Strong enhancement of level densities in the crossover from spherical to deformed neodymium isotopes
M. Guttormsen, Y. Alhassid, W. Ryssens, K. O. Ay, M. Ozgur, E. Algin, A. C. Larsen, F. L. Bello Garrote, L. Crespo Campo, T. Dahl-Jacobsen, A. Görgen, T. W. Hag… 展开作者
M. Guttormsen, Y. Alhassid, W. Ryssens, K. O. Ay, M. Ozgur, E. Algin, A. C. Larsen, F. L. Bello Garrote, L. Crespo Campo, T. Dahl-Jacobsen, A. Görgen, T. W. Hagen, V. W. Ingeberg, B. V. Kheswa, M. Klintefjord, J. E. Midtbø, V. Modamio, T. Renstrøm, E. Sahin, S. Siem, G. M. Tveten, F. Zeiser
Understanding the evolution of level densities in the crossover from spherical to well-deformed nuclei has been a long-standing problem in nuclear physics. We measure nuclear level densities for a chain of neodymium isotopes $^{142,144-151}$Nd which exhibit such a crossover. These results represent to date the most complete data set of nuclear level densities for an isotopic chain between neutron shell-closure and towards mid-shell. We observe a strong increase of the level densities along the chain with an overall increase by a factor of $\approx 170$ at an excitation energy of 7.5 MeV and saturation around mass 150. Level densities calculated by the shell model Monte Carlo (SMMC) are in excellent agreement with these experimental results. Based on our experimental and theoretical findings, we offer an explanation of the observed mass dependence of the level densities in terms of the intrinsic single-particle level density and the collective enhancement.
Currently, thirty-two zinc, thirty-two selenium, twenty-nine bromine and thirty-one neodymium isotopes have been observed and the discovery of these isotopes is discussed here. For each isotope a brief synopsis of the first refereed publication, including the production and identification method, is presented.
With a new detector setup and the high-resolution performance of the fragment separator FRS at GSI we discovered 57 new isotopes in the atomic number range of 60$\leq Z \leq 78$: \nuc{159-161}{Nb}, \nuc{160-163}{Pm}, \nuc{163-166}Sm, \nuc{167-168}{Eu}, \nuc{167-171}{Gd}, \nuc{169-171}{Tb}, \nuc{171-174}{Dy}, \nuc{173-176}{Ho}, \nuc{176-178}{Er}, \nuc{178-181}{Tm}, \nuc{183-185}{Yb}, \nuc{187-188}{Lu}, \nuc{191}{Hf}, \nuc{193-194}{Ta}, \nuc{196-197}{W}, \nuc{199-200}{Re}, \nuc{201-203}{Os}, \nuc{204-205}{Ir} and \nuc{206-209}{Pt}. The new isotopes have been unambiguously identified in reactions…
The experimental gamma-ray strength functions (gamma-SFs) of 142,144-151Nd have been studied for gamma-ray energies up to the neutron separation energy. The results represent a unique set of gamma-SFs for an isotopic chain with increasing nuclear deformation. The data reveal how the low-energy enhancement, the scissors mode and the pygmy dipole resonance evolve with nuclear deformation and mass number. The data indicate that the mechanisms behind the low-energy enhancement and the scissors mode are decoupled from each other.
