We propose a technique to control the macroscopic collective nuclear spin of a Helium-3 vapor in the quantum regime using light. The scheme relies on metastability exchange collisions to mediate interactions between optically accessible metastable states and the ground-state nuclear spin, giving rise to an effective nuclear spin-light quantum nondemolition interaction of the Faraday form. Our technique enables measurement-based quantum control of nuclear spins, such as the preparation of spin-squeezed states. This, combined with the day-long coherence time of nuclear spin states in Helium-3, opens the possibility for a number of applications in quantum technology.
We discuss the theory and experimental considerations of a quantum feedback scheme for producing deterministically reproducible spin squeezing. Continuous nondemolition atom number measurement from monitoring a probe field conditionally squeezes the sample. Simultaneous feedback of the measurement results controls the quantum state such that the squeezing becomes unconditional. We find that for very strong cavity coupling and a limited number of atoms, the theoretical squeezing approaches the Heisenberg limit. Strong squeezing will still be produced at weaker coupling and even in free space (t…
We use a reservoir engineering technique based on two-tone driving to generate and stabilize a quantum squeezed state of a micron-scale mechanical oscillator in a microwave optomechanical system. Using an independent backaction evading measurement to directly quantify the squeezing, we observe $4.7\pm0.9$ dB of squeezing below the zero-point level, surpassing the 3 dB limit of standard parametric squeezing techniques. Our measurements also reveal evidence for an additional mechanical parametric effect. The interplay between this effect and the optomechanical interaction enhances the amount of …
While the squeezing of a propagating field can, in principle, be made arbitrarily strong, the cavity-field squeezing is subject to the well-known 3 dB limit, and thus has limited applications. Here, we propose the use of a fully quantum degenerate parametric amplifier (DPA) to beat this squeezing limit. Specifically, we show that by {\it simply} applying a two-tone driving to the signal mode, the pump mode can, {\it counterintuitively}, be driven by the photon loss of the signal mode into a squeezed steady state with, in principle, an {\it arbitrarily high} degree of squeezing. Furthermore, we…
We show that the nanoresonator position can be squeezed significantly below the ground state level by measuring the nanoresonator with a quantum point contact or a single-electron transistor and applying a periodic voltage across the detector. The mechanism of squeezing is basically a generalization of quantum nondemolition measurement of an oscillator to the case of continuous measurement by a weakly coupled detector. The quantum feedback is necessary to prevent the ``heating'' due to measurement back-action. We also discuss a procedure of experimental verification of the squeezed state.
We analyze squeezing of the nanoresonator state produced by periodic measurement of position by a quantum point contact or a single-electron transistor. The mechanism of squeezing is the stroboscopic quantum nondemolition measurement generalized to the case of continuous measurement by a weakly coupled detector. The magnitude of squeezing is calculated for the harmonic and stroboscopic modulations of measurement, taking into account detector efficiency and nanoresonator quality factor. We also analyze the operation of the quantum feedback, which prevents fluctuations of the wavepacket center d…
In the scheme of a quantum nondemolition (QND) measurement, an observable is measured without perturbing its evolution. In the context of studies of decoherence in quantum computing, we examine the `open' quantum system of a two-level atom, or equivalently, a spin-1/2 system, in interaction with quantum reservoirs of either oscillators or spins, under the QND condition of the Hamiltonian of the system commuting with the system-reservoir interaction. The propagators for these QND Hamiltonians are shown to be connected to the squeezing and rotation operators for the two baths, respectively. Sque…
We use a quantum nondemolition measurement to probe the collective pseudospin of an atomic ensemble in a high-finesse optical cavity. We analyze the backaction antisqueezing produced by the measurement process to show that our protocol could create conditional spin squeezing in the atomic ensemble.
