We investigate two-color photon correlations in the light emitted by strongly coupled two-level emitters. Spectral filtering allows us to manipulate the collected light statistics and we show that the resonances induced by dipole-dipole interactions give rise to specific correlations, where the time-symmetry of the correlations is broken. Based on the collective dressed states, our study encompasses both the case of real processes, where the photons are associated with specific resonances and classical correlations between each other, and virtual processes, where pairs of photons are emitted with non-classical correlations.
We study the photon blockade phenomenon in a nanocavity containing a single four-level quantum emitter. By numerically simulating the second-order autocorrelation function of the intra-cavity field with realistic parameters achievable in a state-of-the-art photonic-crystal nanocavity, we show that in the strongly coupled regime the resulting photon blockade is significantly better than that achievable with a two-level emitter. We introduce an intuitive picture of the photon blockade with a four-level emitter that explains the performance difference between the two-level and the four-level emit…
We use the scattering matrix formalism to analyze photon blockade in coherently-driven CQED systems with a weak drive. By approximating the weak coherent drive by an input single- and two-photon Fock state, we reduce the computational complexity of the transmission and the two-photon correlation function from exponential to polynomial in the number of emitters. This enables us to easily analyze cavity-based systems containing $\sim$50 quantum emitters with modest computational resources. Using this approach we study the coherence statistics of polaritonic photon blockade while increasing the n…
Entangled photons are crucial for quantum technologies, but generating arbitrary entangled photon states deterministically, efficiently, and with high fidelity remains a challenge. Here, we demonstrate how hybridization and dipole-dipole interactions -- potentially simultaneously available in colloidal quantum dots and molecular aggregates -- leveraged in conjunction can couple simple, well understood emitters into composite emitters with flexible control over the level structure. We show that cascade decay through carefully designed level structures can result in emission of frequency-entangl…
We study single-photon emission of a classically pumped three-level $Λ$-type emitter in a high-$Q$ cavity. In particular, generation of single-photon time-bin double-peak wave packets is shown.
We investigate the origin of imperfections in the fidelity of a two-photon controlled-phase gate based on two-level-emitter non-linearities. We focus on a passive system that operates without external modulations to enhance its performance. We demonstrate that the fidelity of the gate is limited by opposing requirements on the input pulse width for one- and two-photon scattering events. For one-photon scattering, the spectral pulse width must be narrow compared to the emitter linewidth, while two-photon scattering processes require the pulse width and emitter linewidth to be comparable. We fin…
We discuss the scattering of photons from a three-level emitter in a one-dimensional waveguide, where the transport is governed by the interference of spontaneously emitted and directly transmitted waves. The scattering problem is solved in closed form for different level structures. Several possible applications are discussed: The state of the emitter can be switched deterministically by Raman scattering, thus enabling applications in quantum computing such as a single photon transistor. An array of emitters gives rise to a photonic band gap structure, which can be tuned by a classical drivin…
The ability to entangle distant quantum nodes is essential for the construction of quantum networks and for quantum information processing. For solid-state quantum emitters used as qubits, it can be achieved by photon interference. When the emitter is subject to spectral diffusion, this process can become highly inefficient, impeding the achievement of scalable quantum technologies. We study two-photon interference in the context of a Hong-Ou-Mandel (HOM)-type experiment for two separate quantum emitters, with different detunings with respect to a specific target frequency. We evaluate the sec…
By coupling a $Λ$-type quantum emitter to a chiral waveguide, in which the polarization of a photon is locked to its propagation direction, we propose a controllable photon-emitter interface for quantum networks. We show that this chiral system enables the SWAP gate and a hybrid-entangling gate between the emitter and a flying single photon. It also allows deterministic storage and retrieval of single-photon states with high fidelities and efficiencies. In short, this chirally coupled emitter-photon interface can be a critical building block toward a large-scale quantum network.
We show that a three-level lambda quantum emitter with equal spontaneous emission rates on both optically active transitions can absorb an incident light field with a probability approaching unity, provided that the focused light profile matches that of the emitter dipole emission pattern. Even with realistic focusing geometries, our results could find applications in long-distance entanglement of spin qubits.
