Research on photonic cavities with low mode volume and high quality factor garners much attention because of applications ranging from optoelectronics to cavity quantum electrodynamics (QED). We propose a cavity based on surface plasmon modes confined by metallic distributed Bragg reflectors. We analyze the structure with Finite Difference Time Domain simulations and obtain modes with quality factor 1000 (including losses from metals), reduced mode volume relative to photonic crystal cavities, Purcell enhancements of hundreds, and even the capability of enabling cavity QED strong coupling.
Plasmon-enhanced Raman scattering can push single-molecule vibrational spectroscopy beyond a regime addressable by classical electrodynamics. We employ a quantum electrodynamics (QED) description of the coherent interaction of plasmons and molecular vibrations that reveal the emergence of nonlinearities in the inelastic response of the system. For realistic situations, we predict the onset of \textit{phonon-stimulated Raman scattering} and an counter-intuitive dependence of the anti-Stokes emission on the frequency of excitation. We further show that this novel QED framework opens a venue to a…
We report a process for fabricating high quality, defect-free spherical mirror templates suitable for developing high finesse optical Fabry-Perot resonators. The process utilizes the controlled reflow of borosilicate glass and differential pressure to produce mirrors with 0.3 nanometer surface roughness. The dimensions of the mirrors are in the 0.5-5mm range making them suitable candidates for integration with on-chip neutral atom and ion experiments where enhanced interaction between atoms and photons are required. Moreover the mirror curvature, dimension and placement is readily controlled a…
We introduce a second quantization scheme based on quasinormal modes, which are the dissipative modes of leaky optical cavities and plasmonic resonators with complex eigenfrequencies. The theory enables the construction of multi-plasmon/photon Fock states for arbitrary three-dimensional dissipative resonators and gives a solid understanding to the limits of phenomenological dissipative Jaynes-Cummings models. In the general case, we show how different quasinormal modes interfere through an off-diagonal mode coupling and demonstrate how these results affect cavity-modified spontaneous emission.…
We investigate chiral emission and the single-photon scattering of spinning cavities coupled to a meandering waveguide at multiple coupling points. It is shown that nonreciprocal photon transmissions occur in the cavities-waveguide system, which stems from interference effects among different coupling points, and frequency shifts induced by the Sagnac effect. The nonlocal interference is akin to the mechanism in giant atoms. In the single-cavity setup, by optimizing the spinning velocity and number of coupling points, the chiral factor can approach 1, and the chiral direction can be freely swi…
A recent work [1] proposed a type of cluster entangled coherent states and its generation. Here we present an alternative experimental arrangement for its generation in bimodal QED cavities. The scheme employs a single two-level atom that interacts dispersively with cavity modes initially prepared in coherent states. The fidelity and success probability of the state preparation are obtained considering the influence of atomic velocity spread and atomic efficiency detection.
The strong interaction of individual quantum emitters with resonant cavities is of fundamental interest for understanding light matter interactions. Plasmonic cavities hold the promise of attaining the strong coupling regime even under ambient conditions and within subdiffraction volumes. Recent experiments revealed strong coupling between individual plasmonic structures and multiple organic molecules, but so far strong coupling at the limit of a single quantum emitter has not been reported. Here we demonstrate vacuum Rabi splitting, a manifestation of strong coupling, using silver bowtie plas…
We propose an experiment with two coupled microwave cavities and a "tunneling" photon observed by the passage of Rydberg atoms. We model the coupled cavities as in Ref. \cite{art1} and include dissipative effects as well as limited detection efficiency. We also consider realistic finite atom-field interaction times and provide for a simple analytical expression for the photon "tunneling" probability including all these effects. We show that for sufficiently small dissipation constants the effect can be observed with current experimental facilities.
