We analytically treat the scattering of two counter-propagating photons on a two-level emitter embedded in an optical waveguide. We find that the non-linearity of the emitter can give rise to significant pulse-dependent directional correlations in the scattered photonic state, which could be quantified via a reduction in coincident clicks in a Hong-Ou-Mandel measurement setup, analogous to a linear beam splitter. Changes to the spectra and phase of the scattered photons, however, would lead to reduced interference with other photons when implemented in a larger optical circuit. We introduce suitable fidelity measures which account for these changes, and find that high values can still be achieved even when accounting for all properties of the scattered photonic state.
We consider two non-interacting two-level emitters that are coupled weakly to a one-dimensional non-linear wave guide. Due to the Kerr-like non-linearity, the wave guide considered supports -- in addition to the scattering continuum -- a two-body bound state. As such, the wave guide models a bath with non-trivial mode structure. Solving the time-dependent Schrödinger equation, the radiation dynamics of the two emitters, initially prepared in their excited states, is presented. Changing the emitter frequency such that the two-emitter energy is in resonance with one of the two-body bound states,…
In recent years the controlled coupling of single photon emitters to propagating surface plasmons has been intensely studied, which is fueled by the prospect of a giant photonic non-linearity on a nano-scaled platform. In this article we will review the recent progress on coupling single emitters to nano-wires towards the construction of a new platform for strong light-matter interaction. The control over such a platform might open new doors for quantum information processing and quantum sensing at the nanoscale, and for the study of fundamental physics in the ultra-strong coupling regime.
We develop a wavefunction approach to describe the scattering of two photons on a quantum emitter embedded in a one-dimensional waveguide. Our method allows us to calculate the exact dynamics of the complete system at all times, as well as the transmission properties of the emitter. We show that the non-linearity of the emitter with respect to incoming photons depends strongly on the emitter excitation and the spectral shape of the incoming pulses, resulting in transmission of the photons which depends crucially on their separation and width. In addition, for counter-propagating pulses, we ana…
Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition emitters resonantly coupled to a single radiative plasmonic mode. However, plasmonic cavities also support non-radiative (or "dark") modes, which offer much higher coupling strengths. On the other hand, realistic quantum emitters often support multiple electronic transitions of various symmetry, which could overlap with higher order plasmonic transitions -- in the …
We study the characteristics of the light generated by few emitters in a cavity at strong light-matter coupling. By means of the Glauber $g^{(2)}$-function we can identify clearly distinguished parameter regimes with super-Poissonian and sub-Poissonian photon statistics. We establish a relation between the emission characteristics for one and multiple emitters, and explain its origin in terms of the photon-dressed emitter states. Cooperative effects lead to the generation of nonclassical light already at reduced light-matter coupling if the number of emitters is increased. Our results are obta…
We study the stationary solutions of the Gross-Pitaevskii equation that reduce, in the limit of vanishing non-linearity, to the eigenfunctions of the associated Schrödinger equation. By providing analytical and numerical support, we conjecture an existence condition for these solutions in terms of the ratio between their proper frequency (chemical potential) and the corresponding linear eigenvalue. We also give approximate expressions for the stationary solutions which become exact in the opposite limit of strong non-linearity. For one-dimensional systems these solutions have the form of a cha…
We address the problem of optically controlling and quantifying the dissipative dynamics of quantum and classical correlations in a set-up of individual quantum emitters under external laser excitation. We show that both types of correlations, the former measured by the quantum discord, are present in the system's evolution even though the emitters may exhibit an early stage disentanglement. In the absence of external laser pumping,we demonstrate analytically, for a set of suitable initial states, that there is an entropy bound for which quantum discord and entanglement of the emitters are alw…
