We present the creation of a lithium-cesium slow beam using a two-dimensional magneto-optical trap. The two-species atomic beam is directed to load a three-dimensional magneto-optical trap in ultrahigh vacuum. We achieve a loading rate of 1.3$\times$10$^{7}$ lithium atoms/s with the lithium oven temperature at 370~$^{\circ}$C and 2.2$\times$10$^{7}$ cesium atoms/s with the Cs oven temperature at 20~$^{\circ}$C. The maximum numbers of lithium and cesium atoms in the trap are 1.0$\times$10$^{9}$ and 1.4$\times$10$^{8}$, respectively. Our results show that the simple and compact two-dimensional magneto-optical trap is suitable for producing an atomic beam of two species that have a large mass ratio and very different volatilities.
We present first indications of sympathetic cooling between two neutral, optically trapped atomic species. Lithium and cesium atoms are simultaneously stored in an optical dipole trap formed by the focus of a CO$_2$ laser, and allowed to interact for a given period of time. The temperature of the lithium gas is found to decrease when in thermal contact with cold cesium. The timescale of thermalization yields an estimate for the Li-Cs cross-section.
We investigate collisional properties of lithium and cesium which are simultaneously confined in a combined magneto-optical trap. Trap-loss collisions between the two species are comprehensively studied. Different inelastic collision channels are identified, and inter-species rate coefficients as well as cross sections are determined. It is found that loss rates are independent of the optical excitation of Li, as a consequence of the repulsive Li$^*$-Cs interaction. Li and Cs loss by inelastic inter-species collisions can completely be attributed to processes involving optically excited cesium…
We present the first simultaneous trapping of two different ultracold atomic species in a conservative trap. Lithium and cesium atoms are stored in an optical dipole trap formed by the focus of a CO$_2$ laser. Techniques for loading both species of atoms are discussed and observations of elastic and inelastic collisions between the two species are presented. A model for sympathetic cooling of two species with strongly different mass in the presence of slow evaporation is developed. From the observed Cs-induced evaporation of Li atoms we estimate a cross section for cold elastic Li-Cs collision…
The heavy Fermi polaron I: the Lithium-Cesium experiment
Physikalisches Institut, Universität Heidelberg（海德堡大学物理研究所）；Department of Physics and Research Center OPTIMAS, RPTU University Kaiserslautern-Landau（凯泽斯劳滕-兰道理工大学物理系与OPTIMAS研究中心）
We simultaneously trap ultracold lithium and cesium atoms in an optical dipole trap formed by the focus of a CO$_2$ laser and study the exchange of thermal energy between the gases. The cesium gas, which is optically cooled to $20 μ$K, efficiently decreases the temperature of the lithium gas through sympathetic cooling. The measured cross section for thermalizing $^{133}$Cs-$^7$Li collisions is $8 \times 10^{-12}$ cm$^2$, for both species in their lowest hyperfine ground state. Besides thermalization, we observe evaporation of lithium purely through elastic cesium-lithium collisions (sympathet…
Experimental and theoretical studies are presented related to the ground-state magneto-optical resonance prepared in Cesium vapour confined in an Extremely Thin Cell (ETC, with thickness equal to the wavelength of the irradiating light). It is shown that the utilization of the ETC allows one to examine the formation of a magneto-optical resonance on the individual hyperfine transitions, thus distinguishing processes resulting in dark (reduced absorption) or bright (enhanced absorption) resonance formation. We report on an experimental evidence of the bright magneto-optical resonance sign rever…
We describe an apparatus designed to trap and cool a Yb and Cs mixture. The apparatus consists of a dual species effusive oven source, dual species Zeeman slower, magneto-optical traps in a single ultra-high vacuum science chamber, and the associated laser systems. The dual species Zeeman slower is used to load sequentially the two species into their respective traps. Its design is flexible and may be adapted for other experiments with different mixtures of atomic species. The apparatus provides excellent optical access and can apply large magnetic bias fields to the trapped atoms. The apparat…
Bright and dark nonlinear magneto-optical resonances associated with the ground state Hanle effect have been studied experimentally and theoretically for D1 excitation of atomic cesium. This system offers the advantage that the separation between the different hyperfine levels exceeds the Doppler width, and, hence, transitions between individual levels can be studied separately. Experimental measurements for various laser power densities and transit relaxation times are compared with a model based on the optical Bloch equations, which averages over the Doppler contour of the absorption line an…