Electromagnetic cavity modes in photonic and plasmonic resonators offer rich and attractive regimes for tailoring the properties of light-matter interactions. Yet there is a disturbing lack of a precise definition for what constitutes a cavity mode, and as a result their mathematical properties remain largely unspecified. The lack of a definition is evidenced in part by the diverse nomenclature at use - "resonance", "leaky mode", "quasimode", to name but a few - suggesting that the dissipative nature of cavity modes somehow makes them different from other modes, but an explicit distinction is …
The problem of longitudinal oscillations of an electric field and a charge polarization density in QED vacuum is considered. Within the framework of semiclassical analysis, we calculate time-periodic solutions of bosonized (1+1)-dimensional QED (massive Schwinger model). Applying the Bohr--Sommerfeld quantization condition, we determine the mass spectrum of charge-zero bound states (plasmons) which correspond in quantum theory to the found classical solutions. We show that the existence of such plasmons does not contradict any fundamental physical laws and study qualitatively their excitation …
We propose a class of quantum simulators for antiferromagnetic spin systems, based on coupled photonic cavities in presence of two-photon driving and dissipation. By modeling the coupling between the different cavities through a hopping term with negative amplitude, we solve numerically the quantum master equation governing the dynamics of the open system and determine its non-equilibrium steady state. Under suitable conditions, the steady state can be described in terms of the degenerate ground states of an antiferromagnetic Ising model. When the geometry of the cavity array is incommensurate…
We present evidence of cavity quantum electrodynamics from a sparse density of strongly quantum-confined Pb-chalcogenide nanocrystals (between 1 and 10) approaching single-dot levels on moderately high-Q mesoscopic silicon optical cavities. Operating at important near-infrared (1500-nm) wavelengths, large enhancements are observed from devices and strong modifications of the QD emission are achieved. Saturation spectroscopy of coupled QDs is observed at 77K, highlighting the modified nanocrystal dynamics for quantum information processing.
We analyze a coupling scheme for qubits in different cavities of circuit-QED architecture. In contrast to the usual scheme where the cavities are coupled by an interface capacitance we employ a bridge qubit connecting cavities to mediate two-qubit coupling. This active coupling scheme makes it possible to switch on/off and adjust the strength of qubit-qubit coupling, which is essential for scalability of quantum circuit. By transforming the Hamiltonian we obtain an exact expression of two-qubit coupling in the rotating-wave approximation. For the general case of $n$ qubits the Hamiltonian can …
In this article we discuss two schemes of teleportation of cavity field states. In the first scheme we consider cavities prepared in a coherent state and in the second scheme we consider cavities prepared in a superposition of zero and one Fock states.
By exploiting a system of three distant cavities, we propose a scheme for constructing tripartite entangled coherent GHZ and W states which are robust due to the photon losses in the cavities. Each of cavities is doped with a semiconductor quantum dot. By the dynamics, the excitonic modes of quantum dots are enabled to exhibit entan-gled coherent GHZ and W states. Apart from the exciton losses, the master equation approach shows that when the populations of the field modes in the cavities are negli-gible the destruction of entanglement due to decoherence arises from photon losses, is effective…
Plasmonic cavities can confine electromagnetic radiation to deep sub-wavelength regimes. This facilitates strong coupling phenomena to be observed at the limit of individual quantum emitters. Here we report an extensive set of measurements of plasmonic cavities hosting one to a few semiconductor quantum dots. Scattering spectra show Rabi splitting, demonstrating that these devices are close to the strong coupling regime. Using Hanbury Brown and Twiss interferometry, we observe non-classical emission, allowing us to directly determine the number of emitters in each device. Surprising features i…
Single excitons in semiconductor microcavities represent a solid-state and scalable platform for cavity quantum electrodynamics (c-QED), potentially enabling an interface between flying (photon) and static (exciton) quantum bits in future quantum networks. While both single-photon emission and the strong coupling regime have been demonstrated, further progress has been hampered by the inability to control the coherent evolution of the c-QED system in real time, as needed to produce and harness charge-photon entanglement. Here, using the ultrafast electrical tuning of the exciton energy in a ph…
We propose a scheme to unconditionally entangle the internal states of atoms trapped in separate high finesse optical cavities. The scheme uses the technique of quantum reservoir engineering in a cascaded cavity QED setting, and for ideal (lossless) coupling between the cavities generates an entangled pure state. Highly entangled states are also shown to be possible for realizable cavity QED parameters and with nonideal coupling.