Through a quantitative analysis of an atomic transition driven strongly by quantized electromagnetic fields of various quantum states, we explore the role of quantum fluctuations on the behavior of the system. The emphasis is on fields with super-Poissonian statistics manifested in photon bunching, with the case of squeezed vacuum radiation serving as a prototype of superbuching. When combined with non-linearly coupling of the resonant states, bunching and superbunching lead to counter-intuitive behavior. The connection to recent progress in squeezed vacuum sources and the opportunity for expe…
We study the effect of mode-coupling on a single-photon device in which a dipole-quantum-emitter (DQE) is embedded in a bimodal whispering-gallery-mode cavity (WGMC). A scatterer is used to induce mode coupling between counter-clockwise and clockwise propagating light fields, which interact with the DQE. In contrast to models for the interaction between a DQE and a (one-mode or two-mode) cavity field, we find that strong photon antibunching can occur even for a weak DQE-field coupling and large dephasing of the DQE, when mode coupling is introduced. We also find that mode coupling can make the…
In this paper, the dynamics of a system composed by an assembly of two-level atoms coupled to a single-mode cavity is theoretically studied considering the Tavis-Cummings Hamiltonian. Motivated by recent experimental results in non-linear phenomena on squeezed-like states, we have found that a threefold star state for the whole set of emitters can be dynamically generated from the analogue photonic state; beyond this, we numerically demonstrate, that this transfer of star-like states critically depends with the number of emitters. Quantum statistical properties of the system are obtained by co…
We explore photon coincidence counting statistics in the ultrastrong-coupling regime where the atom-cavity coupling rate becomes comparable to the cavity resonance frequency. In this regime usual normal order correlation functions fail to describe the output photon statistics. By expressing the electric-field operator in the cavity-emitter dressed basis we are able to propose correlation functions that are valid for arbitrary degrees of light-matter interaction. Our results show that the standard photon blockade scenario is significantly modified for ultrastrong coupling. We observe parametric…
Quantum emitters interacting with photonic band-gap materials lead to the appearance of qubit-photon bound states that mediate decoherence-free, tunable emitter-emitter interactions. Recently, it has been shown that when these band-gaps have a topological origin, like in the photonic SSH model, these qubit-photon bound states feature chiral shapes and certain robustness to disorder. In this work, we consider a more general situation where the emitters interact with an extended SSH photonic model with longer range hoppings that displays a richer phase diagram than its nearest-neighbour counterp…
Single photon emitters (SPEs) are often identified with a Hanbury Brown and Twiss intensity interferometer (HBTII) consisting of a 50:50 beamsplitter and two time-correlated single photon counters. For an SPE, the cross-correlation of photon arrival time between the two detectors, $g^{(2)}(τ)$, shows a hallmark dip to zero at $τ=0$. One common heuristic for identifying SPEs is by measuring a system to have $g^{(2)}(0)<1/2$. Here in, we use stochastic methods to simulate the case of a SPE observed with non-ideal detectors and optics. We show that identification of SPEs is thwarted when the dete…
We theoretically study a system composed by a waveguide and a moving quantum emitter in the single excitation subspace, treating the emitter motional degree of freedom quantum mechanically. We first characterize single-photon scattering off a single moving quantum emitter, showing both nonreciprocal transmission and recoil-induced reduction of the quantum emitter motional energy. We then characterize the bound states within the bandgap, which display a motion-induced asymmetric phase in real space. We also demonstrate how these bound states form a continuous band with exotic dispersion relatio…
The non-linearity of a conditional photon-counting measurement can be used to `de-Gaussify' a Gaussian state of light. Here we present and experimentally demonstrate a technique for photon number resolution using only homodyne detection. We then apply this technique to inform a conditional measurement; unambiguously reconstructing the statistics of the non-Gaussian one and two photon subtracted squeezed vacuum states. Although our photon number measurement relies on ensemble averages and cannot be used to prepare non-Gaussian states of light, its high efficiency, photon number resolving capabi…
Both non-Hermitian systems and the behaviour of emitters coupled to structured baths have been studied intensely in recent years. Here we study the interplay of these paradigmatic settings. In a series of examples, we show that a single quantum emitter coupled to a non-Hermitian bath displays a number of unconventional behaviours, many without Hermitian counterpart. We first consider a unidirectional hopping lattice whose complex dispersion forms a loop. We identify peculiar bound states inside the loop as a manifestation of the non-Hermitian skin effect. In the same setting, emitted photons m…
