Recently, it has been discovered that systems of Active Brownian particles (APB) at high density organise their velocities into coherent domains showing large spatial structures in the velocity field. Such a collective behavior occurs spontaneously, i.e. is not caused by any specific interparticle force favoring the alignment of the velocities. This phenomenon was investigated in the absence of thermal noise and in the overdamped regime where inertial forces could be neglected. In this work, we demonstrate through numerical simulations and theoretical analysis that the velocity alignment is a robust property of ABP and persists even in the presence of inertial forces and thermal fluctuations. We also show that a single dimensionless parameter, such as the Péclet number customarily employed in the description of self-propelled particles, is not sufficient to fully characterize such a phenomenon neither in the regimes of large viscosity nor small mass. Indeed, the size of the velocity domains, measured through the correlation length of the spatial velocity correlation, remains constant when the swim velocity increases while decreases as the rotational diffusion becomes larger. We find that the spatial velocity correlation depends on the inertia but, contrary to common belief, are non-symmetrically affected by mass and inverse viscosity variations. We conclude that in self-propelled systems, at variance with passive systems, variations of the inertial time (mass over solvent viscosity) and mass act as independent control parameters. Finally, we highlight the non-thermal nature of the spatial velocity correlations that are fairly insensitive both to solvent and active temperatures.
We investigate the transport of suspended Brownian particles dc driven along corrugated narrow channels in a regime of finite damping. We demonstrate that inertial corrections cannot be neglected as long as the width of the channel bottlenecks is smaller than an appropriate particle diffusion length, which depends on both, the temperature and the strength of the dc drive. Therefore, transport through sufficiently narrow constrictions turns out to be sensitive to the viscosity of the suspension fluid. Applications to colloidal systems are discussed.
The noise-assisted, directed transport in a one-dimensional dissipative, inertial Brownian motor of the rocking type that is exposed to an external bias is investigated. We demonstrate that the velocity-load characteristics is distinctly non-monotonic, possessing regimes with a {\em negative differential mobility}. In addition, we evaluate several possible efficiency quantifiers which are compared among each other. These quantifiers characterize the mutual interplay between the viscous drag and the external load differently, weighing the inherent rectification features from different physical …
Based on recent work [L. Machura, M. Kostur, P. Talkner, J. Luczka, and P. Hanggi, Phys. Rev. Lett. 98, 040601 (2007)], we extend the study of inertial Brownian motors to the case of an asymmetric potential. It is found that some transport phenomena appear in the presence of an asymmetric potential. Within tailored parameter regimes, there exists two optimal values of the load at which the mean velocity takes its maximum, which means that a load can facilitate the transport in the two parameter regimes. In addition, the phenomenon of multiple current reversals can be observed when the load is …
We have directly observed short-time stress propagation in viscoelastic fluids using two optically trapped particles and a fast interferometric particle-tracking technique. We have done this both by recording correlations in the thermal motion of the particles and by measuring the response of one particle to the actively oscillated second particle. Both methods detect the vortex-like flow patterns associated with stress propagation in fluids. This inertial vortex flow propagates diffusively for simple liquids, while for viscoelastic solutions the pattern spreads super-diffusively, dependent on…
We study the transport of inertial Brownian particles in steady laminar flows in the presence of two-dimensional Gaussian potentials. Through extensive numerical simulations, it is found that the transport is sensitively dependent on the external constant force and the Gaussian potential. Within tailored parameter regimes, the system exhibits a rich variety of transport behaviors. In the absence of any external driving forces, the spontaneous rectification of the particles can be manipulated by the spatial position of the Gaussian potential. Moreover, when the potential lies at the center of t…
Active Brownian motion commonly assumes spherical overdamped particles. However, self-propelled particles are often neither symmetric nor overdamped yet underlie random fluctuations from their surroundings. Active Brownian motion has already been generalized to include asymmetric particles. Separately, recent findings have shown the importance of inertial effects for particles of macroscopic size or in low-friction environments. We aim to consolidate the previous findings into the general description of a self-propelled asymmetric particle with inertia. We derive the Langevin equation of such …