We discuss a new method for realizing number-resolving and non-demolition photo detectors by strong coupling of light to individual single photon emitters, which act as strong optical non-linearities. As a specific application we show how these elements can be integrated into an error-proof Bell state analyzer, whose efficiency exceeds the best possible performance with linear optics even for a modest atom-field coupling. The methods are error-proof in the sense that every detection event unambiguously projects the photon state onto a Fock or Bell state.
Rayleigh criterion has been continuously broken through with modern detecting instruments, many methods on resolving two emitters below the classical diffraction limit has been developed, one of these methods is detecting high order correlation functions of the emitters. We propose a method to resolve the single-photon emitters with only detecting the highest order correlation functions. We find that the variables that characterize the emitters are contained in the highest order correlation functions. Especially when there are more than two emitters, the spatial distribution of the emitters ca…
We present a fully passive method for implementing a quantum phase gate between two photons travelling in a one-dimensional wave guide. The gate is based on chirally coupled emitters in a three-level $V$ configuration, which only interact through the photon field without any external control fields. We describe the (non-)linear scattering of the emerging polariton states and show that for near resonant photons the scattering dynamics directly implements a perfect control phase gate between the incoming photons in the limit of many emitters. For a finite number of emitters we show that the domi…
Multi-photon entangled graph states are a fundamental resource in quantum communication networks, distributed quantum computing, and sensing. These states can in principle be created deterministically from quantum emitters such as optically active quantum dots or defects, atomic systems, or superconducting qubits. However, finding efficient schemes to produce such states has been a long-standing challenge. Here, we present an algorithm that, given a desired multi-photon graph state, determines the minimum number of quantum emitters and precise operation sequences that can produce it. The algor…
We demonstrate that intensity correlations of second order in the fluorescence light of N > 2 single- photon emitters may violate locality while the visibility of the signal remains below 71%. For this, we derive a homogeneous Bell-Wigner-type inequality, which can be applied to a broad class of experimental setups. We trace the violation of this inequality back to path entanglement created by the process of detection.
The radiation emitted by a classically pumped three-level $Λ$-type emitter in a resonator cavity featuring both radiative and unwanted losses is studied. In particular, the efficiency of one-photon Fock state excitation of the outgoing wave packet and the spatio-temporal shape of the wave packet are investigated. It is shown that for given shape of the emitter--cavity interaction, adjusting the shape of the pump pulse renders it possible to generate the emission of one-photon Fock state wave packets of desired shape with high efficiency.
We present protocols to generate arbitrary photonic graph states from quantum emitters that are in principle deterministic. We focus primarily on two-dimensional cluster states of arbitrary size due to their importance for measurement-based quantum computing. Our protocols for these and many other types of two-dimensional graph states require a linear array of emitters in which each emitter can be controllably pumped, rotated about certain axes, and entangled with its nearest neighbors. We show that an error on one emitter produces a localized region of errors in the resulting graph state, whe…
Quantum networks require flying qubits that transfer information between the nodes. This may be implemented by means of single atoms (the nodes) that emit and absorb single photons (the flying qubits) and requires full control of photon absorption and emission by the individual emitters. In this work, we theoretically characterize the wave packet of a photon emitted by a single atom undergoing a spontaneous Raman transition in a three-level scheme. We investigate several excitation schemes that are experimentally relevant and discuss control parameters that allow one to tailor the spectrum of …
We investigate the properties of a single photon generated by a solid-state emitter subject to strong pure dephasing. We employ a model in which all the elements of the system, including the propagating fields, are treated quantum mechanically. We analytically derive the density matrix of the emitted photon, which contains full information about the photon, such as its pulse profile, power spectrum, and purity. We visualize these analytical results using realistic parameters and reveal the conditions for maximizing the purity of generated photons.