Spin squeezing of collective atomic spins can be achieved conditionally via probing with light and subsequent homodyne detection, as is done in a Quantum Nondemolition measurement. Recently it has been shown that squeezing can also be created unconditionally by a properly designed dissipative dynamics. We compare the two approaches in a Gaussian description, and optimize over all Gaussian light-matter interactions. We find that in the optimal unconditional scheme based on dissipation the level of squeezing scales as $d^{-1/2}$. In contrast, the optimal conditional scheme based on measurement o…
In the scheme of a quantum nondemolition (QND) measurement, an observable is measured without perturbing its evolution. In the context of studies of decoherence in quantum computing, we examine the `open' quantum system of a two-level atom, or equivalently, a spin-1/2 system, in interaction with quantum reservoirs of either oscillators or spins, under the QND condition of the Hamiltonian of the system commuting with the system-reservoir interaction. For completeness, we also examine the well-known non-QND spin-Bose problem. For all these many-body systems, we use the methods of functional inte…
We suggest an interferometric scheme assisted by squeezing and linear feedback to realize the whole class of field-quadrature quantum nondemolition measurements, from Von Neumann projective measurement to fully non-destructive non-informative one. In our setup, the signal under investigation is mixed with a squeezed probe in an interferometer and, at the output, one of the two modes is revealed through homodyne detection. The second beam is then amplitude-modulated according to the outcome of the measurement, and finally squeezed according to the transmittivity of the interferometer. Using str…
We study the enhancement of cooperativity in the atom-light interface near a nanophotonic waveguide for application to quantum nondemolition (QND) measurement of atomic spins. Here the cooperativity per atom is determined by the ratio between the measurement strength and the decoherence rate. Counterintuitively, we find that by placing the atoms at an azimuthal position where the guided probe mode has the lowest intensity, we increase the cooperativity. This arises because the QND measurement strength depends on the interference between the probe and scattered light guided into an orthogonal p…
We derive a measurement operator corresponding to a quantum nondemolition (QND) measurement of an atomic ensemble. The quantum measurement operator takes the form of a positive operator valued measure (POVM) and is valid for arbitrary interaction times, initial coherent state amplitudes, and final photon measurement outcomes. We analyze the dependence on various parameters and show that the effect of the QND measurement for short interaction times is to apply a Gaussian modulation of the initial state wavefunction. We derive approximate expressions for the POVM in various limits, such as the s…
We study the strong coupling between photons and atoms that can be achieved in an optical nanofiber geometry when the interaction is dispersive. While the Purcell enhancement factor for spontaneous emission into the guided mode does not reach the strong-coupling regime for individual atoms, one can obtain high cooperativity for ensembles of a few thousand atoms due to the tight confinement of the guided modes and constructive interference over the entire chain of trapped atoms. We calculate the dyadic Green's function, which determines the scattering of light by atoms in the presence of the fi…
A weak measurement approach is proposed to entangle and squeeze atoms. We show that even for very small coupling strength between light and atoms, one can achieve large squeezing unattainable with normal measurement-based squeezing. Post-selecting the photons interacting with spins via a weak off-resonant quantum nondemolition interaction (QND) in a state nearly orthogonal to its initial state can strengthen the entanglement among elementary spins and thus enhance spin squeezing. The squeezing process is probabilistic but the created state is unconditionally determined. Further control of the …
We present a realistic model for transferring the squeezing or the entanglement of optical field modes to the collective ground state nuclear spin of $^3$He using metastability exchange collisions. We discuss in detail the requirements for obtaining good quantum state transfer efficiency and study the possibility to readout the nuclear spin state optically.
We show that continuous quantum nondemolition (QND) measurement of an atomic ensemble is able to improve the precision of frequency estimation even in the presence of independent dephasing acting on each atom. We numerically simulate the dynamics of an ensemble with up to N = 150 atoms initially prepared in a (classical) spin coherent state, and we show that, thanks to the spin squeezing dynamically generated by the measurement, the information obtainable from the continuous photocurrent scales superclassically with respect to the number of atoms N. We provide evidence that such superclassical…
We propose a quantum feedback scheme for producing deterministically reproducible spin squeezing. The results of a continuous nondemolition atom number measurement are fed back to control the quantum state of the sample. For large samples and strong cavity coupling, the squeezing parameter minimum scales inversely with atom number, approaching the Heisenberg limit. Furthermore, ceasing the measurement and feedback when this minimum has been reached will leave the sample in the maximally squeezed spin state.