Active particles which are self-propelled by converting energy into mechanical motion represent an expanding research realm in physics and chemistry. For micron-sized particles moving in a liquid ("microswimmers"), most of the basic features have been described by using the model of overdamped active Brownian motion. However, for macroscopic particles or microparticles moving in a gas, inertial effects become relevant such that the dynamics is underdamped. Therefore, recently, active particles with inertia have been described by extending the active Brownian motion model to active Langevin dyn…
Phase Separation in a system of Brownian inertial rotors
Università degli Studi di Bari（巴里大学）；INFN, Sezione di Bari（意大利国家核物理研究所巴里分部）；CY Cergy Paris Université（塞吉-蓬图瓦兹巴黎大学）；CNRS UMR 8089（法国国家科学研究中心8089联合研究实验室）；Universitat de Barcelona（巴塞罗那大学）
Broadband molecular dynamics simulation of fluid inertial effects in confined Brownian motion
Université de Mons（蒙斯大学）；Univ. Bordeaux, CNRS, LOMA, UMR 5798（波尔多大学，法国国家科学研究中心，LOMA联合实验室）；University of Vienna（维也纳大学）；Ecole Polytechnique, Institut Polytechnique de Paris（巴黎综合理工学院，巴黎理工学院）
We consider an active Brownian particle moving in a disordered two-dimensional energy or motility landscape. The averaged mean-square-displacement (MSD) of the particle is calculated analytically within a systematic short-time expansion. As a result, for overdamped particles, both an external random force field and disorder in the self-propulsion speed induce ballistic behaviour adding to the ballistic regime of an active particle with sharp self-propulsion speed. Spatial correlations in the force and motility landscape contribute only to the cubic and higher order powers in time for the MSD. …
Quantitative measurement of fluid inertial effects in confined Brownian motion
Univ. Bordeaux, CNRS, LOMA, UMR 5798（波尔多大学）；Dpto. Física Teórica de la Materia Condensada, Universidad Autónoma de Madrid（马德里自治大学凝聚态理论物理系）；Condensed Matter Physics Center, IFIMAC, Spain（IFIMAC凝聚态物理中心）；Mechanics Department, Ecole Polytechnique, Institut Polytechnique de Paris（巴黎理工学院高等学院力学系）
Rheological properties of dense flows of hard particles are singular as one approaches the jamming threshold where flow ceases, both for aerial granular flows dominated by inertia, and for over-damped suspensions. Concomitantly, the lengthscale characterizing velocity correlations appears to diverge at jamming. Here we introduce a theoretical framework that proposes a tentative, but potentially complete scaling description of stationary flows. Our analysis, which focuses on frictionless particles, applies {\it both} to suspensions and inertial flows of hard particles. We compare our prediction…
We present the operational principle for a refrigerator which uses inertial effects in active Brownian particles to locally reduce their (kinetic) temperature by two orders of magnitude below the environmental temperature. This principle exploits the peculiar but so-far unknown shape of the phase diagram of inertial active Brownian particles to initiate motility-induced phase separation in the targeted cooling regime only. Remarkably, active refrigerators operate without requiring isolating walls opening the route towards using them to systematically absorb and trap, e.g., toxic substances fro…
We have performed a case study investigating a recently proposed scheme to obtain an effective pair potential for active Brownian particles [Farage et al., Phys. Rev. E 91, 042310 (2015)]. Applying this scheme to the Lennard-Jones potential, numerical simulations of active Brownian particles are compared to simulations of passive Brownian particles interacting by the effective pair potential. Analyzing the static pair correlations, our results indicate a limited range of activity parameters (speed and orientational correlation time) for which we obtain quantitative, or even qualitative, agreem…
We investigate the mean first passage time of an active Brownian particle in one dimension using numerical simulations. The activity in one dimension is modeled as a two state model; the particle moves with a constant propulsion strength but its orientation switches from one state to other as in a random telegraphic process. We study the influence of a finite resetting rate $r$ on the mean first passage time to a fixed target of a single free Active Brownian Particle and map this result using an effective diffusion process. As in the case of a passive Brownian particle, we can find an optimal …
We present a microscopic theory for the nonequilibrium interfacial tension $γ_{\rm gl}$ of the free interface between gas and liquid phases of active Brownian particles. The underlying square gradient treatment and the splitting of the force balance in flow and structural contributions is general and applies to inhomogeneous nonequilibrium steady states. We find $γ_{\rm gl}\geq 0$, which opposes claims by Bialké et al. [Phys. Rev. Lett. $\bf{115}$, 098301 (2015)] and delivers the theoretical justification for the widely observed interfacial stability in active Brownian dynamics many-body simul…
We use a first-passage time approach to study the statistics of the trapping times induced by persistent motion of active particles colliding with flat boundaries. The angular first-passage time distribution and mean first-passage time is calculated exactly for active Brownian and run-and-tumble particles and the results are compared. Theoretical predictions are in excellent agreement with Langevin simulations. Our results shed further light onto how active particles with different dynamics may be equivalent in the bulk, yet behave differently near boundaries or obstacles.
