Using the recently developed time-dependent Landauer-Büttiker formalism and Jefimenko's retarded solutions to the Maxwell equations, we show how to compute the time-dependent electromagnetic field produced by the charge and current densities in nanojunctions out of equilibrium. We then apply this formalism to a benzene ring junction, and show that geometry-dependent quantum interference effects can be used to control the magnetic field in the vicinity of the molecule. Then, treating the molecular junction as a quantum emitter, we demonstrate clear signatures of the local molecular geometry in the non-local radiated power.
The conductance of breaking metallic nanojunctions shows plateaus alternated with sudden jumps, corresponding to the stretching of stable atomic configurations and atomic rearrangements, respectively. We investigate the structure of the conductance plateaus both by measuring the voltage dependence of the plateaus' slope on individual junctions and by a detailed statistical analysis on a large amount of contacts. Though the atomic discreteness of the junction plays a fundamental role in the evolution of the conductance, we find that the fine structure of the conductance plateaus is determined b…
We consider nanojunctions in the single-electron tunnelling regime which, due to a high degree of spatial symmetry, have a degenerate many body spectrum. As a consequence, interference phenomena which cause a current blocking can occur at specific values of the bias and gate voltage. We present here a general formalism to give necessary and sufficient conditions for interference blockade also in the presence of spin polarized leads. As an example we analyze a triple quantum dot single electron transistor (SET). For a set-up with parallel polarized leads, we show how to selectively prepare the …
Progress of experimental techniques at nanoscale in the last decade made optical measurements in current-carrying nanojunctions a reality thus indicating emergence of a new field of research coined as optoelectronics. Optical spectroscopy of open nonequilibrium systems is a natural meeting point for (at least) two research areas: nonlinear optical spectroscopy and quantum transport, each with its own theoretical toolbox. We review recent progress in the field comparing theoretical treatments of optical response in nanojunctions as is accepted in nonlinear spectroscopy and quantum transport com…
We examine the effect of a hexagonal boron nitride (hBN) substrate on electron transport through graphene nanojunctions just before gap formation. Junctions in vacuum and on hBN are formed using classical molecular dynamics to create initial structures, followed by relaxation using density functional theory. We find that the hBN only slightly reduces the current through the junctions at low biases. Furthermore due to quantum interference at the last moments of breaking, the current though a single carbon filament spanning the gap is found to be higher than the current through two filaments spa…
In this paper we address several new developments in the theory of dc Josephson effect in superconducting weak links. We analyze an interplay between quantum interference effects and Andreev reflection in SNS nanojunctions with insulating barriers and demonstrate that such effects may qualitatively modify the Josephson current in such structures. We also investigate an impact of the parity effect on persistent currents in superconducting nanorings interrupted by a quantum point contact (QPC). In the limit of zero temperature and for the odd number of electrons in the ring we predict complete s…
Provided the electrical properties of electro-burnt graphene junctions can be understood and controlled, they have the potential to underpin the development of a wide range of future sub-10nm electrical devices. We examine both theoretically and experimentally the electrical conductance of electro-burnt graphene junctions at the last stages of nanogap formation. We account for the appearance of a counterintuitive increase in electrical conductance just before the gap forms. This is a manifestation of room-temperature quantum interference and arises from a combination of the semi-metallic band …
Negative differential conductance (NDC) is a non-linear transport phenomenon ubiquitous in molecular nanojunctions. Its physical origin can be the most diverse. In rotationally symmetric molecules with orbitally degenerate many-body states, it can be ascribed to interference effects. We establish in this paper a criterion to identify the interference blocking scenario by correlating the spectral and the topographical information achievable in an STM single molecule measurement. Simulations of current voltage characteristics and current maps for a Cu-Phthalocyanine (CuPc) on a thin insulating f…
We predict and analyze {\it radiation-induced quantum interference effect} in low-dimensional $n$-$p$ junctions. This phenomenon manifests itself by large oscillations of the photocurrent as a function of the gate voltage or the frequency of the radiation. The oscillations result from the quantum interference between two electron paths accompanied by resonant absorption of photons. They resemble Ramsey quantum beating and Stueckelberg oscillations well-known in atomic physics. The effect can be observed in one- and two-dimensional $n$-$p$ junctions based on nanowires, carbon nanotubes, monolay…
Control and manipulation of electric current and, especially, its degree of spin polarization (spin filtering) across single molecules are currently of great interest in the field of molecular spintronics. We explore one possible strategy based on the modification of nanojunction symmetry which can be realized, for example, by a mechanical strain. Such modification can activate new molecular orbitals which were inactive before due to their orbital mismatch with the electrode's conduction states. This can result in several important consequences such as (i) quantum interference effects appearin…
We report on the observation of the circular (helicity-dependent) and linear photogalvanic effects in Si-MOSFETs with inversion channels. The developed microscopic theory demonstrates that the circular photogalvanic effect in Si structures it is of pure orbital nature originating from the quantum interference of different pathways contributing to the light absorption.