We examine how non-destructive measurements generate spin squeezing in an atomic Bose-Einstein condensate confined in a double-well trap. The condensate in each well is monitored using coherent light beams in a Mach-Zehnder configuration that interacts with the atoms through a quantum nondemolition Hamiltonian. We solve the dynamics of the light-atom system using an exact wavefunction approach, in the presence of dephasing noise, which allows us to examine arbitrary interaction times and a general initial state. We find that monitoring the condensate at zero detection current and with identica…
This dissertation studies spin squeezing, entanglement and decoherence in large ensembles of cold, trapped alkali atoms with hyperfine spin f interacting with optical fields. Restricting the state of each atom to a qutrit embedded in the 2f+1 dimensional hyperfine spin enables us to efficiently model the coherent and dissipative dynamics of the ensemble. This formalism also allows us to explore the effects of local control on the internal hyperfine spins of the atoms. State preparation using such control increases the entangling power of the atom-light interface for f>1/2. Subsequent control o…
We propose an approach for collective enhancement of precision for remotely located optical lattice clocks and a way of generation of the Einstein-Podolsky-Rosen state of remote clocks. Close to Heisenberg scaling of the clock precision with the number of clocks M can be achieved even for an optical channel connecting clocks with substantial losses. This scenario utilizes a collective quantum nondemolition measurement on clocks with parallel Bloch vectors for enhanced measurement precision. We provide an optimal network solution for distant clocks as well as for clocks positioned in close prox…
Squeezing of quantum fluctuations by means of entanglement is a well recognized goal in the field of quantum information science and precision measurements. In particular, squeezing the fluctuations via entanglement between two-level atoms can improve the precision of sensing, clocks, metrology, and spectroscopy. Here, we demonstrate 3.4 dB of metrologically relevant squeezing and entanglement for ~ 10^5 cold cesium atoms via a quantum nondemolition (QND) measurement on the atom clock levels. We show that there is an optimal degree of decoherence induced by the quantum measurement which maximi…
We use the vacuum Rabi splitting to perform quantum nondemolition (QND) measurements that prepare a conditionally spin-squeezed state of a collective atomic psuedo-spin. We infer a 3.4(6) dB improvement in quantum phase estimation relative to the standard quantum limit for a coherent spin state composed of uncorrelated atoms. The measured collective spin is composed of the two-level clock states of nearly 10^6 Rb-87 atoms confined inside a low finesse F = 710 optical cavity. This technique may improve atomic sensor precision and/or bandwidth, and may lead to more precise tests of fundamental p…
We discuss how large amounts of steady-state quantum squeezing (beyond 3 dB) of a mechanical resonator can be obtained by driving an optomechanical cavity with two control lasers with differing amplitudes. The scheme does not rely on any explicit measurement or feedback, nor does it simply involve a modulation of an optical spring constant. Instead, it uses a dissipative mechanism with the driven cavity acting as an engineered reservoir. It can equivalently be viewed as a coherent feedback process, obtained by minimally perturbing the quantum nondemolition measurement of a single mechanical qu…
We study the three-dimensional nature of the quantum interface between an ensemble of cold, trapped atomic spins and a paraxial laser beam, coupled through a dispersive interaction. To achieve strong entanglement between the collective atomic spin and the photons, one must match the spatial mode of the collective radiation of the ensemble with the mode of the laser beam while minimizing the effects of decoherence due to optical pumping. For ensembles coupling to a probe field that varies over the extent of the cloud, the set of atoms that indistinguishably radiates into a desired mode of the f…
The relationship between orientation-to-alignment conversion (a form of atomic polarization evolution induced by an electric field) and the phenomenon of spin squeezing is demonstrated. A "stretched" state of an atom or molecule with maximum angular-momentum projection along the quantization axis possesses orientation and is a quantum-mechanical minimum-uncertainty state, where the product of the equal uncertainties of the angular-momentum projections on two orthogonal directions transverse to the quantization axis is the minimum allowed by the uncertainty relation. Application of an electric …
We describe and characterize a simple, low cost, low phase noise microwave source that operates near 6.800 GHz for agile, coherent manipulation of ensembles of 87Rb. Low phase noise is achieved by directly multiplying a low phase noise 100 MHz crystal to 6.8 GHz using a non-linear transmission line and filtering the output with custom band-pass filters. The fixed frequency signal is single sideband modulated with a direct digital synthesis frequency source to provide the desired phase, amplitude, and frequency control. Before modulation, the source has a single sideband phase noise near -140 d…
We study a continuous-variable (CV) teleportation protocol based on a shared entangled state produced by the quantum-nondemolition (QND) interaction of two vacuum states. The scheme utilizes the QND interaction or an unbalanced beam splitter in the Bell measurement. It is shown that in the non-unity gain regime the signal transfer coefficient can be enhanced while the conditional variance product remains preserved by applying appropriate local squeezing operation on sender's part of the shared entangled state. In the unity gain regime it is demonstrated that the fidelity of teleportation can b…