We present a quantum theory for the interaction of a two level emitter with surface plasmon polaritons confined in single-mode waveguide resonators. Based on the Green's function approach, we develop the conditions for the weak and strong coupling regimes by taking into account the sources of dissipation and decoherence: radiative and non-radiative decays, internal loss processes in the emitter, as well as propagation and leakage losses of the plasmons in the resonator. The theory is supported by numerical calculations for several quantum emitters, GaAs and CdSe quantum dots and NV centers tog…
We propose a scheme on the basis of a N+2 identical single-mode coupled-cavity QED system for selective transfer of a qubit constructed from superposition of standard coherent states. The cavities arranged in such way that the intermediate or channel cavity is connected uniformly to the sender and N receiver cavities. We consider N different ternary sets of identical QDs whose QDs have been distributed in the sender, channel and one of the receiver cavities respectively. We demonstrate a situation in which the dynamics of the system is confined selectively in a sub sector belongs to one of the…
Photonic crystal nanobeam cavities are versatile platforms of interest for optical communications, optomechanics, optofluidics, cavity QED, etc. In a previous work \cite{quan10}, we proposed a deterministic method to achieve ultrahigh \emph{Q} cavities. This follow-up work provides systematic analysis and verifications of the deterministic design recipe and further extends the discussion to air-mode cavities. We demonstrate designs of dielectric-mode and air-mode cavities with $Q>10^9$, as well as cavities with both high-\emph{Q} ($>10^7$) and high on-resonance transmissions ($T>95%$).
We propose a scheme for quantum computing using high-Q cavities in which the qubits are represented by single cavity modes restricted in the space spanned by the two lowest Fock states. We show that single qubit operations and universal multiple qubit gates can be implemented using atoms sequentially crossing the cavities.
In a cavity quantum electrodynamics (QED) system, where atoms coherently interact with photons in a cavity, the eigenstates of the system are the superposition states of atoms and cavity photons, the so-called dressed states of atoms. When two cavities are connected by an optical fiber with negligible loss, the coherent coupling between the cavities gives rise to photonic normal modes. One of these normal modes is the fiber-dark mode, in which photons are delocalized in the two distant cavities. Here we demonstrate the setting of coupled-cavities QED, where two nanofiber cavity-QED systems are…
Using carefully designed hybrid metal-dielectric resonators, we study molecular optomechanics in the strong coupling regime ($g_{\rm }^2/ω_m {>} κ$), which manifests in anharmonic emission lines in the sideband-resolved region of the cavity-emitted spectrum ($κ{<}ω_m$). This nonlinear optomechanical strong coupling regime is enabled through a metal-dielectric cavity system that yields not only deep sub-wavelength plasmonic confinement, but also dielectric-like confinement times that are more than two orders of magnitude larger than those from typical localized plasmon modes. These hybrid metal…
A potential scheme is proposed to generate complete sets of entangled photons in the context of cavity quantum electrodynamics (QED). The scheme includes twice interactions of atoms with cavities, in which the first interaction is made in two-mode optical cavities and the second one exists in a microwave cavity. In the optical cavities the atoms are resonant with the cavity modes, while the detuned interaction of the atoms with a single-mode of the microwave cavity is driven by a classical field. We show that our scheme is carried out with higher efficiency than previeous schemes, and is close…
We propose a method for transferring quantum entangled states of two photonic cat-state qubits (cqubits) from two microwave cavities to the other two microwave cavities. This proposal is realized by using four microwave cavities coupled to a superconducting flux qutrit. Because of using four cavities with different frequencies, the inter-cavity crosstalk is significantly reduced. Since only one coupler qutrit is used, the circuit resources is minimized. The entanglement transfer is completed with a single-step operation only, thus this proposal is quite simple. The third energy level of the co…
We propose to detect the Mott insulator-superfluid quantum phase transition in an array of coupled cavities by studying the polariton and photon fluctuations in a block of linear dimension M (in units of the lattice constant of the array). We explicitly show this for a one-dimensional array; the analysis can be however extended to higher dimensions. In the Mott phase polariton fluctuations are independent of the block size. In the superfluid phase they grow logarithmically with M, the prefactor being related to the compressibility of the system. In the case of photon fluctuations, the critical…
We investigate the phenomenon of sudden transition between classical and quantum decoherence in the study of quantum discord for a dissipative cavity QED system, which consists of two noninteracting two-level atoms, each trapped in a dissipative cavity. It is found that the quantum discord between two atoms, which are prepared initially in the X-type quantum states, is not destroyed by the dissipation of the cavities for a finite time interval and the stationary quantum discord can arise in the interaction of atoms with cavities as the time approach to infinite. The transition time is sensitiv…
