Detection of graphene's divergent orbital diamagnetism at the Dirac point
J. Vallejo, N. J. Wu, C. Fermon, M. Pannetier-Lecoeur, T. Wakamura, K. Watanabe, T. Tanigushi, T. Pellegrin, A. Bernard, S. Daddinounou, V. Bouchiat, S. Guéron,… 展开作者
J. Vallejo, N. J. Wu, C. Fermon, M. Pannetier-Lecoeur, T. Wakamura, K. Watanabe, T. Tanigushi, T. Pellegrin, A. Bernard, S. Daddinounou, V. Bouchiat, S. Guéron, M. Ferrier, G. Montambaux, H. Bouchiat
The electronic properties of graphene have been intensively investigated over the last decade, and signatures of the remarkable features of its linear Dirac spectrum have been displayed using transport and spectroscopy experiments. In contrast, the orbital magnetism of graphene, which is one of the most fundamental signature of the characteristic Berry phase of graphene's electronic wave functions, has not yet been measured in a single flake. In particular, the striking prediction of a divergent diamagnetic response at zero doping calls for an experimental test. Using a highly sensitive Giant Magnetoresistance sensor (GMR) we have measured the gate voltage-dependent magnetization of a single graphene monolayer encapsulated between boron nitride crystals. The signal exhibits a diamagnetic peak at the Dirac point whose magnetic field and temperature dependences agree with theoretical predictions starting from the work of Mc Clure \cite{McClure1956}. Our measurements open a new field of investigation of orbital currents in graphene and 2D topological materials, offering a new means to monitor Berry phase singularities and explore correlated states generated by combined effects of Coulomb interactions, strain or moiré potentials.
The orbital magnetism is studied in graphene monolayer within the effective mass approximation. In models of short-range and long-range disorder, the magnetization is calculated with self-consistent Born approximation. In the zero-field limit, the susceptibility becomes highly diamagnetic around zero energy, while it has a long tail proportional to the inverse of the Fermi energy. We demonstrated how the magnetic oscillation vanishes and converges to the susceptibility, on going from a strong-field regime to zero-field. The behavior at zero energy is shown to be highly singular.
We present a theoretical study on the orbital magnetism in multilayer graphenes within the effective mass approximation. The Hamiltonian and thus susceptibility can be decomposed into contributions from sub-systems equivalent to monolayer or bilayer graphene. The monolayer-type subband exists only in odd layers and exhibits a delta-function susceptibility at $E_F=0$. The bilayer-type subband appearing in every layer number gives a singular structure in the vicinity of $E_F=0$ due to the trigonal warping as well as a logarithmic tail away from $E_F=0$. The integral of the susceptibility over en…
We study how the electron-hole pairing reveals itself in the response of a double layer graphene system to the vector and scalar potentials. Electron-hole pairing results in a rigid (London)relation between the current and the difference of vector potentials in two adjacent layers. The diamagnetic effect can be observed in multiple connected systems in the magnetic field parallel to the graphene layers. Such an effect would be considered as a hallmark of the electron-hole pairing, but the value of the effect is extremely small. Electron-hole pairing significantly changes the response to the sc…
The diamagnetism of confined Dirac fermions submitted to a uniform magnetic field in disordered graphene is investigated. The solutions of the energy spectrum are used to discuss the orbital magnetism from a statistical mechanical point of view. More precisely, by the technique of Green functions the self-energy for short and long-ranged disorders is obtained. This allows us to determine the susceptibility for short and long-ranged disorders together with confinement. We compare our results with already published work and point out the relevance of these findings to a systematic formulation of…
Orbital magnetism is studied for graphene flakes with various shapes and edge configurations using the tight-binding approximation. In the low-temperature regime where the thermal energy is much smaller than to the energy level spacing, the susceptibility rapidly changes between diamagnetism and paramagnetism as a function of Fermi energy, in accordance with the energy level structure. The susceptibility at charge neutral point is generally larger in armchair flake than in zigzag flake, and larger in hexagonal flake than in triangular flake. As the temperature increases, the discrete structure…
