A CUPID Li$_{2}$$^{100}$MoO$_4$ scintillating bolometer tested in the CROSS underground facility
The CUPID Interest Group, A. Armatol, E. Armengaud, W. Armstrong, C. Augier, F. T. Avignone, O. Azzolini, I. C. Bandac, A. S. Barabash, G. Bari, A. Barresi, D. … 展开作者
The CUPID Interest Group, A. Armatol, E. Armengaud, W. Armstrong, C. Augier, F. T. Avignone, O. Azzolini, I. C. Bandac, A. S. Barabash, G. Bari, A. Barresi, D. Baudin, F. Bellini, G. Benato, M. Beretta, L. Bergé, Ch. Bourgeois, M. Biassoni, J. Billard, V. Boldrini, A. Branca, C. Brofferio, C. Bucci, J. M. Calvo-Mozota, J. Camilleri, A. Candela, S. Capelli, L. Cappelli, L. Cardani, P. Carniti, N. Casali, A. Cazes, E. Celi, C. Chang, M. Chapellier, A. Charrier, D. Chiesa, M. Clemenza, I. Colantoni, F. Collamati, S. Copello, F. Cova, O. Cremonesi, R. J. Creswick, A. Cruciani, A. D'Addabbo, G. D'Imperio, I. Dafinei, F. A. Danevich, M. de Combarieu, M. De Deo, M. De Jesus, P. de Marcillac, S. Dell'Oro, S. Di Domizio, V. Dompe, A. Drobizhev, L. Dumoulin, G. Fantini, M. Fasoli, M. Faverzani, E. Ferri, F. Ferri, F. Ferroni, E. Figueroa-Feliciano, J. Formaggio, A. Franceschi, C. Fu, S. Fu, B. K. Fujikawa, J. Gascon, A. Giachero, L. Gironi, A. Giuliani, P. Gorla, C. Gotti, P. Gras, M. Gros, E. Guerard, T. D. Gutierrez, K. Han, E. V. Hansen, K. M. Heeger, D. L. Helis, H. Z. Huang, R. G. Huang, A. Ianni, L. Imbert, J. Johnston, A. Juillard, G. Karapetrov, G. Keppel, H. Khalife, V. V. Kobychev, Yu. G. Kolomensky, S. I. Konovalov, Y. Liu, P. Loaiza, L. Ma, M. Madhukuttan, F. Mancarella, R. Mariam, L. Marini, S. Marnieros, M. Martinez, R. H. Maruyama, B. Mauri, D. Mayer, Y. Mei, S. Milana, D. Misiak, T. Napolitano, M. Nastasi, X. -F. Navick, J. Nikkel, R. Nipoti, S. Nisi, C. Nones, E. B. Norman, V. Novosad, I. Nutini, T. O'Donnell, G. Olivier, E. Olivieri, C. Oriol, J. L. Ouellet, S. Pagan, C. Pagliarone, L. Pagnanini, P. Pari, L. Pattavina, B. Paul, M. Pavan, H. Peng, G. Pessina, V. Pettinacci, C. Pira, S. Pirro, D. V. Poda, T. Polakovic, O. G. Polischuk, S. Pozzi, E. Previtali, A. Puiu, A. Ressa, D. Reynet, R. Rizzoli, C. Rosenfeld, V. Sanglard, J. A. Scarpaci, B. Schmidt, V. Sharma, V. N. Shlegel, V. Singh, M. Sisti, D. Speller, P. T. Surukuchi, L. Taffarello, O. Tellier, C. Tomei, V. I. Tretyak, A. Tsymbaliuk, A. Vedda, M. Velazquez, K. J. Vetter, S. L. Wagaarachchi, G. Wang, L. Wang, B. Welliver, J. Wilson, K. Wilson, L. A. Winslow, M. Xue, L. Yan, J. Yang, V. Yefremenko, V. I. Yumatov, M. M. Zarytskyy, J. Zhang, A. S. Zolotarova, S. Zucchelli
A scintillating bolometer based on a large cubic Li$_{2}$$^{100}$MoO$_4$ crystal (45 mm side) and a Ge wafer (scintillation detector) has been operated in the CROSS cryogenic facility at the Canfranc underground laboratory in Spain. The dual-readout detector is a prototype of the technology that will be used in the next-generation $0\nu2β$ experiment CUPID. The measurements were performed at 18 and 12 mK temperature in a pulse tube dilution refrigerator. This setup utilizes the same technology as the CUORE cryostat that will host CUPID and so represents an accurate estimation of the expected performance. The Li$_{2}$$^{100}$MoO$_4$ bolometer shows a high energy resolution of 6 keV FWHM at the 2615 keV $γ$ line. The detection of scintillation light for each event triggered by the Li$_{2}$$^{100}$MoO$_4$ bolometer allowed for a full separation ($\sim$8$σ$) between $γ$($β$) and $α$ events above 2 MeV. The Li$_{2}$$^{100}$MoO$_4$ crystal also shows a high internal radiopurity with $^{228}$Th and $^{226}$Ra activities of less than 3 and 8 $μ$Bq/kg, respectively. Taking also into account the advantage of a more compact and massive detector array, which can be made of cubic-shaped crystals (compared to the cylindrical ones), this test demonstrates the great potential of cubic Li$_{2}$$^{100}$MoO$_4$ scintillating bolometers for high-sensitivity searches for the $^{100}$Mo $0\nu2β$ decay in CROSS and CUPID projects.