We study the dynamics of an active Brownian particle with a nonlinear friction function located in a spatial cubic potential. For strong but finite damping, the escape rate of the particle over the spatial potential barrier shows a nonmonotonic dependence on the noise intensity. We relate this behavior to the fact that the active particle escapes from a limit cycle rather than from a fixed point and that a certain amount of noise can stabilize the sojourn of the particle on this limit cycle.
Active particles may happen to be confined in channels so narrow that they cannot overtake each other (Single File conditions). This interesting situation reveals nontrivial physical features as a consequence of the strong inter-particle correlations developed in collective rearrangements. We consider a minimal model for active Brownian particles with the aim of studying the modifications introduced by activity with respect to the classical (passive) Single File picture. Depending on whether their motion is dominated by translational or rotational diffusion, we find that active Brownian partic…
We study the dynamics of a single active Brownian particle (ABP) in two spatial dimensions. The ABP has an intrinsic time scale $D_R^{-1}$ set by the rotational diffusion constant $D_R$. We show that, at short-times $t \ll D_R^{-1}$, the presence of `activness' results in a strongly anisotropic and non-diffusive dynamics in the $(xy)$ plane. We compute exactly the marginal distributions of the $x$ and $y$ position coordinates along with the radial distribution, which are all shown to be non-Brownian. In addition, we show that, at early times, the ABP has anomalous first-passage properties, cha…
We derive the hydrodynamic equations of motion for a fluid of active particles described by under- damped Langevin equations that reduce to the Active-Brownian-Particle model, in the overdamped limit. The contraction into the hydrodynamic description is performed by locally averaging the par- ticle dynamics with the non-equilibrium many-particle probability density, whose formal expression is found in the physically relevant limit of high-friction through a multiple-time-scale analysis. This approach permits to identify the conditions under which self-propulsion can be subsumed into the fluid …
We investigate the full pair-distribution function of a homogeneous suspension of spherical active Brownian particles interacting by a Weeks-Chandler-Andersen potential in two spatial dimensions. The full pair-distribution function depends on three coordinates describing the relative positions and orientations of two particles, the Péclet number specifying the activity of the particles, and their mean packing density. This five-dimensional function is obtained from Brownian dynamics simulations. We discuss its structure taking into account all of its degrees of freedom. In addition, we present…
We perform a coarse-graining analysis of the paradigmatic active matter model, Active Brownian Particles, yielding a continuum description in terms of balance laws for mass, linear and angular momentum, and energy. The derivation of the balance of linear momentum reveals that the active force manifests itself directly as a continuum-level body force proportional to an order parameter-like director field, which therefore requires its own evolution equation to complete the continuum description of the system. We derive this equation, demonstrating in the process that bulk currents may be sustain…
We investigate a model for a Stirling-like engine consisting of a passive Brownian particle confined by a harmonic potential and interacting with a suspension of active Brownian particles that self-propel in a viscous solvent, which cyclically operates under isothermal conditions by means of temporal variations of the trap stiffness and the self-propulsion speed of the active particles. We derive an effective stochastic equation of motion of the trapped Brownian particle, which includes a friction memory kernel as well as thermal and active fluctuating forces due to its coupling with the activ…
We study analytically the single-trajectory spectral density (STSD) of an active Brownian motion as exhibited, for example, by the dynamics of a chemically-active Janus colloid. We evaluate the standardly-defined spectral density, i.e. the STSD averaged over a statistical ensemble of trajectories in the limit of an infinitely long observation time $T$, and also go beyond the standard analysis by considering the coefficient of variation $γ$ of the distribution of the STSD. Moreover, we analyse the finite-$T$ behaviour of the STSD and $γ$, determine the cross-correlations between spatial compone…
We derive an analytic expression for the mechanical pressure of a generic one-dimensional model of confined active Brownian particles (ABPs) that is valid for all values of Peclet number Pe and all confining scenarios. Our model reproduces the known scaling of bulk pressure with Pe^2 while in strong confinement pressure scales with Pe. Our analytic results are very well reproduced by simulations of ABPs in 2D. We use the pressure formula to calculate both the work performed by an active engine and its efficiency. In particular, efficiency is maximized for work cycles with finite period and not…
We study the pair correlation of Active Brownian Particles at low density using numerical simulations and analytical calculations. We observe a winged pair correlation: while particles accumulate in front of an active particle as expected, the depletion wake consists of two depletion wings. In the limit of soft particles, we obtain a closed equation for the pair correlation, allowing us to characterize the depletion wings. In particular, we unveil two regimes at high activity where the wings adopt a self-similar profile and decay algebraically. We also perform experiments of self-propelled Jan…