We study the orbital magnetism of graphene ribbon in the effective-mass approximation, to figure out the finite-size effect on the singular susceptibility known in the bulk limit. We find that the susceptibility at T = 0 oscillates between diamagnetism and paramagnetism as a function of Fermi energy, in accordance with the subband structure formed by quantum confinement. In increasing T, the oscillation rapidly disappears once the thermal broadening energy exceeds the subband spacing, and the susceptibility approaches the bulk limit i.e., a thermally broadened diamagnetic peak centered at zero…
We investigate the electronic instabilities in carbon nanotubes of short radius, looking for the breakdown of the Luttinger liquid regime from the singular behavior of the charge stiffnesses at low energies. We show that such a breakdown is realized in the undoped (3,3) nanotubes through the onset of phase separation into regions with opposite electronic current. The phenomenology derived from this regime is consistent with the formation of a pseudogap in the single-particle spectrum as well as with a divergent diamagnetic susceptibility, as observed in the experiments carried out in carbon na…
The orbital diamagnetic susceptibility is calculated in monolayer and bilayer graphenes with band gap as well as in three-dimensional Dirac systems. It is demonstrated that the pseudo-spin degree of freedom such as valleys produces paramagnetic susceptibility in an equal manner as the real spin dominating over the Landau diamagnetism. The pseudo-spin paramagnetism explains the origin of a singular diamagnetism which is present only in the band-gap region and disappears rapidly inside the conduction and valence bands.
Graphene [1] and its bilayer have generated tremendous excitement in the physics community due to their unique electronic properties [2]. The intrinsic physics of these materials, however, is partially masked by disorder, which can arise from various sources such as ripples [3] or charged impurities [4]. Recent improvements in quality have been achieved by suspending graphene flakes [5,6], yielding samples with very high mobilities and little charge inhomogeneity. Here we report the fabrication of suspended bilayer graphene devices with very little disorder. We observe fully developed quantize…
Recent experiments reveal a significant increase in the graphene Fermi velocity close to charge neutrality. This has widely been interpreted as a confirmation of the logarithmic divergence of the graphene Fermi velocity predicted by a perturbative approach. In this work, we reconsider this problem using functional bosonization techniques calculating the effects of electron interactions on the density of states non-perturbatively. We find that the renormalized velocity is {\it finite} and independent of the high energy cut-off, and we argue that the experimental observations are better understo…
We study the orbital susceptibility of coupled energy bands with a pair of Dirac points, as in graphene. We show that different systems having the same zero-field energy spectrum exhibit strong differences in their orbital magnetic response at zero energy, ranging from diamagnetism (graphene) to paramagnetism (dice lattice). A lattice model is introduced which interpolates continuously between these two limits. This striking behavior is related to a Berry phase varying continuously from pi to 0. These predictions could be tested with cold atoms in an optical lattice
We apply Laughlin's gauge argument to analyze the $ν=0$ quantum Hall effect observed in graphene when the Fermi energy lies near the Dirac point, and conclude that this necessarily leads to divergent bulk longitudinal resistivity in the zero temperature thermodynamic limit. We further predict that in a Corbino geometry measurement, where edge transport and other mesoscopic effects are unimportant, one should find the longitudinal conductivity vanishing in all graphene samples which have an underlying $ν=0$ quantized Hall effect. We argue that this $ν=0$ graphene quantum Hall state is qualitati…
We analyze the orbital magnetic susceptibility from the band structure of twisted bilayer graphene. Close to charge neutrality, the out-of-plane susceptibility inherits the strong diamagnetic response from graphene. Increasing the doping, a crossover from diamagnetism to paramagnetism is obtained and a logarithmic divergence develops at the van Hove singularity of the Moiré lattice in the first band. The enhanced paramagnetism at the van Hove singularity is stronger for relatively large angle but gets suppressed by the flat spectrum towards the vicinity of the first magic angle. A diverging pa…
