Nanoparticles supporting a distinct series of Mie resonances have enabled a new class of nanoantennas and provide efficient ways to manipulate light at the nanoscale. The ability to flexibly tune the optical resonances and scattering directionality are particularly essential for various applications ranging from biosensing to nanolasers. In this paper, we investigate the core-shell nanoparticles that support both electric and magnetic Mie resonances and for the first time systematically reveal the mode evolution from a pure high-index dielectric nanosphere to a pure plasmonic one, where it has a sudden transition when core-shell ratio increases from 0.4 to 0.5. Furthermore, by engineering the electric and magnetic resonances, we demonstrate the unidirectional forward and backward scattering in such a system and reveal its tunability via geometric tuning.
Unidirectional backward and forward scattering of electromagnetic waves by nanoparticles are usually interpreted as the interference of conventional multipole moments (i.e., electric and magnetic dipole, electric quadrupole, etc.). The role of toroidal dipole moments in unidirectional scattering is generally overlooked. In this work, we investigate the unidirectional scattering for the system of three plasmonic nanospheres. It is found that the unidirectional backward scattering is caused by the interference between the toroidal dipole moment and other conventional multipole moments. Tunable p…
High-index dielectric nanoparticles have become a powerful platform for modern light science, enabling various fascinating applications, especially in nonlinear nanophotonics for which they enable special types of optical nonlinearity, such as electron-hole plasma photoexcitation, which are not inherent to plasmonic nanostructures. Here, we propose a novel geometry for highly tunable all-dielectric nanoantennas, consisting of a chain of silicon nanoparticles excited by an electric dipole source, which allows tuning their radiation properties via electron-hole plasma photoexcitation. We show th…
We study an one-dimensional non-Hermitian lattice with complex hopping rates, which can be realized by a quasi-one-dimensional sawtooth-type Hermitian lattice after adiabatic elimination with proper conditions. By means of synthetic magnetic fluxes, the imaginary parts of the complex hopping rates can be modulated by additional phase, thus a non-reciprocal structure arises. With this lattice, one can realize robust unidirectional transport for both single-site and Gaussian excitations, which is immune to defects and backscattering. Furthermore, we proposed a sandwich structure based on the non…
A method for diffracting the weak probe beam into unidirectional and higher-order directions is proposed via a novel Rydberg electromagnetically induced grating, providing a new way for the implementations of quantum devices with cold Rydberg atoms. The proposed scheme utilizes a suitable and position-dependent adjustment to the two-photon detuning besides the modulation of the standing-wave coupling field, bringing a in-phase modulation which can change the parity of the dispersion. We observe that when the modulation amplitude is appropriate, a perfect unidirectional diffraction grating can …
Engineering of intensity and direction of radiation from a single quantum emitter by means of structuring of their environment at the nanoscale is at the cornerstone of modern nanophotonics. Recently discovered systems exhibiting spin--orbit coupling of light are of particular interest in this context. In this Letter, we have demonstrated that asymmetrical excitation of a high-index subwavelength dielectric nanoparticle by a point dipole source located in a notch at its surface results in formation of a chiral near field, which is similar to that of a circularly polarized dipole or quadrupole.…
Optical forces allow manipulation of small particles and control of nanophotonic structures with light beams. Here, we describe a counter-intuitive lateral optical force acting on particles placed above a substrate, under uniform plane wave illumination without any field gradients. We show that under circularly-polarized illumination, nanoparticles experience a lateral force as a result of dipolar, spin-sensitive scattering, with a magnitude comparable to other optical forces. To this end, we rigorously calculate the force experienced by a circularly polarized dipole radiating above a surface.…
Optical tweezers, which are powerful tools for trapping and manipulating particles, have been widely used in many areas. However, their potential wells are typically symmetrical, which limit their capability of optical trapping and manipulation. Herein, we report an approach for dynamically creating asymmetrical potential wells, by employing variable phase gradient profiles generated by holograms. Its depth, stiffness and location of potential wells can be dynamically controlled. Moreover, the controllable transport of nanoparticle is experimentally demonstrated, which reveals that it exhibits…
We report unidirectional radiation of a magnetic dipole above planar metal surface, the radiation direction can be manipulated via changing the distance between the dipole and the surface. This phenomenon is unique for the combination of magnetic dipole and metal surface and does not happen for linear polarized dipole on metal surface or magnetic dipole on dielectric surface. The underlining physics is analytically disclosed by the interference of two orthogonally-oriented dipole component with π/2 phase lag. A substantially different mechanism of introducing the vectorial nature of the dipole…
Self-organized collective behaviour of active units is inspiring new designs of artificial swarms of micron-sized objects. However, active control at the nanoscale remains elusive. We have accurately solved the collective optofluidic dynamics of gold plasmonic 50 nm-radius nanoparticles moving in aqueous solution under a nonconservative optical vortex lattice. Above a critical field intensity and concentration, the interplay between optical forces, thermal fluctuations and hydrodynamic pairing leads to a spontaneous transition towards synchronised motion exhibiting a rich assortment of collect…