Recently, asymmetric plasmonic nanojunctions [Karnetzky et. al., Nature Comm. 2471, 9 (2018)] have shown promise as on-chip electronic devices to convert femtosecond optical pulses to current bursts, with a bandwidth of multi-terahertz scale, although yet at low temperatures and pressures. Such nanoscale devices are of great interest for novel ultrafast electronics and opto-electronic applications. Here, we operate the device in air and at room temperature, revealing the mechanisms of photoemission from plasmonic nanojunctions, and the fundamental limitations on the speed of optical-to-electro…
Fano Resonances in Mismatched C$_3$N Nanoribbon Junctions
Technische Universität Dresden（德累斯顿工业大学）；Université Paris-Saclay, Centre de Nanosciences et de Nanotechnologies（巴黎萨克雷大学，纳米科学中心）；Universidad del País Vasco UPV/EHU（巴斯克地区大学）；IKERBASQUE, Basque Foundation for Science（伊克尔巴斯克，巴斯克科学基金会）；Donostia International Physics Center (DIPC)（圣塞巴斯蒂安国际物理中心）
Superconducting quantum interference devices (SQUIDs) that incorporate two superconductor/insulator/superconductor (SIS) Josephson junctions in a closed loop form the core of some of the most sensitive detectors of magnetic and electric fields currently available. SQUIDs in these applications are typically operated with a finite voltage which generates microwave radiation through the ac Josephson effect. This radiation may impact the system being measured. We describe here a SQUID in which the Josephson junctions are formed from strips of normal metal (N) in good electrical contact with the su…
Single photon, emitted in a transition between two states, has a frequency distribution of intensity, which is given by Lorentzian if the transition is only naturally broadened and the period of observation $T$ is long compared to the lifetime $T_{1}$ of the excited state. However, when the observation time $T$ is short or comparable to $T_{1}$, the frequency spectrum is appreciably broadened. If only the delayed part of the emitted radiation field is detected, then the radiation spectrum does not change. However, if the radiation field is transmitted through a resonant absorber and then detec…
The dephasing time of electrons in open semiconductor quantum dots, measured using ballistic weak localization, is found to saturate below ~ 100 mK, roughly twice the electron base temperature, independent of dot size. Microwave radiation deliberately coupled to the dots affects quantum interference indistinguishably from elevated temperature, suggesting that direct dephasing due to radiation is not the cause of the observed saturation. Coulomb blockade measurements show that the applied microwaves create sufficient source drain voltages to account for dephasing due to Joule heating.
We demonstrate real-time detection of self-interfering electrons in a double quantum dot embedded in an Aharonov-Bohm interferometer, with visibility approaching unity. We use a quantum point contact as a charge detector to perform time-resolved measurements of single-electron tunneling. With increased bias voltage, the quantum point contact exerts a back-action on the interferometer leading to decoherence. We attribute this to emission of radiation from the quantum point contact, which drives non-coherent electronic transitions in the quantum dots.
We present a detailed analysis of the dynamics of photon transport in waveguiding systems in the presence of a two-level system. In these systems, quantum interference effects generate a strong effective optical nonlinearity on the few-photon level. We clarify the relevant physical mechanisms through an appropriate quantum many-body approach. Based on this, we demonstrate that a single-particle photon-atom bound state with an energy outside the band can be excited via multi-particle scattering processes. We further show that these trapping effects are robust and, therefore, will be useful for …
Photocurrent generation is studied in a system composed of a quantum wire with side-coupled quantum rings. The current generation results from the interplay of the particular geometry of the system and the use of circularly polarized radiation. We study the energy-momentum conservation for optical transitions involving electrons moving forwards and backwards in the wire. Due to the lack of time-reversal symmetry in the radiation, the optical transitions depend on the direction of motion of the electrons, leading to a current at zero bias voltage. The photocurrent increases with the number of r…
Terahertz light helicity sensitive photoresponse in GaAs/AlGaAs high electron mobility transistors. The helicity dependent detection mechanism is interpreted as an interference of plasma oscillations in the channel of the field-effect-transistors (generalized Dyakonov-Shur model). The observed helicity dependent photoresponse is by several orders of magnitude higher than any earlier reported one. Also linear polarization sensitive photoresponse was registered by the same transistors. The results provide the basis for a new sensitive, all-electric, room-temperature and fast (better than 1 ns) c…
We demonstrate the existence of tunable bound-states in continuum (BIC) in a 1-dimensional quantum wire with two impurities induced by an intense monochromatic radiation field. We found that there is a new type of BIC due to the Fano interference between two optical transition channels, in addition to the ordinary BIC due to a geometrical interference between electron wave functions emitted by impurities. In both cases the BIC can be achieved by tuning the frequency of the radiation field.
We propose the implementation of a Josephson Radiation Comb Generator (JRCG) based on a dc superconducting quantum interference device (SQUID) driven by an external magnetic field. When the magnetic flux crosses a diffraction node of the critical current interference pattern, the superconducting phase undergoes a jump of $π$ and a voltage pulse is generated at the extremes of the SQUID. Under periodic drive this allows one to generate a sequence of sharp, evenly spaced voltage pulses. In the frequency domain, this corresponds to a comb-like structure similar to the one exploited in optics and …
We propose a method to evaluate the entropy density and entropy flux in a vacuum gap between two half-spaces that takes into account influence of near-field effects, i.e., interference, diffraction, and tunneling of waves. The method developed is used to determine the maximum work that can be extracted through near-field radiative transfer between two half-spaces at different temperatures.
We theoretically investigate up-conversion process of entangled two photons on a dimer molecule, which is coupled by a cavity or nanoscale metallic structure. Within one-dimensional input-output theory, the propagators of the photons are derived analytically and the up-conversion probability is calculated numerically. It is shown that the coupling with the nanostructure clearly enhances the process. We also find that the enhancement becomes further pronounced for some balanced system parameters such as the quantum correlation between photons, radiation decay rates and coupling between the nano…