We have investigated the behavior of the resistance of graphene at the $n=0$ Landau Level in an intense magnetic field $H$. Employing a low-dissipation technique (with power $P<$3 fW), we find that, at low temperature $T$, the resistance at the Dirac point $R_0(H)$ undergoes a 1000-fold increase from $\sim$10 k$Ω$ to 40 M$Ω$ within a narrow interval of field. The abruptness of the increase suggests that a transition to an insulating, ordered state occurs at the critical field $H_c$. Results from 5 samples show that $H_c$ depends systematically on the disorder, as measured by the offset gate vo…
There is only a handful of scanning techniques that can provide surface topography at nanometre resolution. At the same time, there are no methods that are capable of non-invasive imaging of the three-dimensional surface topography of a thin free-standing crystalline material. Here we propose a new technique - the divergent beam electron diffraction (DBED) and show that it can directly image the inhomogeneity in the atomic positions in a crystal. Such inhomogeneities are directly transformed into the intensity contrast in the first order diffraction spots of DBED patterns and the intensity con…
We discuss the orbital magnetism and the Hall effect in the weak magnetic field in two dimensional Dirac fermion systems with energy gap. This model is related to the graphene sheet, organic conductors, and $d$-density wave superconductors. We found the strong diamagnetism and finite Hall conductivity even in gapped systems. We also discuss the relation between the weak-magnetic field formalism and the Landau quantization with the Euler-Maclaurin expansion.
Divergent density of states offers the unique opportunity to explore a wide variety of correlated electron physics. In the thinnest limit, this has been predicted and verified in the ultra-flat bands of magic-angle twisted bilayer graphene, the band touching points of few-layer rhombohedral graphite, and the lightly doped rhombohedral trilayer graphene. The simpler and seemingly better understood Bernal bilayer graphene is also susceptible to orbital magnetism-driven phases at charge neutrality, such as layer antiferromagnet and quantum anomalous Hall octet. Here we report the discovery of a c…
We analyze, within a minimal model that allows analytical calculations, the electronic structure and Landau levels of graphene multi-layers with different stacking orders. We find, among other results, that electrostatic effects can induce a strongly divergent density of states in bi- and tri-layers, reminiscent of one-dimensional systems. The density of states at the surface of semi-infinite stacks, on the other hand, may vanish at low energies, or show a band of surface states, depending on the stacking order.
We consider the orbital magnetic properties of non-interacting charge carriers in graphene-based nanostructures in the low-energy regime. The magnetic response of such systems results both, frombulk contributions and from confinement effects that can be particularly strong in ballistic quantum dots. First we provide a comprehensive study of the magnetic susceptibility $χ$ of bulk graphene in a magnetic field for the different regimes arising from the relative magnitudes of the energy scales involved, i.e. temperature, Landau level spacing and chemical potential. We show that for finite tempera…
Gapless bilayer graphene (GBG), like monolayer graphene, is a material system with unique properties, such as anti-Klein tunneling and intrinsic Fano resonances. These properties rely on the gapless parabolic dispersion relation and the chiral nature of bilayer graphene electrons. In addition, propagating and evanescent electron states coexist inherently in this material, giving rise to these exotic properties. In this sense, bilayer graphene is unique, since in most material systems in which Fano resonance phenomena are manifested an external source that provides extended states is required. …
We analyze the collective mode spectrum of graphene nanoribbons within the random phase approximation. In the undoped case, only metallic armchair nanoribbons support a propagating plasmon mode. Landau damping of this mode is shown to be suppressed through the chirality of the single particle wavefunctions. We argue that undoped zigzag nanoribbons should not support plasmon excitations because of a broad continuum of particle-hole excitations associated with surface states, into which collective modes may decay. Doped nanoribbons have properties similar to those of semiconductor nanowires, inc…