In the frame of a systematic study of the activation cross sections of charged particle induced nuclear reactions on rare earths for production of therapeutic radionuclides, proton induced reactions on neodymium were measured up to 65 MeV energy, above 45 MeV for the first time. The excitation functions of the natNd(p,x)150,149,148m,148g,146,144,143,141Pm, 149,147,141,140,139m,138Nd, 142,138mPr and 139gCe nuclear reactions were assessed by using stacked foil activation technique and high resolution gamma-spectrometry. The excitation functions were compared to the theoretical predictions, avail…
In the frame of a systematic study of activation cross sections of deuteron induced nuclear reactions on rare earths, the reactions on neodymium for production of therapeutic radionuclides were measured for the first time. The excitation functions of the natNd(d,x) 151,150,149,148m,148g,146,144,143Pm, 149,147,139mNd, 142Pr and 139gCe nuclear reactions were assessed by using the stacked foil activation technique and high resolution $γ@-spectrometry. The experimental excitation functions were compared to the theoretical predictions calculated with the modified model codes ALICE-IPPE-D and EMPIRE…
High spin band structures of neutron-rich $^{152-158}$Pm isotopes have been obtained from the measurement of prompt $γ$-rays of isotopically identified fragments produced in fission of $^{238}$U+$^{9}$Be and detected using the VAMOS++ magnetic spectrometer and EXOGAM segmented Clover array at GANIL and also from the high statistics $γ$-$γ$-$γ$ and $γ$-$γ$-$γ$-$γ$ data from the spontaneous fission of $^{252}$Cf using Gammasphere. The excited states in $^{157}$Pm and those above the isomers in even-A Pm isotopes $^{152,154,156,158}$Pm have been identified for the first time. The spectroscopic in…
Recent experiments have reached the neutron-rich Cr isotope with N=40 and confirmed enhanced collectivity near this sub-shell. The current data focus on low-spin spectroscopy only, with little information on the states where high-j particles align their spins with the system rotation. By applying the Projected Shell Model, we show that rotation alignment occurs in neutron-rich even-even Cr nuclei as early as spin 8 and, due to shell filling, the aligning particles differ in different isotopes. It is suggested that observation of irregularities in moments of inertia is a direct probe of the def…
Ground state properties of carbon isotopes, including root-mean-square radii, neutron separation energies, single particle spectra, and shapes are systematically studied with the deformed relativistic Hartree-Bogoliubov theory in continuum. The calculations with the effective interaction PK1 reproduce the available data reasonably well. The shell evolution in this isotopic chain is investigated by examining the single particle spectra. The inversion of neutron orbitals $ν2s_{1/2}$ and $ν1d_{5/2}$ compared with the order of neutron orbitals in stable nuclei is revealed in $^{15-20,22}\mathrm{C}…
Proton inelastic scattering experiments at energy E_p = 200 MeV and a spectrometer scattering angle of 0 degree were performed on 144,146,148,150Nd and 152Sm exciting the IsoVector Giant Dipole Resonance (IVGDR). Comparison with results from photo-absorption experiments reveals a shift of resonance maxima towards higher energies for vibrational and transitional nuclei. The extracted photo-absorption cross sections in the most deformed nuclei, 150Nd and 152Sm, exhibit a pronounced asymmetry rather than a distinct double-hump structure expected as a signature of K-splitting. This behaviour can b…
It was recently shown that dielectronic recombination measurements can be used for accurately inferring changes in the nuclear mean-square charge radii of highly-charged lithium-like neodymium [Brandau et al., Phys. Rev. Lett. 100 073201 (2008)]. To make use of this method to derive information about the nuclear charge distribution for other elements and isotopes, accurate electronic isotope shift parameters are required. In this work, we calculate and discuss the relativistic mass- and field-shift factors for the two $2s ^{2}S_{1/2} - 2p ^{2}P^{o}_{1/2,3/2}$ transitions along the lithium isoe…
The ground-state bands (GSBs) in the even-even hafnium isotopes $^{170-184}$Hf are investigated by using the cranked shell model (CSM) with pairing correlations treated by the particle-number conserving (PNC) method. The experimental kinematic moments of inertia are reproduced very well by theoretical calculations. The second upbending of the GSB at high frequency $\hbarω\approx0.5$ MeV observed (predicted) in $^{172}$Hf ($^{170,174-178}$Hf) attributes to the sudden alignments of the proton high-$j$ orbitals $\pi1i_{13/2}$ $(1/2^{+}[660])$, $\pi1h_{9/2}$ $(1/2^{-}[541])$ and orbital $\pi1h_{11…
The phenomenon of fine structure of the Isoscalar Giant Quadrupole Resonance (ISGQR) has been studied with high energy-resolution proton inelastic scattering at iThemba LABS in the chain of stable even-mass Nd isotopes covering the transition from spherical to deformed ground states. A wavelet analysis of the background-subtracted spectra in the deformed 146,148,150Nd isotopes reveals characteristic scales in correspondence with scales obtained from a Skyrme RPA calculation using the SVmas10 parameterization. A semblance analysis shows that these scales arise from the energy shift between the …
This report is presented the level densities and gamma strength function which is extracted from primary gamma transitions of (n,2g) measurement on the Dalat Nuclear Research Reactor (DNRR). The comparisons with others results and model calculations, there are outside the scope of uncertainty. These research results are showed that having of complement research for deformed nucleus in order to evaluate nuclear structure models.