The CUPID-0 detector hosted at the Laboratori Nazionali del Gran Sasso, Italy, is the first large array of enriched scintillating cryogenic detectors for the investigation of $^{82}$Se neutrinoless double-beta decay (0$νββ$). CUPID-0 aims at measuring a background index in the region of interest (RoI) for 0$νββ$ at the level of 10$^{-3}$ c/keV/kg/y, the lowest value ever measured using cryogenic detectors. This result can be achieved by a state of the art technology for background suppression and thorough protocols and procedures for detector preparation and construction. In this paper, the di…
A scintillating bolometer technology based on $^{100}$Mo-enriched lithium molybdate (Li$_2$$^{100}$MoO$_4$) crystals has been developed by LUMINEU to search for neutrinoless double-beta ($0ν2β$) decay of $^{100}$Mo. The results of several low temperature tests at underground environments have proved the reproducibility of high detector performance and crystal radiopurity: in particular $\sim$5--6~keV FWHM energy resolution and at least 9$σ$ rejection of $α$'s in the vicinity of the $0ν2β$ decay of $^{100}$Mo (3034 keV) and below 10~$μ$Bq/kg bulk activity of $^{228}$Th and $^{226}$Ra. A modest …
A new R&D on lithium molybdate scintillators has begun within a project CLYMENE (Czochralski growth of Li$_2$MoO$_4$ crYstals for the scintillating boloMeters used in the rare EveNts sEarches). One of the main goals of the CLYMENE is a realization of a Li$_2$MoO$_4$ crystal growth line to be complementary to the one recently developed by LUMINEU in view of a mass production capacity for CUPID, a next-generation tonne-scale bolometric experiment to search for neutrinoless double-beta decay. In the present paper we report the investigation of performance and radiopurity of 158-g and 13.5-g scint…
CUPID-0 is the first large mass array of enriched Zn$^{82}$Se scintillating low temperature calorimeters, operated at LNGS since 2017. During its first scientific runs, CUPID-0 collected an exposure of 9.95 kg yr. Thanks to the excellent rejection of $α$ particles, we attained the lowest background ever measured with thermal detectors in the energy region where we search for the signature of $^{82}$Se neutrinoless double beta decay. In this work we develop a model to reconstruct the CUPID-0 background over the whole energy range of experimental data. We identify the background sources exploiti…
The CUPID-0 experiment searches for neutrinoless double beta decay ($0νββ$) using the first array of enriched Zn$^{82}$Se scintillating bolometers with double (heat and light) read-out. To further enhance the CUPID-0 detector performances, the heat-light correlation has been exploited to improve the energy resolution. Different decorrelation algorithms have been studied and the best result is the average reduction of the full width at half maximum (FWHM) energy resolution to $(90.5\pm0.6)~\%$ of its original value , corresponding to a change from $\text{FWHM}=(20.7\pm0.5)~\text{keV}$ to $\text…
CUPID is a next-generation neutrinoless double-beta decay experiment that will require cryogenic light detectors to improve background suppression, via the simultaneous readout of heat and light channels from its scintillating crystals. In this work we showcase light detectors based on a novel Ir-Pt bilayer transition edge sensor. We have performed a systematic study to improve the thermal coupling between the photon absorber and the sensor, and thereby its responsivity. Our first devices meet CUPID's baseline noise requirement of <100~eV rms. Our detectors have risetimes of $\sim$180 $μ$s and…
Lithium magnesium molybdate (Li$_2$Mg$_2$(MoO$_4$)$_3$) crystals were grown by the low-thermal-gradient Czochralski method. Luminescence properties of the material (emission spectra, thermally stimulated luminescence, dependence of intensity on temperature, phosphorescence) have been studied under X-Ray excitation in the temperature interval from 8 K to 400 K, while at the same being operated as a scintillating bolometer at 20 mK for the first time. We demonstrated that Li$_2$Mg$_2$(MoO$_4)_3$ crystals are a potentially promising detector material to search for neutrinoless double beta decay o…