We analytically treat the scattering of two counter-propagating photons on a two-level emitter embedded in an optical waveguide. We find that the non-linearity of the emitter can give rise to significant pulse-dependent directional correlations in the scattered photonic state, which could be quantified via a reduction in coincident clicks in a Hong-Ou-Mandel measurement setup, analogous to a linear beam splitter. Changes to the spectra and phase of the scattered photons, however, would lead to reduced interference with other photons when implemented in a larger optical circuit. We introduce su…
We propose a scheme for triggering a dissipation dominated highly efficient excitation transfer from a single photon wave packet to a single quantum emitter. This single photon induced optical pumping turns dominant dissipative processes, such as spontaneous photon emission by the emitter or cavity decay, into valuable tools for quantum information processing and quantum communication. It works for an arbitrarily shaped single photon wave packet with sufficiently small bandwidth provided a matching condition is satisfied which balances the dissipative rates involved. Our scheme does not requir…
We develop a general dynamical theory for studying a single photon transport in a one-dimensional (1D) waveguide coupled to multiple emitters which can be either identical or non-identical. In this theory, both the effects of the waveguide and non-waveguide vacuum modes are included. This theory enables us to investigate the propagation of an emitter excitation or an arbitrary single photon pulse along an array of emitters coupled to a 1D waveguide. The dipole-dipole interaction induced by the non-waveguide modes, which is usually neglected in the literatures, can significantly modify the dyna…
We study a system made up of one or two two-level quantum emitters, coupled to a single transverse mode of a closed waveguide, in which photon wavenumbers and frequencies are discretized, and characterize the stable states in which one excitation is steadily shared between the field and the emitters. We unearth finite-size effects in the field-emitter interactions and identify a family of dressed states, that represent the forerunners of bound states in the continuum in the limit of an infinite waveguide. We finally consider the potential interest of such states for applications in the field o…
High-purity fluorescence photon bundle emission from two separate emitters
College of Physical Science and Technology, Central China Normal University（华中师范大学物理科学与技术学院）；School of Science, Hubei University of Technology（湖北工业大学理学院）
Single-photon sources with high brightness and long coherence time are promising qubit candidates for quantum technology. To this end, interfacing emitters with high-finesse cavities is required, especially in the strong coupling regime, which so far has only been limited to cryogenic temperatures. Here, we experimentally demonstrate, at room temperature, strong coupling between a single photon emitter and a novel cavity based on optical bound states in the continuum. A remarkably large Rabi splitting of ~4 meV is achieved thanks to the combination of the narrow linewidth and large oscillator …
A detailed study of the photophysical properties of several novel color centers in chemical vapor deposition diamond is presented. These emitters show narrow luminescence lines in the near infra-red. Single photon emission was verified with continuous and pulsed excitation with emission rates at saturation in the MHz regime, whilst direct lifetime measurements reveal excited state lifetimes ranging from 1-14 ns. In addition, a number of quantum emitters demonstrate two level behavior with no bunching present in the second order correlation function. An improved method of evaluating the quantum…
We study nonclassical features of multiphoton light emitted by clusters of single-photon emitters. As signatures of nonclassicality, we use violation of inequalities for normalized correlation functions of different orders or the probabilities of multiphoton detection. In experiment, for clusters of 2 to 14 colloidal CdSe/CdS dot-in-rods we observe nonclassical behavior, which gets even more pronounced for larger clusters.
We show that two-photon transport can be modulated by a two-level emitter coupled to a cavity in a one-dimensional waveguide. In the ordinary case, the transmitted light has a wider frequency spectrum than the situation without the cavity because it is reflected and scattered many times. But when the two photons are resonant with the cavity resonance reflection frequency, the frequency spectrum of the transmitted light becomes narrower than that without the cavity. This means that properly tuning the cavity resonance frequency can improve the photon-photon interaction. In addition, we show tha…
A highly promising route to scale millions of qubits is to use quantum photonic integrated circuits (PICs), where deterministic photon sources, reconfigurable optical elements, and single-photon detectors are monolithically integrated on the same silicon chip. The isolation of single-photon emitters, such as the G centers and W centers, in the optical telecommunication O-band, has recently been realized in silicon. In all previous cases, however, single-photon emitters were created uncontrollably in random locations, preventing their scalability. Here, we report the controllable fabrication of…
In this work we experimentally demonstrate for the first time a recently proposed criterion adressed to detect nonclassical behavior in the fluorescence emission of ensembles of single-photon emitters. In particular, we apply the method to study clusters of NV centres in diamond observed via single-photon-sensitive confocal microscopy. Theoretical considerations on the behavior of the parameter at any arbitrary order in presence of poissonian noise are presented and, finally, the opportunity of detecting manifold coincidences is discussed.