We present and experimental and theoretical study of nonlinear magneto-optical resonances observed in the fluorescence to the ground state from the 7P_{3/2} state of cesium, which was populated directly by laser radiation at 455 nm, and from the 6P_{1/2} and 6P_{3/2} states, which were populated via cascade transitions that started from the 7P_{3/2} state and passed through various intermediate states. The laser-induced fluorescence (LIF) was observed as the magnetic field was scanned through zero. Signals were recorded for the two orthogonal, linearly polarized components of the LIF. We compa…
We report our studies on an intense source of cold cesium atoms based on a two-dimensional magneto-optical trap with independent axial cooling and pushing. The new-designed source, proposed as 2D-HP MOT, uses hollow laser beams for axial cooling and a thin pushing laser beam for cold atomic beam extraction. Regulated independently by the pushing beam, the atomic flux can be substantially optimized. The atomic flux maximum obtained in the 2D-HP MOT is $4.02\times 10^{10}$ atoms/s, increased by 60 percent compared to the traditional 2D$^+$ MOT in our experiment. Moreover, with the pushing power …
We demonstrate the single-photon Rydberg excitation of cesium atoms in a magneto-optical trap (MOT). We excite atoms directly from ${{6S}_{1/2}}$ ground state to ${{nP}_{3/2}}(n=70-100)$ Rydberg state with a narrow-linewidth 319 nm ultra-violet laser. The detection of Rydberg states is performed by monitoring the reduction of fluorescence signal of the MOT as partial population on ${{6S}_{1/2}} (F = 4)$ ground state are transferred to Rydberg state. We clearly observe Autler-Townes doublet in the trap-loss spectra due to the cooling lights. Utilizing the large electric polarizibility of Rydber…
A novel cesium (Cs) two-color magneto-optical trap (TC-MOT), which partially employs the optical radiation forces due to photon scattering of the 6P3/2 (F'=5) - 7S1/2 (F"=4) excited-state transition in the Cs 6S1/2 - 6P3/2 - 7S1/2 (852 + 1470 nm) ladder-type system, has been proposed and experimentally investigated. One of the three pairs of 852 nm cooling/trapping beams (CTBs) in a conventional Cs MOT is replaced with a pair of the 1470 nm CTBs (type-I) or with one 852 nm CTB plus another counter-propagating 1470 nm CTB (type-II). Both the type-I and type-II Cs TC-MOTs can cool and trap atoms…
We have measured magneto-optical signals obtained by exciting the $D_1$ line of cesium atoms confined to an extremely thin cell (ETC), whose walls are separated by less than one micrometer, and developed an improved theoretical model to describe these signals with experimental precision. The theoretical model was based on the optical Bloch equations and included all neighboring hyperfine transitions, the mixing of the magnetic sublevels in an external magnetic field, and the Doppler effect, as in previous studies. However, in order to model the extreme conditions in the ETC more realistically,…
We report on the design, implementation, and performance of a compact two-dimensional magneto-optical trap (2D MOT) for cesium. In a small-volume vacuum chamber, the setup uses cesium dispensers in close proximity to the trapping region of the 2D MOT and operates at low vapor pressures in the $10^{-9}$ torr range. We achieve a cold atom flux of $4 \times 10^8$ atoms/s that is comparable to the performance of more complex atomic sources. The setup is simple to construct and can be adapted to a broad range of atomic species.
We confine 4 10^8 fermionic 6Li atoms simultaneously with 9 10^9 bosonic 7Li atoms in a magneto-optical trap based on an all-semiconductor laser system. We optimize the two-isotope sample for sympathetic evaporative cooling. This is an essential step towards the production of a quantum-degenerate gas of fermionic lithium atoms.
We experimentally investigate trap-loss spectra of the cesium 6S1/2(F=4)-71P3/2 Rydberg state by combining the cesium atomic magneto-optical trap with the narrow-linewidth, continuously-tunable 318.6 nm ultraviolet laser. That is, the atoms in the magneto-optical trap are excited to the Rydberg state due to the ultraviolet laser single-step Rydberg excitation, which leads to the reduction of atomic fluorescence. Based on the trap-loss spectroscopy technology, the Autler-Townes splitting due to strong cooling laser is observed, and the parameter dependence of the AT splitting interval of trap-l…
We present a dual-species oven and Zeeman slower setup capable of producing slow, high-flux atomic beams for loading magneto-optical traps. Our compact and versatile system is based on electronic switching between different magnetic field profiles and is applicable to a wide range of multi-species experiments. We give details of the vacuum setup, coils and simple electronic circuitry. In addition, we demonstrate the performance of our system by optimized, sequential loading of magneto-optical traps of lithium-6 and cesium-133.
