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arXiv 2102.02397cond-mat.mtrl-sci
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Bi $_{1-x}$ Sb $_{x}$中Weyl半金属相相干声子的超快散射动力学

Ultrafast scattering dynamics of coherent phonons in Bi$_{1-x}$Sb$_{x}$ in the Weyl semimetal phase

Yuta Komori, Yuta Saito, Paul Fons, Muneaki Hase

摘要:

利用反射式飞秒泵浦-探测技术研究了Bi $_{1-x}$ Sb $_{x}$合金系统中不同成分$x$的超快声子动力学。在几皮秒的退相时间内,在时域内产生并观察到了对应于Bi-Bi,Bi-Sb和Sb-Sb的A $_{1g}$局域振动模的相干光学声子。发现相干光学声子的频率随着Sb组分$x$的变化而变化,更重要的是,当$x$值在0.5- 0.8范围内时,这些声子模式的弛豫时间显著减小。我们认为,声子弛豫动力学不是简单地由合金散射,但显着修改的非谐声子-声子散射与隐含的微小贡献,从电子-声子散射在Weyl半金属相。

英文摘要:

We investigate ultrafast phonon dynamics in the Bi$_{1-x}$Sb$_{x}$ alloy system for various compositions $x$ using a reflective femtosecond pump-probe technique. The coherent optical phonons corresponding to the A$_{1g}$ local vibrational modes of Bi-Bi, Bi-Sb, and Sb-Sb are generated and observed in the time domain with a few picoseconds dephasing time. The frequencies of the coherent optical phonons were found to change as the Sb composition $x$ was varied, and more importantly, the relaxation time of those phonon modes was dramatically reduced for $x$ values in the range 0.5--0.8. We argue that the phonon relaxation dynamics are not simply governed by alloy scattering, but are significantly modified by anharmonic phonon-phonon scattering with implied minor contributions from electron-phonon scattering in a Weyl-semimetal phase.

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