The kinetic magnetoelectric effect is an orbital analogue of the Edelstein effect and offers an additional degree of freedom to control magnetisation via the charge current. Here we theoretically propose a gigantic kinetic magnetoelectric effect in topological insulators and interpret the results in terms of topological surface currents. We construct a theory of the kinetic magnetoelectric effect for a surface Hamiltonian of a topological insulator, and show that it well describes the results by direct numerical calculation. This kinetic magnetoelectric effect depends on the details of the surface, meaning that it cannot be defined as a bulk quantity. We propose that Chern insulators and Z_2 topological insulators can be a platform with a large kinetic magnetoelectric effect, compared to metals by 5 - 8 orders of magnitude, because the current flows only along the surface. We demonstrate the presence of said effect in a topological insulator, identifying Cu$_2$ZnSnSe$_4$ as a potential candidate.
Intrinsic magnetic topological insulator ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ is believed to be an axion insulator in its antiferromagnetic ground state. However, direct identification of axion insulators remains experimentally elusive because the observed vanishing Hall resistance, while indicating the onset of the axion field, is inadequate to distinguish the system from a trivial normal insulator. Using numerical Green's functions, we theoretically demonstrate the quantized magnetoelectric current in a tunnel junction of atomically thin ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ sandwiched be…
We theoretically study magnetoelectric effects in a heterostructure of a generic band insulator and a ferromagnet. In contrast to the kinetic magnetoelectric effect in metals, referred to as the Edelstein effect or the inverse spin galvanic effect, our mechanism relies on virtual interband transitions between the valence and conduction bands and therefore immune to disorder or impurity scattering. By calculating electric field-induced magnetization by the linear response theory, we reveal that the magnetoelectric effect shows up without specific parameter choices. The magnetoelectric effect qu…
Topological magnetoelectric effect (TME) is a hallmark response of the topological field theory, which provides a paradigm shift in the study of emergent topological phenomena. However, its direct observation is yet to be realized due to the demanding magnetic configuration required to gap all the surface states. Here, we theoretically propose that the axion insulators with a simple ferromagnetic configuration, such as MnBi2Te4/(Bi2Te3)n family, provide an ideal playground to realize TME. In a designed triangular prism geometry, all the surface states are magnetically gapped. Under a vertical …
Chromia is a magnetoelectric insulator whose bulk magnetoelectric susceptibility contains a non-zero pseudoscalar component, like that present in magnetized topological insulators. We reveal the dynamic axion field of chromia by measuring the temperature dependence of its non-linear magnetoelectric response using a lock-in technique with an AC electric field stimulus. The electric field dependence, magnetic field dependence, and temperature behavior of the second harmonic lock-in signal are all in agreement with theoretical expectations. Our results demonstrate that chromia magnetoelectric res…
Three-dimensional topological insulators or axion insulators exhibit the topological magnetoelectric effect, which is isotropic with a universal coefficient of proportionality quantized in units of $e^2/2h$. Here we study the finite-size effect of topological magnetoelectric effect, and find the magnetoelectric coefficients are anisotropic, namely $α_{xx}\neqα_{zz}$. Both of them are shown to converge to a quantized value when the thickness of topological insulator film $d$ increases reaching the three-dimensional bulk limit. The nonzero value of $(α_{xx}-α_{zz})\propto1/d$ could be measured b…
Axion insulator is an exotic magnetic topological insulator with zero Chern number but a nonzero quantized Chern-Simons magnetoelectric coupling. A conclusive experimental evidence for axion insulators is still lacking due to the small signal of topological magnetoelectric effect (TME). Here we show that the dynamical magnetoelectric coupling can be induced by the \emph{out-of-plane} surface magnetization dynamics in axion insulator thin films, which further generates a polarization current in the presence of an external magnetic field in the same direction. Such a current is finite in the bul…
Magnetoelectric effect in multiferroic metals via a direct spin-charge interaction
Key Lab of advanced optoelectronic quantum architecture and measurement (MOE), and School of Interdisciplinary Science, Beijing Institute of Technology（北京理工大学光电量子架构与测量教育部重点实验室，交叉科学研究院）