In this work, we provide an overview of how well-established concepts in the fields of quantum chemistry and material sciences have to be adapted when the quantum nature of light becomes important in correlated matter-photon problems. Therefore, we analyze model systems in optical cavities, where the matter-photon interaction is considered from the weak- to the strong coupling limit and for individual photon modes as well as for the multi-mode case. We identify fundamental changes in Born-Oppenheimer surfaces, spectroscopic quantities, conical intersections and efficiency for quantum control. …
We introduce a scheme for perfect routing of quantum states and entanglement in regular cavity QED networks. The couplings between the cavities are quasi-uniform and each cavity is doped with a two-level atom. Quasi-uniform couplings leads the system to evolve in invariant subspaces. Combination the evolutions of the system in its invariant subspaces with quite simple local operations on atoms in the networks, gives the perfect routing of quantum states and entanglement through the network. To provide the protocol be robust due to decoherence arisen from photon loss, the field mode of the cavi…
Highly efficient sources of indistinguishable single photons that can operate at room temperature would be very beneficial for many applications in quantum technology. We show that the implementation of such sources is a realistic goal using solid-state emitters and ultrasmall mode volume cavities. We derive and analyze an expression for photon indistinguishability that accounts for relevant detrimental effects, such as plasmon-induced quenching and pure-dephasing. We then provide the general cavity and emitter conditions required to achieve efficient indistinguishable photon emission, and als…
Within the framework of exact quantization of the electromagnetic field in dispersing and absorbing media the input-output problem of a high-$Q$ cavity is studied, with special emphasis on the absorption losses in the coupling mirror. As expected, the cavity modes are found to obey quantum Langevin equations, which could be also obtained from quantum noise theories, by appropriately coupling the cavity modes to dissipative systems, including the effect of the mirror-assisted absorption losses. On the contrary, the operator input-output relations obtained in this way would be incomplete in gene…
Multimode cavity quantum electrodynamics ---where a two-level system interacts simultaneously with many cavity modes---provides a versatile framework for quantum information processing and quantum optics. Due to the combination of long coherence times and large interaction strengths, one of the leading experimental platforms for cavity QED involves coupling a superconducting circuit to a 3D microwave cavity. In this work, we realize a 3D multimode circuit QED system with single photon lifetimes of $2$ ms and cooperativities of $0.5-1.5\times10^9$ across 9 modes of a novel seamless cavity. We d…
We study the zero-temperature phase diagram of a one-dimensional array of QED cavities where, besides the single-photon hopping, an additional coupling between neighboring cavities is mediated by an N-type four-level system. By varying the relative strength of the various couplings, the array is shown to exhibit a variety of quantum phases including a polaritonic Mott insulator, a density-wave and a superfluid phase. Our results have been obtained by means of numerical density-matrix renormalization group calculations. The phase diagram was obtained by analyzing the energy gaps for the polarit…
Suggestion of modifications of finite-dimensional QED models are proposed for interpreting chemical reactions in terms of artificial atoms and molecules on quantum dots placed in optical cavities. Moving both photons and atoms is possible between the cavities. Super dark states of diatomic systems are described, in which the motion of atoms between cavities is impossible due quantum interference. Chemical processes with two level atoms and three level atoms with lambda spectrum are schematically modeled by solving the single quantum master equation with the Lindblad operators of photon leakage…
We propose and analyze a physical implementation of two-qubit parity measurements as required for continuous error correction, assuming a setup in which the individual qubits are strongly coupled to separate optical cavities. A single optical probe beam scatters sequentially from the two cavities and the continuous parity measurement is realized via fixed quadrature homodyne photo-detection. We present models based on quantum stochastic differential equations (QSDE's) for both an ideal continuous parity measurement and our proposed cavity quantum electrodynamics (cavity QED) implementation; a …
In this article we discuss a teleportation scheme of coherent states of cavity field. The experimental realization proposed makes use of cavity quatum electrodynamics involving the interaction of Rydberg atoms with micromaser and Ramsey cavities. In our scheme the Ramsey cavities and the atoms play the role of auxiliary systems used to teleport the state from a micromaser cavity to another. We show that, even if the correct atomic detection fails in the first trials, one can succeed in teleportating the cavity field state if the proper measurement occurs in a later atom.