The evolution of quadrupole and octupole collectivity in neutron-deficient Xe, Ba, Ce, and Nd nuclei near the "octupole magic" neutron number $N=56$ is investigated within the mapped $sdf$-IBM framework. Microscopic input is obtained via quadrupole and octupole constrained Hartree-Fock-Bogoliubov calculations, based on the parametrization D1M of the Gogny energy density functional. Octupole-deformed mean-field ground states are predicted for Ba and Ce isotopes near $N=56$. Excitation energies of positive- and negative-parity states as well as electric transition rates are computed with wave fu…
We expand the triaxial projected shell model basis to include triaxially-deformed multi-quasiparticle states. This allows us to study the yrast and gamma-vibrational bands up to high spins for both gamma-soft and well-deformed nuclei. As the first application, a systematic study of the high-spin states in Er-isotopes is performed. The calculated yrast and gamma-bands are compared with the known experimental data, and it is shown that the agreement between theory and experiment is quite satisfactory. The calculation leads to predictions for bands based on one- and two-gamma phonon where current…
The aim of this work is to develop the deformed relativistic Hartree-Bogoliubov theory in continuum (DRHBc) theory based on the point-coupling density functionals and extend it to provide a unified description for all even-even nuclei in the nuclear chart by overcoming all possible challenges. The nuclear superfluidity is considered via Bogoliubov transformation. Densities and potentials are expanded in terms of Legendre polynomials to include the axial deformation degrees of freedom. Sophisticated relativistic Hartree-Bogoliubov equations in coordinate space are solved in the DiracWoods-Saxon…
The heaviest N=Z doubly-magic nucleus, $^{100}$Sn, and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction in extreme conditions. In particular, the Cd isotopes are expected to present features similar to those found in the Sn isotopic chain, since they have only two proton holes in the Z=50 shell. In this manuscript, the lifetime measurements of low-lying states in the even-mass $^{102-108}$Cd is presented. Thanks to the powerful detection capabilities of AGATA array and VAMOS++ spectrometer, the unusual employment of multi-nucleon transfer r…
The shell structure underlying shape changes in neutron-rich nuclei near N=28 has been investigated by a novel application of the transient field technique to measure the first-excited state g factors in 38S and 40S produced as fast radioactive beams. There is a fine balance between proton and neutron contributions to the magnetic moments in both nuclei. The g factor of deformed 40S does not resemble that of a conventional collective nucleus because spin contributions are more important than usual.
Inspired by the newly discovered isomeric states in the rare-earth neutron-rich nuclei, high-$K$ isomeric states in neutron-rich samarium and gadolinium isotopes are investigated within the framework of the cranked shell model (CSM) with pairing correlation treated by a particle-number-conserving (PNC) method. The experimental multi-particle state energies and moments of inertia are reproduced quite well by the PNC-CSM calculations. A remarkable effect from the high-order deformation $\varepsilon_{6}$ is demonstrated. Based on the occupation probabilities, the configurations are assigned to th…
We extend the ab initio coupled-cluster effective interaction (CCEI) method to deformed open-shell nuclei with protons and neutrons in the valence space, and compute binding energies and excited states of isotopes of neon and magnesium. We employ a nucleon-nucleon and three-nucleon interaction from chiral effective field theory evolved to a lower cutoff via a similarity renormalization group transformation. We find good agreement with experiment for binding energies and spectra, while charge radii of neon isotopes are underestimated. For the deformed nuclei $^{20}$Ne and $^{24}$Mg we reproduce…
Taking the Coulomb and proximity potential model for deformed nuclei (CPPMDN) as the interacting potential for the post-scission region, the alpha decay properties of 34 isotopes of the superheavy nuclei with Z = 128 within the range 306 $\leq$ A $\leq$ 339 have been studied, considering both the parent and daughter nuclei to be deformed. The manuscript also deals with the decay properties of the isotopes of Z = 126 (within 288 $\leq$ A $\leq$ 339), Z = 124 (within 284 $\leq$A $\leq$ 339) and Z = 122 (within 280 $\leq$ A $\leq$ 339). The alpha decay half lives thus evaluated has been compared …
The available data for E2 transition strengths in the region between neutron-deficient Hf and Pt isotopes are far from complete. More and precise data are needed to enhance the picture of structure evolution in this region and to test state-of-the-art nuclear models. In a simple model, the maximum collectivity is expected at the middle of the major shell. However, for actual nuclei, this picture may no longer be the case, and one should use a more realistic nuclear-structure model. We address this point by studying the spectroscopy of Hf. We remeasure the 2^+_1 half-lives of 172,174,176Hf, for…
