The exact time-dependent potential energy surface driving the nuclear dynamics was recently shown to be a useful tool to understand and interpret the coupling of nuclei, electrons, and photons, in cavity settings. Here we provide a detailed analysis of its structure for exactly-solvable systems that model two phenomena: cavity-induced suppression of proton-coupled electron transfer and its dependence on the initial state, and cavity-induced electronic excitation. We demonstrate the inadequacy of simply using a weighted average of polaritonic surfaces to determine the dynamics. Such a weighted average misses a crucial term that redistributes energy between the nuclear and the polaritonic systems, and this term can in fact become a predominant term in determining the nuclear dynamics when several polaritonic surfaces are involved. Evolving an ensemble of classical trajectories on the exact potential energy surface reproduces the nuclear wavepacket quite accurately while evolving on the weighted polaritonic surface fails after a short period of time. The implications and prospects for application of mixed quantum-classical methods based on this surface are discussed.
Cavity resonators are promising resources for quantum technology, while native nonlinear interactions for cavities are typically too weak to provide the level of quantum control required to deliver complex targeted operations. Here we investigate a scheme to engineer a target Hamiltonian for photonic cavities using ancilla qubits. By off-resonantly driving dispersively coupled ancilla qubits, we develop an optimized approach to engineering an arbitrary photon-number-dependent (PND) Hamiltonian for the cavities while minimizing the operation errors. The engineered Hamiltonian admits various app…
We propose a feasible scheme to cool down a mechanical resonator (MR) in a three-mirror cavity optomechanical system with controllable external optical drives. Under the Born-Oppenheimer (BO) approximation, the whole dynamics of the mechanical resonator and cavities is reduced to that of a time-dependent harmonic oscillator, whose effective frequency can be controlled through the optical driving fields. The fast cooling of the MR can be realized by controlling the amplitude of the optical drives. Significantly, we further show that the ground-state cooling may be achieved via the three-mirror …
We study the creation of photons in resonant cylindrical cavities with time dependent length. The physical degrees of freedom of the electromagnetic field are described using Hertz potentials. We describe the general formalism for cavities with arbitrary section. Then we compute explicitly the number of TE and TM motion-induced photons for cylindrical cavities with rectangular and circular sections. We also discuss the creation of TEM photons in non-simply connected cylindrical cavities.
Cavities with extremely narrow linewidth of 10-100 Hz are required for realizing frequency dependent squeezing to enable gravitational wave detectors to surpass the free mass standard quantum limit over a broad frequency range. Hundred-meter-scale high finesse cavities have been proposed for this purpose. Optomechanically induced transparency (OMIT) enables the creation of optomechanical cavities in which the linewidth limit is set by the extremely narrow linewidth of a high Q factor mechanical resonator. Using an 85mm OMIT cavity with a silicon nitride membrane, we demonstrate a tunable linew…
We report a theoretical study of a quantum optical model consisting of an array of strongly nonlinear cavities incoherently pumped by an ensemble of population-inverted two-level atoms. Projective methods are used to eliminate the atomic dynamics and write a generalized master equation for the photonic degrees of freedom only, where the frequency-dependence of gain introduces non-Markovian features. In the simplest single cavity configuration, this pumping scheme gives novel optical bistability effects and allows for the selective generation of Fock states with a well-defined photon number. Fo…
The transfer of entangled, quantum correlated, flying photons from a squeezed field to single-mode cavities is investigated. It is shown that, while the transfer of photons begins immediately after the input squeezed field is turned on, the time at which quantum correlations start to be transferred to the cavities is strongly dependent on the initial population of the cavities. For the initially empty cavities, the transfer of quantum correlations begins immediately after the squeezed field is turned on, but it is delayed by a certain time interval when the cavities are initially populated. We…
An electron floating on the liquid Helium is proposed to be trapped (by a micro-electrode set below the liquid Helium) in a high finesse cavity. Two lowest levels of the vertical motion of the electron acts as a two-level "atom", which could resonantly interact with the THz cavity. In the Lamb-Dicke regime, wherein the electron's in-plane activity region is much smaller than the wavelength of the cavity mode, the famous Jaynes-Cummings model (JCM) could be realized. By applying an additional external classical laser beam to the electron, a driven JCM could also be implemented. With such a driv…
Significant improvements in superconducting qubit coherence times have been achieved recently with three-dimensional microwave waveguide cavities coupled to transmon qubits. While many of the measurements in this direction have utilized superconducting aluminum cavities, other recent work has involved qubits coupled to copper cavities with coherence times approaching 0.1 ms. The copper provides a good path for thermalizing the cavity walls and qubit chip, although the substantial cavity loss makes conventional dispersive qubit measurements challenging. We are exploring various approaches for i…
The Quantum-Electrodynamical Time-Dependent Density Functional Theory (QED-TDDFT) equations are solved by time propagating the wave function on a tensor product of a Fock-space and real-space grid. Applications for molecules in cavities show the accuracy of the approach. Examples include the coupling strength and light frequency dependence of the energies, wave functions, optical absorption spectra, and Rabi splitting magnitudes in cavities, as well as a description of high harmonic generation in cavities.