We report the measurement of collision rate coefficient for collisions between ultracold Cs atoms and low energy Cs+ ions. The experiments are performed in a hybrid trap consisting of a magneto-optical trap (MOT) for Cs atoms and a Paul trap for Cs+ ions. The ion-atom collisions impart kinetic energy to the ultracold Cs atoms resulting in their escape from the shallow MOT and, therefore, in a reduction in the number of Cs atoms in the MOT. By monitoring, using fluorescence measurements, the Cs atom number and the MOT loading dynamics and then fitting the data to a rate equation model, the ion-…
We present a systematic study on the Raman gray molasses cooling (RGMC) of cesium atoms on the $D_2$ transition. Due to the large splitting in the excited hyperfine transitions of cesium $D_2$ line, it is relatively simple to implement the RGMC with suitable frequency control on the trapping and repumping lasers of the magneto-optical trap (MOT). We have achieved an atom temperature of 1.7$\pm$0.2 $μ$K after the RGMC with $3.2\times 10^8$ atoms. The phase space density is $1.43\times 10^{-4}$. Compared to the condition with a bare MOT or the MOT with a standard polarization gradient cooling, t…
We have successfully implemented the first simultaneous magneto-optical trapping (MOT) of lithium ($^6$Li) and ytterbium ($^{174}$Yb) atoms, towards production of ultracold polar molecules of LiYb. For this purpose, we developed the dual atomic oven which contains both atomic species as an atom source and successfully observed the spectra of the Li and Yb atoms in the atomic beams from the dual atomic oven. We constructed the vacuum chamber including the glass cell with the windows made of zinc selenium (ZnSe) for the CO$_2$ lasers, which are the useful light sources of optical trapping for ev…
We present studies of strong coupling in single-photon photoassociation of cesium dimers using an optical dipole trap. A thermodynamic model of the trap depletion dynamics is employed to extract absolute rate coefficents. From the dependence of the rate coefficient on the photoassociation laser intensity, we observe saturation of the photoassociation scattering probability at the unitarity limit in quantitative agreement with the theoretical model by Bohn and Julienne [Phys. Rev. A, 60, 414 (1999)]. Also the corresponding power broadening of the resonance width is measured. We could not observ…
A compact setup for two-way single-photon-level frequency conversion between 852 nm and 1560 nm has been implemented with the same periodically-poled magnesium-oxide-doped lithium niobate (PPMgO:LN) bulk crystals for connecting cesium D2 line (852 nm) to telecom C-band. By single-pass mixing a strong continuous-wave pump laser at 1878 nm and the single-photon-level periodical signal pulses in a 50-mm-long PPMgO:LN bulk crystal, the conversion efficiency of ~1.7% ( ~1.9%) for 852-nm to 1560-nm down-conversion (1560-nm to 852-nm up-conversion) have been achieved. We analyzed noise photons induce…
Trapping lithium with a big number in a simplified experimental setup has difficulties and challenges today. In this paper, we experimentally demonstrate the enhancement of \textsuperscript{6}Li trapping efficiency in a three-dimensional magneto-optical trap (3D MOT) by using the multiple-sideband cooling in a two-dimensional magneto-optical trap (2D MOT). To improve the number of trapped atoms, we broaden the cooling light spectrum to 102 MHz composed of seven frequency components and then trap atoms with a number of $6.0\times10^8$ which is about 4 times compared to that in the single-freque…
We present an analytic and numerical study for realizing single photon sideband cooling in an ultracold sample of fermionic Lithium trapped in a periodic optical potential. We develop an analytical model and obtain a master equation for the bound level populations. The cooling sequence is simulated both with a laser at a fixed frequency and with a frequency sweep. Finally, a Monte Carlo simulation is performed taking into account the full hyperfine spectrum of $^6\!$Li. We find that a gas of $^6\!$Li atoms loaded from a Magneto-Optical trap into a deep optical lattice can be cooled down to a $…
We demonstrate loading of a Li magneto-optical trap using light-induced atomic desorption. The magneto-optical trap confines up to approximately $4\times10^{4}$ $^{7}\text{Li}$ atoms with loading rates up to approximately $4\times10^{3}$ atoms per second. We study the Li desorption rate as a function of the desorption wavelength and power. The extracted wavelength threshold for desorption of Li from fused silica is approximately $470$ nm. In addition to desorption of lithium, we observe light-induced desorption of background gas molecules. The vacuum pressure increase due to the desorbed backg…