For the first time, a cadmium tungstate crystal scintillator enriched in $^{116}$Cd has been succesfully tested as a scintillating bolometer. The measurement was performed above ground at a temperature of 18 mK. The crystal mass was 34.5 g and the enrichment level ~82 %. Despite a substantial pile-up effect due to above-ground operation, the detector demonstrated a high energy resolution (2-7 keV FWHM in 0.2-2.6 MeV $γ$ energy range), a powerful particle identification capability and a high level of internal radiopurity. These results prove that cadmium tungstate is an extremely promising dete…
Large lithium molybdate (Li$_2$MoO$_4$) crystal boules were produced by using the low thermal gradient Czochralski growth technique from deeply purified molybdenum. A small sample from one of the boules was preliminary characterized in terms of X-ray-induced and thermally-excited luminescence. A large cylindrical crystalline element (with a size of $\oslash 40\times40$ mm) was used to fabricate a scintillating bolometer, which was operated aboveground at $\sim 15$ mK by using a pulse-tube cryostat housing a high-power dilution refrigerator. The excellent detector performance in terms of energy…
The CUPID Collaboration is designing a tonne-scale, background-free detector to search for double beta decay with sufficient sensitivity to fully explore the parameter space corresponding to the inverted neutrino mass hierarchy scenario. One of the CUPID demonstrators, CUPID-Mo, has proved the potential of enriched Li$_{2}$$^{100}$MoO$_4$ crystals as suitable detectors for neutrinoless double beta decay search. In this work, we characterised cubic crystals that, compared to the cylindrical crystals used by CUPID-Mo, are more appealing for the construction of tightly packed arrays. We measured …
Random coincidences of nuclear events can be one of the main background sources in low-temperature calorimetric experiments looking for neutrinoless double-beta decay, especially in those searches based on scintillating bolometers embedding the promising double-beta candidate $^{100}$Mo, because of the relatively short half-life of the two-neutrino double-beta decay of this nucleus. We show in this work that randomly coinciding events of the two-neutrino double decay of $^{100}$Mo in enriched Li$_2$$^{100}$MoO$_4$ detectors can be effectively discriminated by pulse-shape analysis in the light …
The R&D activity performed during the last years proved the potential of ZnSe scintillating bolometers to the search for neutrino-less double beta decay, motivating the realization of the first large-mass experiment based on this technology: CUPID-0. The isotopic enrichment in $^{82}$Se, the Zn$^{82}$Se crystals growth, as well as the light detectors production have been accomplished, and the experiment is now in construction at Laboratori Nazionali del Gran Sasso (Italy). In this paper we present the results obtained testing the first three Zn$^{82}$Se crystals operated as scintillating bolom…
The LUMINEU project aims at performing a demonstrator underground experiment searching for the neutrinoless double beta decay of the isotope $^{100}$Mo embedded in zinc molybdate (ZnMoO$_4$) scintillating bolometers. In this context, a zinc molybdate crystal boule enriched in $^{100}$Mo to 99.5\% with a mass of 171 g was grown for the first time by the low-thermal-gradient Czochralski technique. The production cycle provided a high yield (the crystal boule mass was 84\% of initial charge) and an acceptable level -- around 4\% -- of irrecoverable losses of the costy enriched material. Two cryst…
This paper reports on the development of a technology involving $^{100}$Mo-enriched scintillating bolometers, compatible with the goals of CUPID, a proposed next-generation bolometric experiment to search for neutrinoless double-beta decay. Large mass ($\sim$1~kg), high optical quality, radiopure $^{100}$Mo-containing zinc and lithium molybdate crystals have been produced and used to develop high performance single detector modules based on 0.2--0.4~kg scintillating bolometers. In particular, the energy resolution of the lithium molybdate detectors near the $Q$-value of the double-beta transit…