The exact reduced dynamics for the independent oscillator model in the RWA approximation at zero and finite temperatures is derived. It is shown that the information about the interaction and the environment is encapsulated into three time dependent coefficients of the master equation, one of which vanishes in the zero temperature case. In currently used optical cavities all the information about the field dynamics is contained into {\it two} (or three) experimentally accesible and physically meaningful real functions of time. From the phenomenological point of view it suffices then to careful…
We study the optical properties of coupled quantum dot-microcavity systems with elliptical cross section. First, we develop an analytic model that describes the spectrum of the cavity modes that are split due to the reduced symmetry of the resonator. By coupling the QD emission to the polarized fundamental cavity modes, we observe the vectorial nature of the Purcell enhancement, which depends on the intrinsic polarization of the quantum dot and its relative alignment with respect to the cavity axis. The variable interaction strength of the QD with the polarized cavity modes leads to the observ…
We explore the photon transfer in the nonlinear parity-time-symmetry system of two coupled cavities, which contains nonlinear gain and loss dependent on the intracavity photons. Analytical solution to the steady state gives a saturated gain, which satisfy the parity-time symmetry automatically. The eigen-frequency self-adapts the nonlinear saturated gain to reach the maximum efficiency in the steady state. We find that the saturated gain in the weak coupling regime does not match the loss in the steady state, exhibiting an appearance of a spontaneous symmetry-breaking. The photon transmission …
The standard description of cavity-modified molecular reactions typically involves a single (resonant) mode, while in reality the quantum cavity supports a range of photon modes. Here we demonstrate that as more photon modes are accounted for, physico-chemical phenomena can dramatically change, as illustrated by the cavity-induced suppression of the important and ubiquitous process of proton-coupled electron-transfer. Using a multi-trajectory Ehrenfest treatment for the photon-modes, we find that self-polarization effects become essential, and we introduce the concept of self-polarization-modi…
Research on photonic cavities with low mode volume and high quality factor garners much attention because of applications ranging from optoelectronics to cavity quantum electrodynamics (QED). We propose a cavity based on surface plasmon modes confined by metallic distributed Bragg reflectors. We analyze the structure with Finite Difference Time Domain simulations and obtain modes with quality factor 1000 (including losses from metals), reduced mode volume relative to photonic crystal cavities, Purcell enhancements of hundreds, and even the capability of enabling cavity QED strong coupling.
Strong coupling of molecules to the vacuum field of micro cavities can modify the potential energy surfaces opening new photophysical and photochemical reaction pathways. While the influence of laser fields is usually described in terms of classical field, coupling to the vacuum state of a cavity has to be described in terms of dressed photon-matter states (polaritons) which require quantized fields. We present a derivation of the non-adiabatic couplings for single molecules in the strong coupling regime suitable for the calculation of the dressed state dynamics. The formalism allows to use qu…
The ongoing global effort to detect gravitational waves continues to push the limits of precision measurement while aiming to provide a new tool for understanding both astrophysics and fundamental physics. Squeezed states of light offer a proven means of increasing the sensitivity of gravitational wave detectors, potentially increasing the rate at which astrophysical sources are detected by more than an order of magnitude. Since radiation pressure noise plays an important role in advanced detectors, frequency dependent squeezing will be required. In this paper we propose a practical approach t…
We present a novel method of machining optical fiber surfaces with a CO${}_2$ laser for use in Fiber-based Fabry-Perot Cavities (FFPCs). Previously FFPCs were prone to large birefringence and limited to relatively short cavity lengths ($\le$ 200 $μ$m). These characteristics hinder their use in some applications such as cavity quantum electrodynamics with trapped ions. We optimized the laser machining process to produce large, uniform surface structures. This enables the cavities to achieve high finesse even for long cavity lengths. By rotating the fibers around their axis during the laser mach…
Spoof surface modes on nanostructured metallic surfaces are known to have tailorable dispersion dependent on the geometric characteristics of the periodic pattern. Here we examine the spoof plasmon dispersion on an isolated grating and a grating-planar mirror cavity configuration. The spoof polariton dispersion in the cavity is obtained using the scattering matrix approach, and the related differential modal density of states is introduced to obtain the mode dispersion and classify the cavity polariton modes. The grating-mirror cavity geometry is an example of periodically nanostructured metal…
We report on measurements of the Casimir force in a sphere-plane geometry using a cryogenic force microscope to move the force probe in situ over different materials. We show how the electrostatic environment of the interacting surfaces plays an important role in weak force measurements and can overcome the Casimir force at large distance. After minimizing these parasitic forces, we measure the Casimir force between a gold-coated sphere and either a gold-coated or a heavily doped silicon surface in the 100-400 nm distance range. We compare the experimental data with theoretical predictions and…
We demonstrate the fabrication of ultra-low-loss, all-fiber Fabry-Pérot cavities containing a nanofiber section, optimized for cavity quantum electrodynamics. By continuously monitoring the finesse and fiber radius during fabrication of a nanofiber between two fiber Bragg gratings, we are able to precisely evaluate taper transmission as a function of radius. The resulting cavities have an internal round-trip loss of only 0.31% at a nanofiber waist radius of 207 nm, with a total finesse of 1380, and a maximum expected internal cooperativity of $\sim$ 1050 for a cesium atom on the nanofiber surf…
We study a range of radio-frequency ion trap geometries and investigate the effect of integrating dielectric cavity mirrors on their trapping potential. We aim to identify ion trap and cavity configurations that are best suited for achieving small cavity volumes and thus large ion-photon coupling as required for scalable quantum information networks. In particular, we investigate the trapping potential distortions caused by the dielectric material of the cavity mirrors for different mirror orientations with respect to the trapping electrodes, as well as for mirror misalignment. We also analyze…