Directed transport of interacting active (self-propelled)Brownian particles is numerically investigated in confined geometries (entropic barriers). The self-propelled velocity can break thermodynamical equilibrium and induce the directed transport. It is found that the interaction between active particles can greatly affect the ratchet transport. For attractive particles, on increasing the interaction strength, the average velocity firstly decreases to its minima, then increases, and finally decreases to zero. For repulsive particles, when the interaction is very weak, there exists a critical …
By now active Brownian motion is a well-established model to describe the motion of mesoscopic self-propelled particles in a Newtonian fluid. On the basis of the generalized Langevin equation, we present an analytic framework for active Brownian motion with memory delay assuming time-dependent friction kernels for both translational and orientational degrees of freedom to account for the time-delayed response of a viscoelastic medium. Analytical results are obtained for the orientational correlation function, mean displacement and mean-square displacement which we evaluate in particular for a …
Micro- and nano-swimmers moving in a fluid solvent confined by structures that produce entropic barriers are often described by overdamped active Brownian particle dynamics, where viscous effects are large and inertia plays no role. However, inertial effects should be considered for confined swimmers moving in media where viscous effects are no longer dominant. Here, we study how inertia affects the rectification and diffusion of self-propelled particles in a two-dimensional asymmetric channel. We show that most of the particles accumulate at the channel walls as the masses of the particles in…
We derive from first principles the mechanical pressure $P$, defined as the force per unit area on a bounding wall, in a system of spherical, overdamped, active Brownian particles at density $ρ$. Our exact result relates $P$, in closed form, to bulk correlators and shows that (i) $P(ρ)$ is a state function, independent of the particle-wall interaction; (ii) interactions contribute two terms to $P$, one encoding the slow-down that drives motility-induced phase separation, and the other a direct contribution well known for passive systems; (iii) $P(ρ)$ is equal in coexisting phases. We discuss t…
The kinetic separation of repulsive active Brownian particles into a dense and a dilute phase is analyzed using a systematic coarse-graining strategy. We derive an effective Cahn-Hilliard equation on large length and time scales, which implies that the separation process can be mapped onto that of passive particles. A lower density threshold for clustering is found, and using our approach we demonstrate that clustering first proceeds via a hysteretic nucleation scenario and above a higher threshold changes into a spinodal-like instability. Our results are in agreement with particle-resolved co…
Suspensions of purely repulsive but self-propelled Brownian particles might undergo phase separation, a phenomenon that strongly resembles the phase separation of passive particles with attractions. Here we employ computer simulations to study the nucleation kinetics and the microscopic pathway active Brownian disks take in two dimensions when quenched from the homogeneous suspension to propulsion speeds beyond the binodal. We find the same qualitative behavior for the nucleation rate as a function of density as for a passive suspension undergoing liquid-vapor separation, suggesting that the s…
Particles kicked by external forces to produce mobility distinct from thermal diffusion are an iconic feature of the active matter problem. Here, we map this onto a minimal model for experiment and theory covering the wide time and length scales of usual active matter systems. A particle diffusing in a harmonic potential generated by an optical trap is kicked by programmed forces with time correlation at random intervals following the Poisson process. The model's generic simplicity allows us to find conditions for which displacements are Gaussian (or not), how diffusion is perturbed (or not) b…
We develop a formally exact technique for obtaining steady-state distributions of non-interacting active Brownian particles in a variety of systems. Our technique draws on results from the theory of two-way diffusion equations to solve the steady-state Smoluchowski equation for the 1-particle distribution function. The methods are employed to study in detail three scenarios: 1) confinement in a channel, 2) a constant flux steady state, and 3) sedimentation in a uniform external field. In each scenario, known behaviors are reproduced and precisely quantified, and new results are presented. In p…
The equilibrium properties of a system of passive diffusing particles in an external magnetic field are unaffected by the Lorentz force. In contrast, active Brownian particles exhibit steady-state phenomena that depend on both the strength and the polarity of the applied magnetic field. The intriguing effects of the Lorentz force, however, can only be observed when out-of-equilibrium density gradients are maintained in the system. To this end, we use the method of stochastic resetting on active Brownian particles in two dimensions by resetting them to the line $x=0$ at a constant rate and peri…
Phase separation in a chiral active fluid of inertial self-spinning disks
Dipartimento di Fisica, Università degli studi di Bari（巴里大学物理系）；INFN, Sezione di Bari（意大利国家核物理研究所巴里分部）；Universitat de Barcelona Institute of Complex Systems (UBICS)（巴塞罗那大学复杂系统研究所）；Departament de Física de la Matèria Condensada, Universitat de Barcelona（巴塞罗那大学凝聚态物理系）；Universidad de Extremadura（埃斯特雷马杜拉大学）
