cutoff functional renormalization group approach to analyze the order parameter structure for the leading instabilities of the 2D t-t' Hubbard model. We find significant deviations from pure s-, d-, or p-wave forms, which is due to the frustration of antiferromagnetism at small and intermediate t'. With adding a direct antiferromagnetic spin-exchange coupling the eigenfunctions in the particle-hole channel have extended s-wave form, while in the particle-particle singlet pairing channel a higher angular momentum component arises besi…
We apply the fermion renormalization group method, implemented numerically by Honerkamp et.al., to a two-band model of FeAs-based materials. At half filling we find the $(π,0)$ or $(0,π)$ spin density wave order and a sub-dominant superconducting pairing tendency. Due to a topological reason, the spin density wave gap has nodes on the fermi surfaces. Away from half filling we find an unconventional s-wave and a sub-dominant $d_{x^2-y^2}$ pairing instability. The former has $s$ symmetry around the hole fermi surface but exhibits $s+d_{x^2-y^2}$ symmetry around the electron pockets where the 90 …
A BCS (Bardeen-Cooper-Schrieffer) superconductor, which is placed out of equilibrium, can develop quantum instabilities, which manifest themselves in oscillations of the superconductor's order parameter (pairing amplitude $Δ$). These instabilities are a manifestations of the Cooper instability. Inelastic collisions are essential in resolving those instabilities. Incorporating the quantum instabilities and collisions in a unified approach based on Richardson's exact solution of the pairing Hamiltonian, we find that a BCS superconductor may end up in a state in which the spectrum has more than o…
In certain unconventional superconductors with sizable electronic correlations, the availability of closely competing pairing channels leads to characteristic soft collective fluctuations of the order parameters, which leave fingerprints in many observables and allow to scrutinize the phase competition. Superconducting layered materials, where electron-electron interactions are enhanced with decreasing thickness, are promising candidates to display these correlation effects. In this work, we report the existence of a soft collective mode in single-layer NbSe$_2$, observed as a characteristic r…
The recent discovery of AV$_3$Sb$_5$ (A=K,Rb,Cs) has uncovered an intriguing arena for exotic Fermi surface instabilities in a kagome metal. Among them, superconductivity is found in the vicinity of multiple van Hove singularities, exhibiting indications of unconventional pairing. We show that the sublattice interference mechanism is central to understanding the formation of superconductivity in a kagome metal. Starting from an appropriately chosen minimal tight-binding model with multiple with multiple van Hove singularities close to the Fermi level for AV$_3$Sb$_5$, we provide a random phase…
Motivated by the experimental detection of superconductivity in the low-carrier density half-Heusler compound YPtBi, we study the pairing instabilities of three-dimensional strongly spin-orbit coupled semimetals with a quadratic band touching point. In these semimetals the electronic structure at the Fermi energy is described by spin j=3/2 quasiparticles, which are fundamentally different from those in ordinary metals with spin j=1/2. We develop a general approach to analyzing pairing instabilities in j=3/2 materials by decomposing the pair scattering interaction into irreducible channels, pro…
We study the superconducting instabilities of singlet and triplet pairing in a two-dimensional Hubbard model on the basis of the third-order perturbation theory (TOPT). We investigate the effect of the vertex correction that is given by TOPT, comparing with the study with only the second-order effective interaction. In our results, a stable p-wave pairing state spreads from low to intermediate electron density. A dx2-y2-wave pairing is dominant for the high density near a half-filling. It is shown that the vertex correction plays an essential role in making the p-wave pairing state dominant.
Recent experiments on the organic compound κ-(ET)_2Cu_2(CN)_3 have provided a promising example of a two dimensional spin liquid state. This phase is described by a two-dimensional spinon Fermi sea coupled to a U(1) gauge field. We study Kohn-Luttinger-like pairing instabilities of the spinon Fermi surface due to singular interaction processes with twice-the-Fermi-momentum transfer. We find that under certain circumstances the pairing instability occurs in odd-orbital-angular-momentum/spin-triplet channels. Implications to experiments are discussed.