The controllable positioning of a vacuum-levitated object near a material surface is of importance for studying short-range forces, such as Casimir forces, interfacial friction forces, or gravity in yet unexplored parameter regimes. Here we optically levitate a nanoparticle in a laser beam strongly focused on a dielectric membrane. By investigating the motion of the trapped particle in vacuum, we map the position-dependent optical potential of the particle. We interferometrically measure the distance between the particle and the surface and demonstrate stable trapping in sub-wavelength proximi…
Optically generated electron-hole plasma in high-index dielectric nanostructures was demonstrated as a means of tuning of their optical properties. However, until now an ultrafast operation regime of such plasma driven nanostructures has not been attained. Here, we perform pump-probe experiments with resonant silicon nanoparticles and report on dense optical plasma generation near the magnetic dipole resonance with ultrafast (about 2.5 ps) relaxation rate. Basing on experimental results, we develop an analytical model describing transient response of a nanocrystalline silicon nanoparticle to a…
By using the real-space method, switching of a single plasmon interacting with a hybrid nanosystem composed of a semiconductor quantum dot (SQD) and a metallic nanoparticle (MNP) coupled to one-dimensional surface plasmonic waveguide is investigated theoretically. We discussed that the dipole coupling between an exciton and a localized surface plasmon results in the formation of a hybrid exciton and the transmission and reflection of the propagating single plasmon could be controlled by changing the interparticle distance between the SQD and the MNP and the size of the nanoparticles. The contr…
Surface-enhanced Raman spectroscopy (SERS) sensing of DNA sequences by plasmonic nanopores could pave a way to new generation single-molecule sequencing platforms. The SERS discrimination of single DNA bases depends critically on the time that a DNA strand resides within the plasmonic hot spot. However, DNA molecules flow through the nanopores so rapidly that the SERS signals collected are not sufficient for single-molecule analysis. In this work, we report an approach to control the time that molecules reside in the hot spot by physically adsorbing them onto a gold nanoparticle and then trapp…
Ultrashort laser pulses allows to deliver electromagnetic energy to matter causing its localized heating that can be used for both material removal via ablation/evaporation and drive interface chemical reactions. Here, we showed that both mentioned processes can be simultaneously combined within straightforward laser nanotexturing of Si wafer in functionalizing solution to produce a practically relevant metal-semiconductor surface nano-morphology. Such unique hybrid morphology represent deep-subwavelength Si LIPSSs with a extremely short period down to 70 nm with their high-aspect-ratio nanotr…
Brownian ratchet has emerged as a promising tool for understanding motion mechanism of molecules and proteins, and dynamically manipulating particles in non-equilibrium thermodynamics state. Here, we propose and experimentally demonstrate a new type of optical Brownian ratchets, which is generated by using controllable phase profiles in holographic optical trapping system. The potential energy profiles are dynamically switched in on-off mode, controlled by Labview software. Experimental results reveal that not only high speed but also large step distance can be easily achieved in Brownian ratc…
Controlling directional emission of nanophotonic radiation sources is fundamental to tailor radiation-matter interaction and to conceive highly efficient nanophotonic devices for on-chip wireless communication and information processing. Nanoantennas coupled to quantum emitters have proven to be very efficient radiation routers, while electrical control of unidirectional emission has been achieved through inelastic tunneling of electrons. Here we prove that the radiation emitted from the interaction of a high-energy electron beam with a graphene-nanoparticle composite has beaming directions wh…
We show and give examples of how unidirectional propagation of light rays in the limit of geometric optics could arise in some magnetic fluids due to the magnetoelectric effect under weak DC magnetic fields and strong DC electric fields around half of their dielectric breakdown. For such liquids as kerosene and transformer oils, one-way propagation of light may occur for 30 nm diameter magnetic nanoparticles (e.g. cobalt) and concentrations of 2% or larger.
Complex optical systems such as high-quality microcavities enabled by advanced lithography and processing techniques paved the way to various light-matter interactions (LMI) studies. Without lattice-matching constraints in epitaxy, coating techniques or shaky open cavity constructions, sub-micrometer-precise lithographic development of a polymer photoresist paves the way to polymer microcavity structures for various spectral regions based on the material's transparency and the geometrical sizes. We introduce a new approach based on 3D nanowriting in photoresist, which can be employed to achiev…
All-dielectric resonant nanophotonics lies at the heart of modern optics and nanotechnology due to the unique possibilities to control scattering of light from high-index dielectric nanoparticles and metasurfaces. One of the important concepts of dielectric Mie-resonant nanophotonics is associated with the Kerker effect that drives the unidirectional scattering of light from nanoantennas and Huygens' metasurfaces. Here we suggest and demonstrate experimentally a novel effect manifested in the nearly complete simultaneous suppression of both forward and backward scattered fields. This effect is…
The ever-growing field of microfluidics requires precise and flexible control over fluid flow at the micro- and nanoscales. Current constraints demand a variety of controllable components for performing different operations inside closed microchambers and microreactors. In this context, novel nanophotonic approaches can significantly enhance existing capabilities and provide new functionalities via finely tuned light-matter interaction mechanisms. Here we propose a novel design, featuring a dual functionality on-chip: boosted optically-driven particle diffusion and nanoparticle sorting. Our me…