A quantized version of the magnetoelectric effect, known as the topological magnetoelectric effect, can exist in a time-reversal invariant topological insulator with all its surface states gapped out by magnetism. This topological phase, called the axion insulator phase, has been theoretically proposed but is still lack of conclusive experimental evidence due to the small signal of topological magnetoelectric effect. In this work, we propose that the dynamical in-plane magnetization in an axion insulator can generate a "pseudo-electric field", which acts on the surface state of topological ins…
Topological states of quantum matter have attracted great attention in condensed matter physics and materials science. The study of time-reversal-invariant (TRI) topological states in quantum materials has made tremendous progress in both theories and experiments. As a great success, thousands of TRI topological materials are predicted through sweeping search. Richer exotic phenomena are expected to appear in magnetic topological materials because of varied magnetic configurations, but this study falls much behind due to the complex magnetic structures and transitions. Here, we predict the tet…
It has been proposed that topological insulators can be best characterized not as surface conductors, but as bulk magnetoelectrics that -- under the right conditions-- have a universal quantized magnetoelectric response coefficient $e^2/2h$. However, it is not clear to what extent these conditions are achievable in real materials that can have disorder, finite chemical potential, residual dissipation, and even inversion symmetry. This has led to some confusion and misconceptions. The primary goal of this work is to illustrate exactly under what real life scenarios and in what context topologic…
One of the hallmarks of time-reversal-symmetric topological insulators in three dimensions is the topological magnetoelectric effect (TME). So far, a time-reversal breaking variant of this effect has attracted much attention, in the sense that the induced electric charge changes sign when the direction of an externally applied magnetic field is reversed. Theoretically, this effect is described by the so-called axion term. Here, we discuss a time-reversal-symmetric TME, where the electric charge depends only on the magnitude of the magnetic field but is independent of its sign. We obtain this n…
We study the kinetic magnetoelectric effect (current-induced magnetization including both the orbital and spin contributions) in three-dimensional conductors, specializing to the case of p-doped trigonal tellurium. We include both intrinsic and extrinsic contributions to the effect, which stem from the band structure of the crystal, and from disorder scattering, respectively. Specifically, we determine the dependence of the kinetic magnetoelectric response on the hole doping in tellurium, and show that the intrinsic and extrinsic effects dominate for low and high levels of doping, respectively…
Topological insulator (TI) thin films with surface magnetism are expected to exhibit a quantized anomalous Hall effect (QAHE) when the magnetizations on the top and bottom surfaces are parallel, and a quantized topological magnetoelectric (QTME) response when the magnetizations have opposing orientations (axion insulator phase) and the films are sufficiently thick. We present a unified picture of both effects that associates deviations from exact quantization of the QTME caused by finite thickness with non-locality in the side-wall current response function. Using realistic tight-binding model…
Observation of the universal magnetoelectric effect in a 3D topological insulator
拓扑绝缘体（TI）的电动力学由修改的麦克斯韦方程描述，其包含将电场耦合到介质的磁化和将磁场耦合到介质的极化的附加项，使得耦合系数被量化为每个表面$e^2 / 2 h c $的奇数倍。在这里，我们报告观察到的这种所谓的拓扑磁电（TME）效应。我们使用单色太赫兹（THz）光谱的TI结构配备了半透明的门选择性地解决表面状态。在强外磁场中，当一定频率的线偏振太赫兹辐射通过应变碲化汞三维薄膜的两个表面时，我们观察到一个与精细结构常数$α= e^2 / \hbar c$相等的普遍法拉第旋转角.这些实验提供了对TI的轴子电动力学的深入了解，并可能用于三个基本物理常数的精确定义。
Topological insulators (TIs) exhibit a quantized magnetoelectric response when time-reversal symmetry is broken on its surface. This unusual electromagnetic (EM) response is a unique macroscopic manifestation of the quantum Hall effect on the TI surface and it is described by a quantized Chern-Simons theory. In this paper, we construct the Green's function (GF) describing the EM response of two topological media separated by a cylindrical interface. This GF, in the appropriate limits, describes the magnetoelectric effect of both i) a cylindrical TI surrounded by a dielectric fluid, and ii) a T…