Low-energy electronic states in monolayer and bilayer graphenes present chiral charge carriers with unique and unusual properties of interest for electronic applications. Here, we report the magnetotransport measurements in the ABC-stacked trilayer graphene as a function of charge carrier density, magnetic field, and temperature, which show clear evidence of l = 3 chiral quasiparticles with cubic dispersion, existing in a large, 20x60 sq. microns device. Shubnikov-deHaas oscillations (SdHO) reveal the Berry's phase 3π, and the marked increase of cyclotron mass near charge neutrality, consisten…
Building unconventional magnetic phases on graphene by H atom manipulation: From altermagnets to Lieb ferrimagnets
Universidad Autónoma de Madrid（马德里自治大学）；Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid（马德里自治大学凝聚态物理中心）；Instituto Nicolás Cabrera (INC), Universidad Autónoma de Madrid（马德里自治大学尼古拉斯·卡布雷拉研究所）
We investigate the development of a gapped phase in the field theory of Dirac fermions in graphene with long-range Coulomb interaction. In the large-N approximation, we show that the chiral symmetry is only broken below a critical number of two-component Dirac fermions $N_c = 32/π^2$, that is exactly half the value found in quantum electrodynamics in 2+1 dimensions. Adopting otherwise a ladder approximation, we give evidence of the existence of a critical coupling at which the anomalous dimension of the order parameter of the transition diverges. This result is consistent with the observation …
We compute the Coulomb correction $\mathcal{C}$ to the a. c. conductivity of interacting massless Dirac particles in graphene in the collisionless limit using the polarization tensor approach in a regularization independent framework. Arbitrary parameters stemming from differences between logarithmically divergent integrals are fixed on physical grounds exploiting only spatial $O(2)$ rotational invariance of the model which amounts to transversality of the polarization tensor. Consequently $\mathcal{C}$ is unequivocally determined to be $(19- 6π)/12$ within this effective model. We compare our…
We map out the possible ordered states in bilayer graphene at the neutrality point by extending the previous renormalization group treatment of many-body instabilities to finite temperature, trigonal warping and externally applied perpendicular electric field. We were able to analytically determine all outcomes of the RG flow equations for the 9 four-fermion coupling constants. While the full phase diagram exhibits a rich structure, we confirm that when forward scattering dominates, the only ordering tendency with divergent susceptibility at finite temperature is the nematic. At finite tempera…
We study two lattice models, the honeycomb lattice (HCL) and a special square lattice (SQL), both reducing to the Dirac equation in the continuum limit. In the presence of disorder (gaussian potential disorder and random vector potential), we investigate the behaviour of the density of states (DOS) numerically and analytically. While an upper bound can be derived for the DOS on the SQL at the Dirac point, which is also confirmed by numerical calculations, no such upper limit exists for the HCL in the presence of random vector potential. A careful investigation of the lowest eigenvalues indeed …
Transport through edge-channels is responsible for conduction in quantum Hall (QH) phases. Topology dictates quantization of both charge and thermal transport coefficients. These turn out to approach robust quantized values when incoherent equilibration processes become dominant. Here, we report on measurements of both electrical and thermal conductances of integer and fractional quantum Hall (FQH) phases, realized in hBN encapsulated graphite gated bilayer graphene devices. Remarkably, for the complex edge at filling factors $ν=5/3$ and $ν=8/3$, which correspond to the paradigmatic hole-conju…
By considering analytical expressions for the self-energies of intervalley and intravalley phonons in graphene, we describe the behavior of D, 2D, and D$'$ Raman bands with changes in doping ($μ$) and light excitation energy ($E_L$). Comparing the self-energy with the observed $μ$ dependence of the 2D bandwidth, we estimate the wavevector $q$ of the constituent intervalley phonon at $\hbar vq\simeq E_L/1.6$ ($v$ is electron's Fermi velocity) and conclude that the self-energy makes a major contribution (60%) to the dispersive behavior of the D and 2D bands. The estimation of $q$ is based on an …