Shape evolution of krypton isotopes calculated with axially deformed relativistic Hartree-Bogoliubov approach
Advanced Energy Science and Technology, Guangdong Laboratory（广东实验室先进能源科学与技术）；CAS Key Laboratory of High Precision Nuclear Spectroscopy, Institute of Modern Physics , Chinese Academy of Sciences（中国科学院近代物理研究所高精度核谱学重点实验室）；Zhejiang Key Laboratory of Quantum State Control and Optical Field Manipulation, Department of Physics, Zhejiang Sci-Tech University（浙江理工大学物理学院量子态调控与光场操控浙江省重点实验室）；Astrophysical Big Bang Laboratory, Pioneering Research Institute, RIKEN（理化学所先驱研究院天体物理大爆炸实验室）；Physik-Department der Technische Universität München（慕尼黑工业大学物理系）；State Key Laboratory of Nuclear Physics and Technology, School of Physics, Peking University（北京大学物理学院核物理与核技术国家重点实验室）
The shapes of neutron-rich exotic Ni isotopes are studied. Large-scale shell model calculations are performed by advanced Monte Carlo Shell Model (MCSM) for the $pf$-$g_{9/2}$-$d_{5/2}$ model space. Experimental energy levels are reproduced well by a single fixed Hamiltonian. Intrinsic shapes are analyzed for MCSM eigenstates. Intriguing interplays among spherical, oblate, prolate and gamma-unstable shapes are seen including shape fluctuations, $E$(5)-like situation, the magicity of doubly-magic $^{56,68,78}$Ni, and the coexistence of spherical and strongly deformed shapes. Regarding the last …
We have calculated the binding energy, root-mean-square radius and quadrupole deformation parameter for the recently synthesized superheavy element Z=117, using the axially deformed relativistic mean field (RMF) model. The calculation is extended to various isotopes of Z=117 element, strarting from A=286 till A=310. We predict almost spherical structures in the ground state for almost all the isotopes. A shape transition appears at about A=292 from prolate to a oblate shape structures of Z=117 nucleus in our mean field approach. The most stable isotope (largest binding energy per nucleon) is f…
The mass region with A~100 and Z~40 is known to experience a sudden onset of deformation. The presence of the subshell closure $Z=40$ makes feasible to create particle-hole excitations at a moderate excitation energy and, therefore, likely intruder states could be present in the low-lying spectrum. In other words, shape coexistence is expected to be a key ingredient to understand this mass region. The aim of this work is to describe excitation energies, transition rates, radii, and two-neutron separation energies for the even-even 94-110Zr nuclei and, moreover, to obtain information about wave…
Whereas previous works for B(E2)'s in the even-even Ti isotopes focused on yrast transitions we here also consider inter-band transitions to a second group i.e. states like 1_{1} , 2_{2}, 3_{1} , 4_{2} , 5_{1}e.t.c.. We focus on variations from one even-even Ti isotope to the next. We make a qualitative comparison with similar transitions in a heavier deformed nucleus.
The effective field theory for collective rotations of triaxially deformed nuclei is generalized to odd-mass nuclei by including the angular momentum of the valence nucleon as an additional degree of freedom. The Hamiltonian is constructed up to next-to-leading order within the effective field theory formalism. The applicability of this Hamiltonian is examined by describing the wobbling bands observed in the lutetium isotopes $^{161,163,165,167}$Lu. It is found that by taking into account the next-to-leading order corrections, quartic in the rotor angular momentum, the wobbling energies $E_{\t…
Octupole deformation and the relevant spectroscopic properties of neutron-rich odd-mass barium isotopes are investigated in a theoretical framework based on nuclear density functional theory and the particle-core coupling scheme. The interacting-boson Hamiltonian that describes the octupole-deformed even-even core nucleus, as well as the single-particle energies and occupation probabilities of an unpaired nucleon, are completely determined by microscopic axially-symmetric $(β_{2},β_{3})$-deformation constrained self-consistent mean-field calculations for a specific choice of the energy density…
In rapid-proton capture (rp-process), N=Z nuclei above Ni are understood to act as waiting-point nuclei. The N=Z nuclei 68Se, 72Kr, 76Sr and 80Zr among others are known to give rise to a large-energy x-ray flux and peaks in abundances of these nuclei synthesized in the astrophysical rp-process. Investigating the experimental isotope shifts in Kr isotopes near the proton drip-line within the framework of the deformed Relativistic Hartree-Bogoliubov theory, we have discovered that N=Z rp-process nuclei 68Se, 72Kr, 76Sr and 80Zr exhibit large shell gap both at the proton and neutron numbers in th…