We have used the narrow $2S_{1/2} \rightarrow 3P_{3/2}$ transition in the ultraviolet (uv) to laser cool and magneto-optically trap (MOT) $^6$Li atoms. Laser cooling of lithium is usually performed on the $2S_{1/2} \rightarrow 2P_{3/2}$ (D2) transition, and temperatures of $\sim$300 $μ$K are typically achieved. The linewidth of the uv transition is seven times narrower than the D2 line, resulting in lower laser cooling temperatures. We demonstrate that a MOT operating on the uv transition reaches temperatures as low as 59 $μ$K. Furthermore, we find that the light shift of the uv transition in …
We present a combined theoretical and experimental study of magnetic resonance transitions induced by polarization-modulated light in cesium vapor exposed to a transverse magnetic field. Signals are obtained by phase-sensitive analysis of the light power traversing the vapor cell at six harmonics of the polarization modulation frequency. Resonances appear whenever the Larmor frequency matches an integer multiple of the modulation frequency. We have further investigated the modifications of the spectra when varying the modulation duty cycle. The resonance amplitudes of both in-phase and quadrat…
We demonstrate a Magneto-Optical Trap (MOT) configuration which employs optical forces due to light scattering between electronically excited states of the atom. With the standard MOT laser beams propagating along the {\it x}- and {\it y}- directions, the laser beams along the {\it z}-direction are at a different wavelength that couples two sets of {\it excited} states. We demonstrate efficient cooling and trapping of cesium atoms in a vapor cell and sub-Doppler cooling on both the red and blue sides of the two-photon resonance. The technique demonstrated in this work may have applications in …
We study optical gain in a gas of cold 39K atoms. The gain is observed during operation of a conventional magneto-optical trap without the need for additional fields. Measurements of transmission spectra from a weak probe show that the gain is due to stimulated Raman scattering between hyperfine ground states. The experimental results are reproduced by a simplified six-level model, which also helps explain why such gain is not observed in similar experiments with rubidium or cesium.
Nonlinear magneto-optical Faraday rotation (NMOR) on the potassium D1 and D2 lines was used to study Zeeman relaxation rates in an antirelaxation paraffin-coated 3-cm diameter potassium vapor cell. Intrinsic Zeeman relaxation rates of $γ^{NMOR}/2π=2.0(6) {\rm Hz}$ were observed. The relatively small hyperfine intervals in potassium lead to significant differences in NMOR in potassium compared to rubidium and cesium. Using laser optical pumping, widths and frequency shifts were also determined for transitions between ground-state hyperfine sublevels of $^{39}$K atoms contained in the same paraf…
We report observation of sub-Doppler cooling of lithium using an irregular-tetrahedral laser beam arrangement, which is produced by a nanofabricated diffraction grating. We are able to capture 11(2) % of the lithium atoms from a grating magneto-optical trap into $Λ$-enhanced $D_1$ gray molasses. The molasses cools the captured atoms to a radial temperature of 60(9) $μ$K and an axial temperature of 23(3) $μ$K. In contrast to results from conventional counterpropagating beam configurations, we do not observe cooling when our optical fields are detuned from Raman resonance. An optical Bloch equat…
This thesis is divided into two parts, each of which supports constructing and using a lithium magneto-optical trap for cold collision studies: Part I: One outgoing channel of interest from cold collisions is the production of ion pairs. We describe an effective method for calculating bound-to-continuum cross-sections for charged binary systems by examining transitions to states above the binding energy that become bound when the system is placed within an infinite spherical well. This approach is verified for ionization of a hydrogen atom, and is then applied to the heavy Rydberg system Li+..…
We have detected and analysed narrow high-contrast coherent population trapping (CPT) resonances, which are induced in absorption of the weak probe light beam by the counterpropagating two-frequency pumping radiation. Our experimental investigations have been carried out on example of nonclosed three level Lambda systems formed by spectral components of the Doppler broadened D2 line of cesium atoms. We have established that CPT resonances in transmission of the probe beam (in the cesium vapor), at definite conditions, may have not only more contrast but also much lesser width in comparison wit…
Vector field measurement is demonstrated with an all-optical scalar atomic magnetometer using intrinsic parameters related to its scalar operation. The Bell-Bloom type atomic magnetometer measures the Larmor precession of cesium atoms through on-resonant absorption of a probe beam. While the AC component of the probe signal is used for the field magnitude measurement, the probe DC signal contains information about the polar angle, defined as the angle between the magnetic field and the probe beam. Additional polar angle information is obtained from the light-shift-induced magnetic field caused…