Single photon sources (SPS) based on semiconductor quantum dot (QD) platforms are restricted to low temperature (T) operation due to the presence of strong dephasing processes. Despite the integration of QD in optical cavities provides an enhancement of its emission properties, the technical requirements for maintaining high indistinguishability (I) at high T are beyond the state of the art. Recently, new theoretical approaches have shown promising results by implementing two-dipole-coupled-emitter systems. Here, we have developed a theory to estimate I in a two-emitter system with strong deph…
We study the dynamics of a mechanical resonator parametrically coupled to a driven dissipative quantum emitter in the ultra-strong coupling regime. We show that this regime is fully compatible with a semi-classical treatment, and we derive master equations for the emitter and the resonator. We show that the fluctuations of the driven emitter's population induce the non-symmetrical scattering of the mechanical quadratures. At long timescales, such scattering back-acts on the emitter, which eventually decouples from the driving light. This optical noise at the quantum limit is observable with st…
Encoding high-dimensional quantum information into single photons can provide a variety of benefits for quantum technologies, such as improved noise resilience. However, the efficient generation of on-demand, high-dimensional entanglement was thought to be out of reach for current and near-future photonic quantum technologies. We present a protocol for the near-deterministic generation of $N$-photon, $d$-dimensional photonic Greenberger-Horne-Zeilinger (GHZ) states using an array of $d$ non-interacting single-photon emitters. We analyse the impact on performance of common sources of error for …
We investigate the single photon scattering by an emitter chirally coupled to a one-dimensional waveguide. The single-photon transport property is essentially different from the symmetrical coupling case. The single photons propagating towards the emitter in opposite directions show different transmission behaviors, which is a manifestation of the single-photon diode. In the ideal chiral coupling case, the transmission probability of the single photon transport in one direction is zero by critical coupling, while in the opposite direction it is unity. The diode works well only when the single-…
A single quantum emitter coupled to a one-dimensional photon field can perfectly trap a photon when placed close to a mirror. This occurs when the interference between the emitted and reflected light is completely destructive, leading to photon confinement between the emitter and the mirror. In higher dimensions, the spread of the light field in all directions hinders interference and, consequently, photon trapping by a single emitter is considered to be impossible. In this work, we show that is not the case by proving that a single emitter can indeed trap light in any dimension. We provide a …
Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the excitonic fine-structure splitting. This work demonstrates that, even if this splitting is absent, the degree of entanglement cannot reach unity when the excitation pulse in a two-photon resonance scheme has a finite duration. The degradation of the entanglement has its origin in a dynamically induced splitting of the exciton states caused by the laser puls…
Bell states are the most prominent maximally entangled photon states. In a typical four-level emitter, like a semiconductor quantum dot, the photon states exhibit only one type of Bell state entanglement. By adding an external driving to the emitter system, also other types of Bell state entanglement are reachable without changing the polarization basis. In this paper, we show under which conditions the different types of entanglement occur and give analytical equations to explain these findings. We further identify special points, where the concurrence, being a measure for the degree of entan…
We devise a mathematical framework for assessing the fidelity of multi-photon entangled states generated by a single solid-state quantum emitter, such as a quantum dot or a nitrogen-vacancy center. Within this formalism, we theoretically study the role of imperfections present in real systems on the generation of time-bin encoded Greenberger-Horne-Zeilinger and one-dimensional cluster states. We consider both fundamental limitations, such as the effect of phonon-induced dephasing, interaction with the nuclear spin bath, and second-order emissions, as well as technological imperfections, such a…
We analyze a novel method that uses fixed, minimal physical resources to achieve generation and nested purification of quantum entanglement for quantum communication over arbitrarily long distances, and discuss its implementation using realistic photon emitters and photonic channels. In this method, we use single photon emitters with two internal degrees of freedom formed by an electron spin and a nuclear spin to build intermediate nodes in a quantum channel. State-selective fluorescence is used for probabilistic entanglement generation between electron spins in adjacent nodes. We analyze in d…
