Photon loss in optical fibers prevents long-distance distribution of quantum information on the ground. Quantum repeater is proposed to overcome this problem, but the communication distance is still limited so far because of the system complexity of the quantum repeater scheme. Alternative solutions include transportable quantum memory and quantum-memory-equipped satellites, where long-lived optical quantum memories are the key components to realize global quantum communication. However, the longest storage time of the optical memories demonstrated so far is approximately 1 minute. Here, by employing a zero-first-order-Zeeman magnetic field and dynamical decoupling to protect the spin coherence in a solid, we demonstrate coherent storage of light in an atomic frequency comb memory over 1 hour, leading to a promising future for large-scale quantum communication based on long-lived solid-state quantum memories.
Light storage, the controlled and reversible mapping of photons onto long-lived states of matter [1], enables memory capability in optical quantum networks [2-6]. Prominent storage media are warm alkali gases due to their strong optical coupling and long-lived spin states [7,8]. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds [9,10]. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. Th…
We present spectral hole-burning measurements of the $^{4}I_{9/2}\rightarrow{}^4F_{3/2}$ transition in Nd$^{3+}$:YLiF$_4$. The isotope shifts of Nd$^{3+}$ can be directly resolved in the optical absorption spectrum. We report atomic frequency comb storage with an echo efficiency of up to 35% and a memory bandwidth of 60 MHz in this material. The interesting properties show the potential of this material for use in both quantum and classical information processing.
We study the efficiency of the Atomic Frequency Comb storage protocol. We show that for a given optical depth, the preparation procedure can be optimize to significantly improve the retrieval. Our prediction is well supported by the experimental implementation of the protocol in a \TMYAG crystal. We observe a net gain in efficiency from 10% to 17% by applying the optimized preparation procedure. In the perspective of high bandwidth storage, we investigate the protocol under different magnetic fields. We analyze the effect of the Zeeman and superhyperfine interaction.
We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory i…
We suggest an all-optical scheme for the storage, retrieval and processing of a single-photon wave packet through its off-resonant Raman interaction with a series of coherent control beams. These control beams, each with distinct carrier frequency, are distributed along the way of single-photon propagation, thus effectively forming a gradient absorption structure which can be controlled in various ways to achieve different single-photon processing functionalities. Such a controllable frequency comb is a hybrid of Raman, gradient echo memory (GEM) and atomic frequency comb (AFC) methods, theref…
153Eu3+:Y2SiO5 is a very attractive candidate for a long lived, multimode quantum memory due to the long spin coherence time (~15 ms), the relatively large hyperfine splitting (100 MHz) and the narrow optical homogeneous linewidth (~100 Hz). Here we show an atomic frequency comb memory with spin wave storage in a promising material 153Eu3+:Y2SiO5, reaching storage times slightly beyond 10 μs. We analyze the efficiency of the storage process and discuss ways of improving it. We also measure the inhomogeneous spin linewidth of 153Eu3+:Y2SiO5, which we find to be 69 \pm 3 kHz. These results repre…
Atomic Frequency Comb (AFC) protocol has been particularly successful recently to demonstrate the storage of quantum information in a solid medium (rare-earth doped crystals). The AFC is inspired by the photon-echo technique. We show in this paper that the AFC is actually closely related to the slow-light based storage protocols extensively used in atomic vapours. Experimental verifications are performed in thulium doped YAG (Tm3+:YAG). We clarify the interplay between absorption and dispersion and propose a classification of the existing protocols.