Photon-mediated interactions between quantum emitters in engineered photonic baths is an emerging area of quantum optics. At the same time, non-Hermitian (NH) physics is currently thriving, spurred by the exciting possibility to access new physics in systems ruled by non-trivial NH Hamiltonians - in particular photonic lattices - which can challenge longstanding tenets such as the Bloch theory of bands. Here, we combine these two fields and study the exotic interaction between emitters mediated by the photonic modes of a lossy photonic lattice described by a NH Hamiltonian. We show in a paradi…
This is an introduction to antilinear operators. In following E.P.Wigner the terminus "antilinear" is used as it is standard in Physics. Mathematicians prefer to say "conjugate linear". By restricting to finite-dimensional complex-linear spaces, the exposition becomes elementary in the functional analytic sense. Nevertheless it shows the amazing differences to the linear case. Basics of antilinearity is explained in sections 2, 3,4, 7 and in subsection 1.2: Spectrum, canonical Hermitian form, antilinear rank one and two operators, the Hermitian adjoint, classification of antilinear normal oper…
We establish a general framework for studying the bound states and the photon-emission dynamics of quantum emitters coupled to structured nanophotonic lattices with engineered dissipation (loss). In the single-excitation sector, the system can be described exactly by a non-Hermitian formalism. We have pointed out in the accompanying letter [Gong \emph{et al}., arXiv:2205.05479] that a single emitter coupled to a one-dimensional non-Hermitian lattice may already exhibit anomalous behaviors without Hermitian counterparts. Here we provide further detail on these observations. We also present seve…
The gravitational field of a laser pulse, although not detectable at the moment, comes with a peculiar feature which continues to attract attention; cause and effect propagate with the same speed, that of light. A particular result of this feature is that the gravitational field of an emitted laser pulse and the gravitational effect of the emitter's energy-momentum change are intimately entangled. In this article, a specific example of an emission process is considered - an atom, modeled as a point mass, emits two counter-propagating pulses. The corresponding curvature and the effect on massiv…
Quantum emitters respond to resonant illumination by radiating electromagnetic fields. A component of these fields is phase-coherent with the driving tone, while another one is incoherent, consisting of spontaneously emitted photons and forming the fluorescence signal. Atoms and molecules are routinely detected by their fluorescence at optical frequencies, with important applications in quantum technology and microscopy. Spins, on the other hand, are usually detected by {their coherent response} at radio- or microwave frequencies, either in continuous-wave or pulsed magnetic resonance. Indeed,…
We study the dynamics of a quantum emitter coupled to a two-dimensional photonic crystal featuring a finite bandwidth with sharp edges and a Van-Hove singularity. We study the effect of strong system-bath coupling and non-Markovianity of the photonic environment using a nonperturbative approach based on the recently introduced NCA dynamical map for open quantum systems. We show that several characteristic features of the dynamics near a photonic band-edge such as the freezing of spontaneous emission and the maximum light-matter entanglement, get strongly modified in presence of counter-rotatin…
Optical waveguides in the form of glass fibers are the backbone of global telecommunication networks. In such optical fibers, the light is guided over long distances by continuous total internal reflection which occurs at the interface between the fiber core with a higher refractive index and the lower index cladding. Although this mechanism ensures that no light escapes from the waveguide, it gives rise to an evanescent field in the cladding. While this field is protected from interacting with the environment in standard optical fibers, it is routinely employed in air- or vacuum-clad fibers i…
An outstanding goal in quantum optics is the realization of fast optical non-linearities at the single-photon level. Such non-linearities would allow for the realization of optical devices with new functionalities such as a single-photon switch/transistor or a controlled-phase gate, which could form the basis of future quantum optical technologies. While non-linear optics effects at the single-emitter level have been demonstrated in different systems, including atoms coupled to Fabry-Perot or toroidal micro-cavities, super-conducting qubits in strip-line resonators or quantum dots (QDs) in nan…