In the framework of cavity QED, we propose a quantum repeater scheme that uses coherent light and atoms coupled to optical cavities. In contrast to conventional schemes, we exploit solely the cavity QED evolution for the entire quantum repeater scheme and, thus, avoid any explicit execution of quantum logical gates. The entanglement distribution between the repeater nodes is realized with the help of pulses of coherent light interacting with the atom-cavity system in each repeater node. In our previous paper [D. Gonta and P. van Loock, Phys. Rev. A 86, 052312 (2012)], we already proposed a dyn…
We propose a Ramsey interferometry experiment using an entangled state of N atoms to reach the Heisenberg limit for the estimation of an atomic phase shift if the atom number parity is perfectly determined. In a more realistic situation, due to statistical fluctuations of the atom source and the finite detection efficiency, the parity is unknown. We then achieve about half the Heisenberg limit. The scheme involves an ensemble of circular Rydberg atoms which dispersively interact successively with two initially empty microwave cavities. The scheme does not require very high-Q cavities. An exper…
We explore the photon population dynamics in two coupled circuit QED systems. For a sufficiently weak inter-cavity photon hopping, as the photon-cavity coupling increases, the dynamics undergoes double transitions first from a delocalized to a localized phase and then from the localized to another delocalized phase. The latter delocalized phase is distinguished from the former one; instead of oscillating between the two cavities, the photons rapidly quasi-equilibrate over the two cavities. These intrigues are attributed to an interplay between two qualitatively distinctive nonlinear behaviors …
We investigate a chain of superconducting stripline resonators, each interacting with a transmon qubit, that are capacitively coupled in a row. We show that the dynamics of this system can be described by a Bose-Hubbard Hamiltonian with attractive interactions for polaritons, superpositions of photons and qubit excitations. This setup we envisage constitutes one of the first platforms where all technological components that are needed to experimentally study chains of strongly interacting polaritons have already been realized. By driving the first stripline resonator with a microwave source an…
We study the propagation and distribution of quantum correlations through two chains of atoms inside cavities joined by optical fibers. We consider an effective Hamiltonian for the system and cavity losses, in the dressed atom picture, using the Generalized Master Equation.
We investigate the quantum-optical properties of the light emitted by a nanoparticle-on-mirror cavity filled with a single quantum emitter. Inspired by recent experiments, we model a dark-field set-up and explore the photon statistics of the scattered light under grazing laser illumination. Exploiting analytical solutions to Maxwell's equations, we quantize the nanophotonic cavity fields and describe the formation of plasmon exciton polaritons (or plexcitons) in the system. This way, we reveal that the rich plasmonic spectrum of the nanocavity offers unexplored mechanisms for nonclassical ligh…
Development of scalable quantum photonic technologies requires on-chip integration of components such as photonic crystal cavities and waveguides with nonclassical light sources. Recently, hexagonal boron nitride (hBN) has emerged as a promising platform for nanophotonics, following reports of hyperbolic phonon-polaritons and optically stable, ultra-bright quantum emitters. However, exploitation of hBN in scalable, on-chip nanophotonic circuits, quantum information processing and cavity quantum electrodynamics (QED) experiments requires robust techniques for the fabrication of monolithic optic…
This chapter will primarily focus on the studies of quantum optics with semiconductor, epitaxially grown quantum dots embedded in photonic crystal cavities. We will start by giving brief introductions into photonic crystals and quantum dots, then proceed with the introduction to cavity quantum electrodynamics (QED) effects, with a particular emphasis on the demonstration of these effects on the quantum dot-photonic crystal platform. Finally, we will focus on the applications of such cavity QED effects.