More than forty years ago, axion was postulated as an elementary particle with a low mass and weak interaction in particle physics to solve the strong $\mathcal{CP}$ (charge conjugation and parity) puzzle. Axions are also considered as a possible component of dark matter of the universe. However, the existence of axions in nature has not been confirmed. Interestingly, axions arise as pseudoscalar fields derived from the Chern-Simons theory in condensed matter physics. In antiferromagnetic insulators, the axion field can become dynamical induced by spin-wave excitations and exhibits rich exotic…
When time-reversal symmetry is broken on its surface, topological insulators exhibit a magnetoelectric response which is described by axion electrodynamics. A direct consequence of this theory is the appearance of a magnetic field that resembles the one produced by a magnetic image monopole when a point-like electric charge is located near the surface of the material. In this paper we investigate the more realistic problem when the point-like charge is replaced by a finite size sphere at constant potential. We calculate the electromagnetic fields using the potential formulation in a particular…
We investigate the interaction between a topological insulator nanoparticle and a quantum dot in an impulse magnetic field. Since topological insulators are nonmagnetic, after the impulse has ended only the localised topological surface modes, which are quantised in terms of dipolar bosonic modes, thus coupling dipolarly to the quantum dot. Hence, the hybrid system can be treated as a single bosonic mode interacting with a two-level system, where the coupling strength is quantised in terms of the magnetoelectric polarizability. We implement the interaction of the hybrid with the environment th…
Axion Insulator State in Hundred-Nanometer-Thick Magnetic Topological Insulator Sandwich Heterostructures
Department of Physics, The Pennsylvania State University（宾夕法尼亚州立大学物理系）；Department of Physics, Hong Kong University of Science and Technology（香港科技大学物理系）；Materials Research Institute, The Pennsylvania State University（宾夕法尼亚州立大学材料研究所）
The dynamical axion field is a new state of quantum matter where the magnetoelectric response couples strongly to its low-energy magnetic fluctuations. It is fundamentally different from an axion insulator with a static quantized magnetoelectric response. The dynamical axion field exhibits many exotic phenomena such as axionic polariton and axion instability. However, these effects have not been experimentally confirmed due to the lack of proper topological magnetic materials. Here by combining analytic models and first-principles calculations, we predict a series of van der Waal layered Mn$_2…
We study the generalization of the three-dimensional two-band Hopf insulator to the case of many bands, where all the bands are separated from each other by band gaps. The obtained $\mathbb{Z}$ classification of such a $N$-band Hopf insulator is related to the quantized isotropic magnetoelectric coefficient of its bulk. The boundary of a $N$-band Hopf insulator can be fully gapped, and we find that there is no unique way of dividing a finite system into bulk and boundary. Despite this non-uniqueness, we find that the magnetoelectric coefficient of the bulk and the anomalous Hall conductivity o…
Topological insulators have been predicted to exhibit a variety of interesting phenomena including a quantized magnetoelectric response and novel spintronics effects due to spin textures on their surfaces. However, experimental observation of these phenomena has proved difficult due to the finite bulk carrier density which may overwhelm the intrinsic topological responses that are expressed at the surface. Here, we demonstrate a novel ionic gel gating technique to tune the chemical potential of Bi$_{2}$Se$_{3}$ thin films while simultaneously performing THz spectroscopy. We can tune the carrie…
The 'magnetoelectric effect' arises from the coupling between magnetic and electric properties in materials. The Z2 invariant of topological insulators (TIs) leads to a quantized version of this phenomenon, known as the topological magnetoelectric (TME) effect. This effect can be realized in a new topological phase called an 'axion insulator' whose surface states are all gapped but the interior still obeys time reversal symmetry. We demonstrate such a phase using electrical transport measurements in a quantum anomalous Hall (QAH) sandwich heterostructure, in which two compositionally different…
The optical properties of a spherical topological insulator embedded concentrically in a single-electron system consisting of a core-shell GaAs quantum dot are analyzed, when the system is under a uniform external magnetic field. The topological insulator's magnetoelectric response is computed in the effective framework of $θ$-electrodynamics, which allows analytical calculations for the induced electric and magnetic potentials by Green's Function method. The GaAs Hamiltonian is constructed in the effective-mass approximation, and its corresponding Schrödinger equation is numerically solved th…