We report on a simple oven-loaded magneto-optical trap (MOT) apparatus for the creation of both molecular Bose-Einstein condensates (mBEC) and degenerate Fermi gases (DFGs) of lithium. The apparatus does not require a Zeeman slower or a 2D MOT nor does it require any separation or differential pumping between the effusive atom source and the science chamber. The result is an exceedingly simple, inexpensive, and compact vacuum system ideal for miniaturization. We discuss our work in the context of other realizations of quantum degenerate gases by evaporation in optical dipole traps and illustra…
Atom interferometry has become one of the most powerful technologies for precision measurements. To develop simple, precise, and versatile atom interferometers for inertial sensing, we demonstrate an atom interferometer measuring acceleration, rotation, and inclination by pointing Raman beams toward individual faces of a pyramidal mirror. Only a single diode laser is used for all functions, including atom trapping, interferometry, and detection. Efficient Doppler-sensitive Raman transitions are achieved without the velocity selecting the atom sample, and with zero differential AC Stark shift b…
We demonstrate trapping and quantum state control of single Cesium atoms in a 532 nm wavelength bottle beam trap. The three dimensional trap is formed by crossing two unit charge vortex beams. Single atoms are loaded with 50% probability directly from a magneto-optical trap. We achieve a trapping lifetime of up to 6 s, and demonstrate fast Rabi oscillations with a coherence time of $T_2\sim 43 \pm 9\rm ms$.
We have shown that it is possible to model accurately optical phenomena in intense laser fields by taking into account the intensity distribution over the laser beam. We developed a theoretical model that divided an intense laser beam into concentric regions, each with a Rabi frequency that corresponds to the intensity in that region, and solved a set of coupled optical Bloch equations for the density matrix in each region. Experimentally obtained magneto-optical resonance curves for the $F_g=2\longrightarrow F_e=1$ transition of the $D_1$ line of $^{87}$Rb agreed very well with the theoretica…
We present an efficient scheme to implement a gray optical molasses for sub-Doppler cooling of $^{6}$Li atoms with minimum experimental overhead. To integrate the $D_1$ light for the gray molasses (GM) cooling into the same optical setup that is used for the $D_2$ light for a standard magneto-optical trap (MOT), we rapidly switch the injection seeding of a slave laser between the $D_2$ and $D_1$ light sources. Switching times as short as $30\,μ\textrm{s}$ can be achieved, inferred from monitor optical beat signals. The resulting low-intensity molasses cools a sample of $N=9\times10^8$ atoms to…
We present quantitative measurements of the photoassociation of cesium molecules inside a far-detuned optical dipole trap. A model of the trap depletion dynamics is derived which allows to extract absolute photoassociation rate coefficients for the initial single-photon photoassociation step from measured trap-loss spectra. The sensitivity of this approach is demonstrated by measuring the Franck-Condon modulation of the weak photoassociation transitions into the low vibrational levels of the outer well of the 0g- state that correlates to the 6s+6p3/2 asymptote. The measurements are compared to…
We report the design and performance of a non-magnetic drift stable optically pumped cesium magnetometer with a measured sensitivity of 35 fT at 200 s integration time and stability below 50 fT between 70 s and 600 s. To our knowledge this is the most stable magnetic field measurement to date. The sensor is based on the nonlinear magneto-optical rotation effect: in a Bell-Bloom configuration a higher order polarization moment (alignment) of Cs atoms is created with a pump laser beam in an anti-relaxation coated Pyrex cell under vacuum, filled with Cs vapor at room temperature. The polarization…
A reaction microscope (ReMi) has been combined with a magneto-optical trap (MOT) for the kinematically complete investigation of atomic break-up processes. With the novel MOTReMi apparatus, the momentum vectors of the fragments of laser-cooled and state-prepared lithium atoms are measured in coincidence and over the full solid angle. %Earlier attempts to realize this combination failed due to intrinsic incompatibilities of the magnetic fields required for MOT and ReMi. The first successful implementation of a MOTReMi could be realized due to an optimized design of the present setup, a nonstand…