The superconductor Sr2RuO4 has been the subject of enormous interest over more than two decades, but until now the form of its order parameter has not been determined. Since groundbreaking NMR experiments revealed that the pairs are of dominant spin-singlet character, attention has focused on time-reversal symmetry breaking linear combinations of $s$-, $d$- and $g$-wave one-dimensional (1D) irreducible representations. However, a state of the form $d_{xz}+id_{yz}$ has also been proposed. We present a systematic study of the stability of various superconducting candidate states, assuming that p…
We discuss the low energy theory of two-dimensional metals near the onset of spin density wave order. It is well known that such a metal has a superconducting instability induced by the formation of spin-singlet pairs of electrons, with the pairing amplitude changing sign between regions of the Fermi surface connected by the spin density wave ordering wavevector. Here we review recent arguments that there is an additional instability which is nearly as strong: towards the onset of a modulated bond order which is locally an Ising-nematic order. This new instability is a consequence of an emerge…
We present an approach for determining susceptibilities and order parameters in multi-band Hubbard model within functional renormalization group method, and apply it to study various instabilities of the FeAs-based high temperature superconductor. First, we derive the formulae of susceptibilities and order parameters of superconducting parings, spin density waves and charge density waves with diverse wave vectors which could occur in multi-band Hubbard model. Second, we apply it to the FeAs-based high temperature superconductor and find an electronic-driven superconducting pairing instability …
Electron instabilities in the Hubbard model with the next nearest neighbor coupling are calculated by exact diagonalization in finite, two-dimensional Betts cells (lattices). A viable spin and charge coherent pairing, signaled by quantum critical points and a negative charge gap region, is found in 8- and 10-site Betts lattices at small and moderate U regions consistent with our exact results in elementary bipartite geometries [Phys. Rev. B 78 (2008) 075431]. The contour isolines for continuous temperature driven-crossover between the Mott-Hubbard insulating and coherent pairing phases are dem…
We study the superconducting pairing instabilities and gap functions for prototypical two-dimensional (2D) transition-metal dichalcogenides (TMDCs) WS$_2$, MoTe$_2$, and MoS$_2$ in the 2H phase under both hole and electron doping at 10 K. Our first-principles quantum many-body Green's function approach allows us to treat the full $d$ and $p$ manifold of orbitals with strong spin-orbit coupling, yielding pairing predictions with material specific detail. The resulting gap functions exhibit a variety of mixed-parity superconducting states, including $s$, $p$, $d$, $f$, $d\pm id$, and $p\pm ip$ p…
The one-band extended Hubbard model in two dimensions near band-filling 1/2 is solved in the fluctuation exchange approximation, including the long-range (1/r) part of the Coulomb interaction, up to 4th neighbor distance. Our results suggest that d_(x^2 - y^2) pairing in the Hubbard model is robust against the inclusion of long-range Coulomb interactions with moderate 1st neighbor repulsion strength V_1. d_(x^2 - y^2) pairing is suppressed only at large V_1 (>~ 0.25U-0.4U), due to incipient charge density wave instabilities.
In analogy with ordinary BCS superconductivity, we identify possible pairing instabilities with poles in a certain class of Green functions of the two-dimensional repulsive Hubbard model, which normally signify bound states. Relating the gap to the location of these poles, we find that these instabilities exist in the range of hole doping between 0.03 and 0.24. The magnitude of the gap can be calculated without introducing an explicit cut-off, and for reasonably large coupling U/t = 10, the maximum gap is on the order of 0.08 in units of the hopping parameter t.