Achieving quantum correlations between two distant systems is a desirable feature for quantum networking. In this work, we study a system composed of two quantum emitter-cavity subsystems spatially separated. A mechanical resonator couples to either both quantum emitters or both cavities leading to quantum correlations between both subsystems such as non-local light-matter dressed states and cavity-cavity normal mode splitting. These indirect couplings can be explained by an effective Hamiltonian for large energy detuning between the mechanical resonator and the atoms/cavities. Moreover, it is…
We propose an experimental setup, feasible with present day technology, involving two highquality- factor cavities, one Ramsey zone and a two-level atom which interacts with them. The dynamics in the cavities is modeled by a dissipative dispersive Jaynes-Cummings model. Analytical expresions for the evolution superoperator in each part of the proposed setup and for the concurrence between the atom and the first cavity are given, and the pairwise entanglement of the subsystems is calculated numerically. We consider initial separable states given by the tensor product of a superposition of the t…
Based on a multimode multilevel Jaynes-Cummings model and multiphoton resonance theory, a set of universal two- and three-qubit gates, namely the iSWAP and the Fredkin gates, has been realized where dual-rail qubits are encoded in cavities. In this way the information has been stored in cavities and the off-resonant atomic levels have been eliminated by the semi-classical theory of an effective two-level Hamiltonian. A further semi-classical model, namely the spin-$J$ model, has been introduced so that a complete population inversion for levels of interest has been achieved and periodic multil…
We calculate the weak-driving transmission of a linearly polarized cavity mode strongly coupled to the D2 transition of a single Cesium atom. Results are relevant to future experiments with microtoroid cavities, where the single-photon Rabi frequency g exceeds the excited-state hyperfine splittings, and photonic bandgap resonators, where g is greater than both the excited- and ground-state splitting.
Si3N4 is an excellent material for applications of nanophotonics at visible wavelengths due to its wide bandgap and moderately large refractive index (n $\approx$ 2.0). We present the fabrication and characterization of Si3N4 photonic crystal nanobeam cavities for coupling to diamond nanocrystals and Nitrogen-Vacancy centers in a cavity QED system. Confocal micro-photoluminescence analysis of the nanobeam cavities demonstrates quality factors up to Q ~ 55,000, which is limited by the resolution of our spectrometer. We also demonstrate coarse tuning of cavity resonances across the 600-700nm ran…
In the framework of cavity QED, we propose a practical scheme to purify dynamically a bipartite entangled state using short chains of atoms coupled to high-finesse optical cavities. In contrast to conventional entanglement purification protocols, we avoid CNOT gates, thus reducing complicated pulse sequences and superfluous qubit operations. Our interaction scheme works in a deterministic way, and together with entanglement distribution and swapping, opens a route towards efficient quantum repeaters for long-distance quantum communication.
Considering two-level media in the array of weakly coupled nano-cavities, we reveal a variety of dynamical regimes, such as diffusion, self-trapping, soliton, and breathers for the wave-packets in the presence of photon tunneling processes between the next-nearest cavities. We focus our attention on the low branch (LB) bright polariton soliton formation, due to the two-body polariton-polariton scattering processes. When detuning frequency is manipulated adiabatically, the low-branch lattice polariton localized states, i.e., that are solitons and breathers evolving between photon-like and matte…
We introduce a model of quantum magnetism induced by the non-perturbative exchange of microwave photons between distant superconducting qubits. By interconnecting qubits and cavities, we obtain a spin-boson lattice model that exhibits a quantum phase transition where both qubits and cavities spontaneously polarise. We present a many-body ansatz that captures this phenomenon all the way, from a the perturbative dispersive regime where photons can be traced out, to the non-perturbative ultra-strong coupling regime where photons must be treated on the same footing as qubits. Our ansatz also repro…
