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arXiv 2102.08230cond-mat.mtrl-sci
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Tm $_\textbf{2}$ Cu $_\textbf{2}$ In的Shastry-Sutherland晶格中的自旋玻璃行为

Spin-glass behavior in Shastry-Sutherland lattice of Tm$_\textbf{2}$Cu$_\textbf{2}$In

Baidyanath Sahu, R. Djoumessi Fobasso, Andre M. Strydom

摘要:

通过直流磁化、交流磁化和非平衡动力学研究了$\mathrm{Tm_2Cu_2In}$铁磁相的自旋玻璃行为。电弧熔化的多晶化合物$\mathrm{Tm_2Cu_2In}$以$\mathrm{Mo_2FeB_2}$型四元结构(空间群$P_4/mbm$)结晶。随温度变化的直流磁化强度表现出铁磁行为,居里温度$T_C$ = 32.5 K。零场冷却(ZFC)和场冷却(FC)的磁性曲线显示低于$T_C$的热磁不可逆行为。不可逆温度与场的关系遵循Almeida-Schloss线。交流磁化率结果中频率和交流驱动场相关的异常表明$\mathrm{Tm_2Cu_2In}$中存在自旋玻璃态。磁化强度的时间依赖性进一步支持在$\mathrm{Tm_2Cu_2In}$中观察到的自旋玻璃行为。根据幂律发散和Vogel-Fulcher定律,分析了交流磁化率实部冻结温度的频率依赖性。结果表明,$\mathrm{Tm_2Cu_2In}$属于铁磁正则自旋玻璃类化合物。

英文摘要:

The spin-glass behavior in the ferromagnetic phase of $\mathrm{Tm_2Cu_2In}$ was investigated by dc-, ac-magnetization, and non-equilibrium dynamics characterizations. Arc-melted polycrystalline compound of $\mathrm{Tm_2Cu_2In}$ crystallizes in $\mathrm{Mo_2FeB_2}$-type tetragonal structure (space group $P_4/mbm$). The temperature variation dc-magnetization exhibits a ferromagnetic behavior with Curie temperature $T_C$ = 32.5 K. The zero-field cooled (ZFC) and field cooled (FC) magnetic curves show a thermomagnetic irreversible behavior below $T_C$. The field dependence of irreversible temperature follows Almeida-Thouless line. The frequency and ac-driven field-dependent anomalies in ac-susceptibility results indicate the existence of spin-glass state in $\mathrm{Tm_2Cu_2In}$. The time dependence of magnetization further supports the spin-glass behavior observed in $\mathrm{Tm_2Cu_2In}$. The frequency dependence of the freezing temperature in the real part of ac-susceptibility has been analyzed on the basis power-law divergence and Vogel-Fulcher law. The obtained results revealed that $\mathrm{Tm_2Cu_2In}$ belongs to a ferromagnetic canonical spin-glass class of compounds.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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