Motivated by recent experiments on atomic Dirac fermions in a tunable honeycomb optical lattice, we study the attractive Hubbard model of superfluidity in the anisotropic honeycomb lattice. At weak-coupling, we find that the maximum mean field pairing transition temperature, as a function of density and interaction strength, occurs for the case with isotropic hopping amplitudes. In this isotropic case, we go beyond mean field theory and study collective fluctuations, treating both pairing and density fluctuations for interaction strengths ranging from weak to strong coupling. We find evidence …
We construct a family of translationally invariant lattice models with a large number ($N$) of orbitals at every site coupled together via single electron tunneling. By tuning the relative strength of the electronic bandwidth and on-site interactions, that have a modified Sachdev-Ye-Kitaev (SYK) form, we demonstrate a number of unusual features at strong coupling and in the large$-N$ limit. We find examples of (i) an intrinsic non-BCS superconducting instability arising out of an incoherent non-Fermi liquid metal, and, (ii) an instability of an incipient heavy Fermi liquid metal to superconduc…
Superconductivity in many strongly correlated materials appears in proximity to a density-wave or nematic order and is believed to be mediated by quantum-critical (QC) fluctuations of the corresponding order parameter. We argue that fingerprints of QC pairing can be extracted from the angular dependence of the gap $Δ(θ)$. We consider pairing by QC nematic fluctuations and show that there exist multiple pairing instabilities within the same symmetry ($s-$wave in our case), with closely spaced transition temperatures $T_{c,n}$. The corresponding $Δ_n (θ)$ change sign $8n$ times along the FS. Onl…
We studied the pairing instabilities in K$_x$Fe$_{2-y}$Se$_2$ using a two stage functional renormalization group (FRG) method. Our results suggest the leading and subleading pairing symmetries are nodeless $d_{x^2-y^2}$ and nodal extended $s$ respectively. In addition, despite having no Fermi surfaces we find the buried hole bands make important contributions to the final effective interaction. From the bandstructure, spin susceptibility and the FRG results we conclude that the low energy effective interaction in K$_x$Fe$_{2-y}$Se$_2$ is well described by a $J_1-J_2$ model with dominant neares…
Proposals for superconductivity emerging from correlated electrons in the doped Hubbard model on the honeycomb lattice range from chiral $d+id$ singlet to $p+ip$ triplet pairing, depending on the considered range of doping and interaction strength, as well as the approach used to analyze the pairing instabilities. Here, we consider these scenarios using large-scale dynamic cluster approximation (DCA) calculations to examine the evolution in the leading pairing symmetry from weak to intermediate coupling strength. These calculations focus on doping levels around the van Hove singularity (VHS) a…
A simple yet paradigmatic model for the interplay of strong electronic correlations and geometric frustration is the triangular lattice Hubbard model. Recently it was proposed that moiré structures of transition metal dichalcogenides can be used to simulate extended versions that include non-local density-density interactions. We study competing instabilities of interacting electrons in such an extended Hubbard model on the triangular lattice near a filling where the density of states has a Van Hove singularity. We employ a truncated-unity functional renormalization group approach to investiga…
We study the phase diagram of a two component Fermi system with a weak attractive interaction. Our analysis includes the leading order Hartree energy shifts and pairing correlations at finite temperature and chemical potential difference between the two fermion species. We show that in an asymmetric system, the Hartree shift to the single particle energies are important for the phase competition between normal and superfluid phase and can change the phase transition curve qualitatively. At large asymmetry we find that a novel but somewhat fragile superfluid state can be favored due to finite t…
We present a systematic classification and analysis of possible pairing instabilities in graphene-based moiré superlattices. Motivated by recent experiments on twisted double-bilayer graphene showing signs of triplet superconductivity, we analyze both singlet and triplet pairing separately, and describe how these two channels behave close to the limit where the system is invariant under separate spin rotations in the two valleys, realizing an SU(2)$_+$ $\times$ SU(2)$_-$ symmetry. Further, we discuss the conditions under which singlet and triplet can mix via two nearly degenerate transitions, …
We study attractively interacting spin-1/2 fermions on the square lattice subject to a spin population imbalance. Using unbiased diagrammatic Monte Carlo simulations we find an extended region in the parameter space where the Fermi liquid is unstable towards formation of Cooper pairs with non-zero center-of-mass momentum, known as the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. In contrast to earlier mean-field and quasi-classical studies we provide quantitative and well-controlled predictions on the existence and location of the relevant Fermi-liquid instabilities. The highest temperature …
Conventional topological superconductors are fully gapped in the bulk but host gapless Majorana modes on their boundaries. We instead focus on a new class of superconductors, second-order topological superconductors, that have gapped, topological surfaces and gapless Majorana modes instead on lower-dimensional boundaries, i.e., corners of a two-dimensional system or hinges for a three-dimensional system. Here we propose two general scenarios in which second-order topological superconductivity can be realized spontaneously with weak-pairing instabilities. First, we show that $p_x+ip_y$-wave pai…
We study fermion pairing and condensation towards an ordered state in strongly coupled quantum critical systems with a holographic AdS/CFT dual. On the gravity side this is modeled by a system of charged fermion interacting through a BCS coupling. At finite density such a system has a BCS instability. We combine the relativistic version of mean-field BCS with the semi-classical fluid approximation for the many-body state of fermions. The resulting groundstate is the AdS equivalent of a charged neutron star with a superconducting core. The spectral function of the fermions confirms that the gro…
