We theoretically investigate the Floquet generation of second-order topological superconducting (SOTSC) phase in the high-temperature platform both in two-dimension (2D) and three-dimension (3D). Starting from a $d$-wave superconducting pairing gap, we periodically kick the mass term to engineer the dynamical SOTSC phase within a specific range of the strength of the drive. Under such dynamical breaking of time-reversal symmetry (TRS), we show the emergence of the \textit{weak} SOTSC phase, harboring eight corner modes \ie two zero-energy Majorana per corner, with vanishing Floquet quadrupole moment. On the other hand, our study interestingly indicates that upon the introduction of an explicit TRS breaking Zeeman field, the \textit{weak} SOTSC phase can be transformed into \textit{strong} SOTSC phase, hosting one zero-energy Majorana mode per corner, with quantized quadrupole moment. We also compute the Floquet Wannier spectra that further establishes the \textit{weak} and \textit{strong} nature of these phases. We numerically verify our protocol computing the exact Floquet operator in open boundary condition and then analytically validate our findings with the low energy effective theory (in the high-frequency limit). The above protocol is applicable for 3D as well where we find one dimensional (1D) hinge mode in the SOTSC phase. We then show that these corner modes are robust against moderate disorder and the topological invariants continue to exhibit quantized nature until disorder becomes substantially strong. The existence of zero-energy Majorana modes in these higher-order phases is guaranteed by the anti-unitary spectral symmetry.
Superconductors with unconventional pairings have been a fascinating subject of research, for which a central issue is to explore effects that can be used to characterize the pairing. The process of Andreev reflection--the reflection of an electron as a hole at a normal-mental-superconductor interface by transferring a Cooper pair into the superconductor--offers a basic mechanism to probe the pairing through transport. Here we predict that in Andreev reflection from unconventional superconductors, the reflected hole acquires an anomalous spatial shift normal to the plane of incidence, arising …
We study an unconventional quantum Hall effect for the surface states of ultrathin Floquet topological insulators in a perpendicular magnetic field. The resulting band structure is modified by photon dressing and the topological property is governed by the low-energy dynamics of a single surface. An exchange of symmetric and antisymmetric surface states occurs by reversing the light's polarization. We find a novel quantum Hall state in which the zeroth Landau level undergoes a phase transition from a trivial insulator state, with Hall conductivity $σ_{yx}=0$ at zero Fermi energy, to a Hall ins…
Fingerprints of unconventional pairing in superconductor-hole-gas heterostructures
Institute of Science and Technology Austria (ISTA)（奥地利科学技术研究所）；Niels Bohr Institute, University of Copenhagen（哥本哈根大学尼尔斯·玻尔研究所）；Department of Physics, Norwegian University of Science and Technology（挪威科技大学物理系）
Floquet engineering provides a toolbox for the realization of novel quantum phases without static counterparts, while conventionally the realization may rely on the manipulation of complex temporal evolution. Here we propose a systematic and high-precision scheme to realize unconventional Floquet topological phases by engineering local band structures in particular momentum subspace called band inversion surfaces (BISs). This scheme is based on a new bulk-boundary correspondence that for a class of generic $d$-dimensional periodically driven systems, the local topological structure formed in e…
We report observation of the nonlinear Meissner effect (NLME) in Nb films by measuring the resonance frequency of a planar superconducting cavity as a function of the magnitude and the orientation of a parallel magnetic field. Use of low power rf probing in films thinner than the London penetration depth, significantly increases the field for the vortex penetration onset and enables NLME detection under true equilibrium conditions. The data agree very well with calculations based on the Usadel equations. We propose to use NLME angular spectroscopy to probe unconventional pairing symmetries in …
We study and classify the proximity-induced superconducting pairing in a topological insulator (TI)-superconductor (SC) hybrid structure for SCs with different symmetries. The Dirac surface state gives a coupling between spin-singlet and spin-triplet pairing amplitudes as well as pairing that is odd in frequency for p-wave SCs. We also find that all SCs induce pairing that is odd in both frequency and orbital (band) index, with oddness in frequency and orbital index being completely interchangeable. The different induced pairing amplitudes significantly modifies the density of states in the TI…
Revealing Hidden Unconventional Pairing through Nonreciprocal Transport