It has been shown that an inhomogeneously broadened optical transition shaped into an atomic frequency comb can store a large number of temporal modes of the electromagnetic field at the single photon level without the need to increase the optical depth of the storage material. The readout of light modes is made efficient thanks to the rephasing of the optical-wavelength coherence similarly to photon echo-type techniques and the re-emission time is given by the comb structure. For on-demand readout and long storage times, two control fields are used to transfer back and forth the optical coher…
Quantum memories with long storage times are key elements in long-distance quantum networks. The atomic frequency comb (AFC) memory in particular has shown great promise to fulfill this role, having demonstrated multimode capacity and spin-photon quantum correlations. However, the memory storage times have so-far been limited to about one millisecond, realized in a Eu${}^{3+}$ doped Y${}_2$SiO${}_5$ crystal at zero applied magnetic field. Motivated by studies showing increased spin coherence times under applied magnetic field, we developed a AFC spin-wave memory utilizing a weak 15 mT magnetic…
An optical-fibre-integrated buffer for packet-switched quantum networks
Linköpings Universitet（林雪平大学）；RISE-Research Institutes of Sweden（瑞研所）；Universidad de Concepción（康塞普西翁大学）；Millennium Institute for Research in Optics（光学研究千年研究所）
We present a light-storage experiment in a praseodymium-doped crystal where the light is mapped onto an inhomogeneously broadened optical transition shaped into an atomic frequency comb. After absorption of the light the optical excitation is converted into a spin-wave excitation by a control pulse. A second control pulse reads the memory (on-demand) by reconverting the spin-wave excitation to an optical one, where the comb structure causes a photon-echo type rephasing of the dipole moments and directional retrieval of the light. This combination of photon echo and spin-wave storage allows us …
We demonstrate efficient and reversible mapping of a light field onto a thulium-doped crystal using an atomic frequency comb (AFC). Thanks to an accurate spectral preparation of the sample, we reach an efficiency of 9%. Our interpretation of the data is based on an original spectral analysis of the AFC. By independently measuring the absorption spectrum, we show that the efficiency is both limited by the available optical thickness and the preparation procedure at large absorption depth for a given bandwidth. The experiment is repeated with less than one photon per pulse and single photon coun…
Photon-echo based optical quantum memory schemes often employ intermediate steps to transform optical coherences to spin coherences for longer storage times. We analyze a scheme that uses three identical chirped control pulses for coherence rephasing in an inhomogeneously broadened ensemble of three-level $Λ$-systems. The pulses induce a cyclic permutation of the atomic populations in the adiabatic regime. Optical coherences created by a signal pulse are stored as spin coherences at an intermediate time interval, and are rephased for echo emission when the ensemble is returned to the initial s…
Atomic population transfer in an inhomogeneously broadened optical medium is analyzed for on-demand photon storage-time control in both atomic frequency comb (AFC) and phase locked echoes. In AFC the photon storage mechanism belongs to the conventional three-pulse photon echoes, while the storage time control is limited by conventional two-pulse photon echoes.
We present two quantum memory protocols for solids: A stopped light approach based on spectral hole burning and the storage in an atomic frequency comb. These procedures are well adapted to the rare-earth ion doped crystals. We carefully clarify the critical steps of both. On one side, we show that the slowing-down due to hole-burning is sufficient to produce a complete mapping of field into the atomic system. On the other side, we explain the storage and retrieval mechanism of the Atomic Frequency Comb protocol. This two important stages are implemented experimentally in Tm$^{3+}$- doped yttr…
A cryogenic neutral-atom platform with full optical access and 2-hour trap lifetime
Max-Planck-Institut für Quantenoptik（马克斯·普朗克量子光学研究所）；Fakultät für Physik, Ludwig-Maximilians-Universität München（慕尼黑大学物理学院）；Munich Center for Quantum Science and Technology（慕尼黑量子科学与技术中心）
We analyze the performance of a quantum computer architecture combining a small processor and a storage unit. By focusing on integer factorization, we show a reduction by several orders of magnitude of the number of processing qubits compared with a standard architecture using a planar grid of qubits with nearest-neighbor connectivity. This is achieved by taking advantage of a temporally and spatially multiplexed memory to store the qubit states between processing steps. Concretely, for a characteristic physical gate error rate of $10^{-3}$, a processor cycle time of 1 microsecond, factoring a…
We propose to store non-classical states of light into the macroscopic collective nuclear spin ($10^{18}$ atoms) of a $^3$He vapor, using metastability exchange collisions. These collisions, commonly used to transfer orientation from the metastable state $2^{3}S\_1$ to the ground state state of $^3$He, can also transfer quantum correlations. This gives a possible experimental scheme to map a squeezed vacuum field state onto a nuclear spin state with very long storage times (hours).
We present an extension of the atomic frequency comb protocol that utilizes the Stark effect to perform noise-free, on-demand, control. An experimental realization of this protocol was implemented in the Pr$^{3+}$:Y$_2$SiO$_5$ solid-state system, and a recall efficiency of 38\% for a 0.8 $μ$s storage time was achieved. Experiments were performed with both bright pulses as well as weak-coherent states, the latter achieving a signal-to-noise ratio of $570 \pm 120$ using input pulses with an average photon number of $\sim 0.1$. The principal limitation for a longer storage time was found to be th…
We present a versatile electric trap for the exploration of a wide range of quantum phenomena in the interaction between polar molecules. The trap combines tunable fields, homogeneous over most of the trap volume, with steep gradient fields at the trap boundary. An initial sample of up to 10^8 CH3F molecules is trapped for as long as 60 seconds, with a 1/e storage time of 12 seconds. Adiabatic cooling down to 120 mK is achieved by slowly expanding the trap volume. The trap combines all ingredients for opto-electrical cooling, which, together with the extraordinarily long storage times, brings …