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been generated by dispersive interaction with a quantized probe field, or by state dependent collisions in a quantum gas. Such experiments typically use complex multilevel atoms like Rb or Cs, with the relevant interactions designed so atoms behave like pseudo-spin-$1/2$ particles. We demonstrate the viability of spin squeezing for collective spins composed of the physic…
We experimentally demonstrate, with an all-optical setup, a nonlocal deterministic quantum non-demolition interaction gate applicable to quantum states at nodes separated by a physical distance and connected by classical communication channels. The gate implementation, based on entangled states shared in advance, local operations, and classical communication, runs completely in parallel fashion at both the local nodes, requiring minimum resource. The nondemolition character of the gate up to the local unitary squeezing is verified by the analysis using several coherent states. A genuine quantu…
Only a few years ago, it was realized that the zero-area Sagnac interferometer topology is able to perform quantum nondemolition measurements of position changes of a mechanical oscillator. Here, we experimentally show that such an interferometer can also be efficiently enhanced by squeezed light. We achieved a nonclassical sensitivity improvement of up to 8.2 dB, limited by optical loss inside our interferometer. Measurements performed directly on our squeezed-light laser output revealed squeezing of 12.7 dB. We show that the sensitivity of a squeezed-light enhanced Sagnac interferometer can …
Quantum enhanced sensing is a powerful technique in which nonclassical states are used to improve the sensitivity of a measurement. For enhanced mechanical displacement sensing, squeezed states of light have been shown to reduce the photon counting noise that limits the measurement noise floor. It has long been predicted, however, that suppressing the noise floor with squeezed light should produce an unavoidable increase in radiation pressure noise that drives the mechanical system. Such nonclassical radiation pressure forces have thus far been hidden by insufficient measurement strengths and …
We observe collective quantum spin states of an ensemble of atoms in a one-dimensional light-atom interface. Strings of hundreds of cesium atoms trapped in the evanescent fiel of a tapered nanofiber are prepared in a coherent spin state, a superposition of the two clock states. A weak quantum nondemolition measurement of one projection of the collective spin is performed using a detuned probe dispersively coupled to the collective atomic observable, followed by a strong destructive measurement of the same spin projection. For the coherent spin state we achieve the value of the quantum projecti…
We study the dynamics of the quantum phase distribution associated with the reduced density matrix of a system for a number of situations of practical importance, as the system evolves under the influence of its environment, interacting via a quantum nondemoliton type of coupling, such that there is decoherence without dissipation, as well as when it interacts via a dissipative interaction, resulting in decoherence as well as dissipation. The system is taken to be either a two-level atom (or equivalently, a spin-1/2 system) or a harmonic oscillator, and the environment is modeled as a bath of …
Micro- and nanoscale optical or microwave cavities are used in a wide range of classical applications and quantum science experiments, ranging from precision measurements, laser technologies to quantum control of mechanical motion. The dissipative photon loss via absorption, present to some extent in any optical cavity, is known to introduce thermo-optical effects and thereby impose fundamental limits on precision measurements. Here, we theoretically and experimentally reveal that such dissipative photon absorption can result in quantum feedback via in-loop field detection of the absorbed opti…
We propose to take advantage of the weak coupling of ground-state helium-3 nuclear spin to its environment to produce long-lived macroscopic quantum states, nuclear spin squeezed states, in a gas cell at room temperature. To perform a quantum non-demolition measurement of a transverse component of the polarized collective nuclear spin, we maintain a population in helium-3 metastable state with a discharge. The collective spin associated to $F=1/2$ metastable level hybridizes with the ground state one by metastability exchange collisions. To access nuclear spin fluctuations, one continuously me…
Iterative $C_Z$-gate-based protocol for squeezed Schrödinger cat state engineering
ITMO University（ITMO大学）；SMARTS-Quanttelecom LLC（SMARTS-Quanttelecom有限责任公司）；Saint-Petersburg State Institute of Technology（圣彼得堡国立技术学院）；Research and Education Center of Photonics and Optical IT, ITMO University（ITMO大学光子学与光学信息技术研究与教育中心）
Although the study of ultracold quantum gases trapped by light is a prominent direction of modern research, the quantum properties of light were widely neglected in this field. Quantum optics with quantum gases closes this gap and addresses phenomena, where the quantum statistical nature of both light and ultracold matter play equally important roles. First, light can serve as a quantum nondemolition (QND) probe of the quantum dynamics of various ultracold particles from ultracold atomic and molecular gases to nanoparticles and nanomechanical systems. Second, due to dynamic light-matter entang…
Superfluid has been realized in Helium-4, Helium-3 and ultra-cold atoms. It has been widely used in making high-precision devices and also in cooling various systems. There have been extensive experimental search for possible exciton superfluid (ESF) in semiconductor electron-hole bilayer (EHBL) systems below liquid Helium temperature. However, exciton superfluid are meta-stable and will eventually decay through emitting photons. Here we study quantum nature of photons emitted from the excitonic superfluid (ESF) phase in the semiconductor EHBL and find that the light emitted from the excitonic…