International Center for Quantum Materials, School of Physics, Peking University（北京大学物理学院量子材料科学中心）；Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）；Department of Physics, Hong Kong University of Science and Technology（香港科技大学物理系）；Department of Physics, The University of Tokyo（东京大学物理学系）；CAS Key Laboratory of Theoretical Physics, Institute of Theoretical Physics, Chinese Academy of Sciences（中国科学院理论物理研究所理论物理国家重点实验室）；School of Physical Science and Technology, Soochow University（苏州大学物理科学与技术学院）；Institute for Advanced Study, Soochow University（苏州大学未来技术学院）；Interdisciplinary Center for Theoretical Physics and Information Sciences, Fudan University（复旦大学理论物理与信息科学交叉研究中心）；Hefei National Laboratory（合肥国家实验室）
We develop a theory for interlayer pairing of chiral electrons in graphene materials which results in an unconventional superconducting (S) state with s-wave spin-triplet order parameter. In a pure bilayer graphene, this superconductivity exhibits a gapless property with an exotic effect of temperature-induced condensation causing an increase of the pairing amplitude (PA) with increasing temperature. We find that a finite doping opens a gap in the excitation spectrum and weakens this anomalous temperature-dependence. We further explore the possibility of realizing variety of pairing patterns w…
The formation of electron pairs is a prerequisite of superconductivity. The fermionic nature of electrons yields four classes of superconducting correlations with definite symmetry in spin, space and time. Here, we suggest double quantum dots coupled to conventional s-wave superconductors in the presence of inhomogeneous magnetic fields as a model system exhibiting unconventional pairing. Due to their small number of degrees of freedom, tunable by gate voltages, quantum-dot systems provide an ideal tool to gain fundamental insight in unconventional pairing. We propose two detection schemes for…
Microscopic details such as interactions and Fermiology determine the structure of superconducting pairing beyond the spatial symmetry classification along irreducible point group representations. From the effective pairing vertex, the pairing wave function related to superconducting order unfolds in its orbital-resolved Fourier profile which we call the harmonic fingerprint (HFP). The HFP allows to formulate a concise connection between microsopic parameter changes and their impact on superconductivity. From a random phase approximation analysis of twisted bilayer graphene (TBG) involving $d+…
College of Science, China University of Petroleum (East China)（中国石油大学（华东）理学院）；Eastern Institute of Technology（东方理工大学）；Center for Quantum Transport and Thermal Energy Science, Institute of Physics Frontiers and Interdisciplinary Sciences, School of Physics and Technology, Nanjing Normal University（南京师范大学物理科学与技术学院前沿交叉科学研究院量子输运与热能源科学中心）；National Laboratory of Solid State Microstructures, Nanjing University（南京大学固体微结构物理全国重点实验室）；Jiangsu Physical Science Research Center（江苏省物理科学研究中心）
It has been shown that long-range {\it p}-wave superconductivity in a Kitaev chain can be engineered via an ac field with a high frequency [Benito et al., Phys. Rev. B 90, 205127 (2014)]. For its experimental realization, however, theoretical understanding of Floquet engineering with a broader range of driving frequencies becomes important. In this work, focusing on the ac-driven tunneling interactions of a Kitaev chain, we investigate effects from the leading correction to the high-frequency limit on the emergent {\it p}-wave superconductivity. Importantly, we find new engineered long-range {…
We study the proximity-induced superconducting state in a general bilayer -- conventional $s$-wave superconductor hybrid structure. For the bilayer we include a general parabolic dispersion, Rashba spin-orbit coupling, and finite layer tunneling as well as the possibility to apply a bias potential and a magnetic Zeeman field, in order to address experimentally relevant bilayer systems, ranging from topological insulator thin films to generic double quantum well systems. By extracting the proximity-induced anomalous Green's function in the bilayer we show on a very rich structure for the superc…
We explore transport properties of a normal metal-superconductor-normal metal (NSN) junction, where the superconducting region supports mixed singlet and chiral triplet pairings. We show that in the subgapped regime when the chiral triplet pairing amplitude dominates over that of the singlet, a resonance phenomena emerges out where all the quantum mechanical scattering probabilities acquire a value of 0.25. At the resonance, crossed Andreev reflection mediating through such junction, acquires a zero energy peak. This reflects as a zero energy peak in the conductance as well in the topological …
Signatures of nodal line/point superconductivity have been observed in half-Heusler compounds, such as LnPtBi (Ln = Y, Lu). Topologically non-trivial band structures, as well as topological surface states, has also been confirmed by angular-resolved photoemission spectroscopy in these compounds. In this work, we present a systematical classification of possible gap functions of bulk states and surface states in half-Heusler compounds and the corresponding topological properties based on the representations of crystalline symmetry group. Different from all the previous studies based on four ban…
We show that a chain of nonmagnetic impurities deposited on a fully gapped two- or three-dimensional superconductor can become a topological one-dimensional superconductor with protected Majorana bound states at its end. A prerequisite is that the pairing potential of the underlying superconductor breaks the spin-rotation symmetry, as it is generically the case in systems with strong spin-orbit coupling. We illustrate this mechanism for a spinless triplet-superconductor p+ip and a time-reversal symmetric Rashba superconductor with a mixture of singlet and triplet pairing. For the latter, we sh…
We have performed angle-resolved photoemission spectroscopy (ARPES) on Cux(PbSe)5(Bi2Se3)6 (CPSBS; x = 1.47), a superconductor derived from a topological insulator heterostructure, to elucidate the electronic states relevant to the occurrence of possible unconventional superconductivity. Upon Cu intercalation into the parent compound (PbSe)5(Bi2Se3)6, we observed a distinct energy shift of the bulk conduction band due to electron doping. Photon-energy dependent ARPES measurements of CPSBS revealed that the observed bulk band forms a cylindrical electronlike Fermi surface at the Brillouin-zone …
Giant perpendicular Edelstein polarization in 2D compensated magnets via bichromatic Floquet driving
Georgetown University（乔治城大学）；Uppsala University（乌普萨拉大学）；Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理学研究所）；Czech Academy of Sciences（捷克科学院）
Bilayer transition metal dichalcogenides (TMDs) belong to a class of materials with two unique features, the coupled spin-valley-layer degrees of freedom and the crystal structure that is globally centrosymmetric but locally non-centrosymmetric. In this work, we will show that the combination of these two features can lead to a rich phase diagram for unconventional superconductivity, including intra-layer and inter-layer singlet pairings and inter-layer triplet pairings, in bilayer superconducting TMDs. In particular, we predict that the inhomogeneous Fulde-Ferrell-Larkin-Ovchinnikov state can…
We study the unconventional superconducting correlations caused by a single isolated magnetic impurity in a conventional s-wave superconductor. Due to the local breaking of time-reversal symmetry, the impurity induces unconventional superconductivity which is even in both space and spin variables but odd under time inversion. We derive an exact proportionality relation between the even-frequency component of the local electron density of states and the imaginary part of the odd-frequency local pairing function. By applying this relation to scanning tunneling microscopy spectra taken on top of …
Unconventional superconductivity arising from the interplay between strong spin-orbit coupling and magnetism is an intensive area of research. One form of unconventional superconductivity arises when Cooper pairs subjected to a magnetic exchange coupling acquire a finite momentum. Here, we report on a signature of finite momentum Cooper pairing in the 3D topological insulator Bi2Se3. We apply in-plane and out-of-plane magnetic fields to proximity-coupled Bi2Se3 and find that the in-plane field creates a spatially oscillating superconducting order parameter in the junction as evidenced by the e…
The recent discoveries of higher-order topological insulators (HOTIs) have shifted the paradigm of topological materials, which was previously limited to topological states at boundaries of materials, to those at boundaries of boundaries, such as corners . So far, all HOTI realisations have assumed static equilibrium described by time-invariant Hamiltonians, without considering time-variant or nonequilibrium properties. On the other hand, there is growing interest in nonequilibrium systems in which time-periodic driving, known as Floquet engineering, can induce unconventional phenomena includi…
Electronic bands featuring nontrivial bulk topological invariant manifest through robust gapless modes at the boundaries, e.g., edges and surfaces. As such this bulk-boundary correspondence is also operative in driven quantum materials. For example, a suitable periodic drive can convert a trivial insulator into a Floquet topological insulator (FTI) that accommodates nondissipative dynamic gapless modes at the interfaces with vacuum. Here we theoretically demonstrate that dislocations, ubiquitous lattice defects in crystals, can probe FTIs as well as unconventional $π$-trivial insulator in the …
Majorana edge modes are candidate elements of topological quantum computing. In this work, we purpose a Floquet engineering approach to generate arbitrarily many non-Hermitian Majorana zero and $π$ modes at the edges of a one-dimensional topological superconductor. Focusing on a Kitaev chain with periodically kicked superconducting pairings and gain/losses in the chemical potential or nearest neighbor hopping terms, we found rich non-Hermitian Floquet topological superconducting phases, which are originated from the interplay between drivings and non-Hermitian effects. Each of the phases is ch…