Li$_2$$^{100\textrm{depl}}$MoO$_4$ Scintillating Bolometers for Rare-Event Search Experiments
National Research Centre Kurchatov Institute（库尔恰托夫国家研究中心研究所）；Nikolaev Institute of Inorganic Chemistry（尼古拉耶夫无机化学研究所）；Universidad Internacional de La Rioja（拉里奥哈国际大学）；INFN, Sezione di Milano Bicocca（意大利国家核物理研究院米兰比科卡分部）；INFN, Sezione di Roma（意大利国家核物理研究院罗马分部）；Institute for Nuclear Research of NASU（乌克兰国家科学院核物理研究所）；INFN Sezione di Roma Tor Vergata（意大利国家核物理研究院罗马托尔维尔加塔分部）；INFN, Laboratori Nazionali del Gran Sasso（意大利国家核物理研究院格兰萨索国家实验室）
The CUPID-Mo experiment is searching for neutrinoless double beta decay in $^{100}$Mo, evaluating the technology of cryogenic scintillating Li$_{2}^{100}$MoO$_4$ detectors for CUPID (CUORE Upgrade with Particle ID). CUPID-Mo detectors feature background suppression using a dual-readout scheme with Li$_{2}$MoO$_4$ crystals complemented by Ge bolometers for light detection. The detection of both heat and scintillation light signals allows the efficient discrimination of $α$ from $γ$&$β$ events. In this proceedings, we discuss results from the first 2 months of data taking in spring 2019. In addi…
CUPID-Mo is a cryogenic detector array designed to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. It uses 20 scintillating $^{100}$Mo-enriched Li$_2$MoO$_4$ bolometers instrumented with Ge light detectors to perform active suppression of $α$ backgrounds, drastically reducing the expected background in the $0νββ$ signal region. As a result, pileup events and small detector instabilities that mimic normal signals become non-negligible potential backgrounds. These types of events can in principle be eliminated based on their signal shapes, which are different from those of regu…
CUPID will be a next generation experiment searching for the neutrinoless double $β$ decay, whose discovery would establish the Majorana nature of the neutrino. Based on the experience achieved with the CUORE experiment, presently taking data at LNGS, CUPID aims to reach a background free environment by means of scintillating Li$_{2}$$^{100}$MoO$_4$ crystals coupled to light detectors. Indeed, the simultaneous heat and light detection allows us to reject the dominant background of $α$ particles, as proven by the CUPID-0 and CUPID-Mo demonstrators. In this work we present the results of the fir…
Molybdenum based crystals such as Li$_2$MoO$_4$ and CaMoO$_4$ are emerging as leading candidates for next generation experiments searching for neutrino-less double beta decay with cryogenic calorimeters (CUPID, AMoRE). The exquisite energy resolution and high radio-purity of these crystals come at the cost of a potentially detrimental background source: the two neutrinos double beta decay of $^{100}$Mo. Indeed, the fast half-life of this decay mode, combined with the slow response of cryogenic calorimeters, would result in pile-up events in the energy region of interest for neutrino-less doubl…
The technology of scintillating bolometers based on zinc molybdate (ZnMoO$_4$) crystals is under development within the LUMINEU project to search for 0$ν$2$β$ decay of $^{100}$Mo with the goal to set the basis for large scale experiments capable to explore the inverted hierarchy region of the neutrino mass pattern. Advanced ZnMoO$_4$ crystal scintillators with mass of $\sim$~0.3 kg were developed and Zn$^{100}$MoO$_4$ crystal from enriched $^{100}$Mo was produced for the first time by using the low-thermal-gradient Czochralski technique. One ZnMoO$_4$ scintillator and two samples (59 g and 63 …
CUPID-Mo is a bolometric experiment to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. In this article, we detail the CUPID-Mo detector concept, assembly, installation in the underground laboratory in Modane in 2018, and provide results from the first datasets. The demonstrator consists of an array of 20 scintillating bolometers comprised of $^{100}$Mo-enriched 0.2 kg Li$_2$MoO$_4$ crystals. The detectors are complemented by 20 thin cryogenic Ge bolometers acting as light detectors to distinguish $α$ from $γ$/$β$ events by the detection of both heat and scintillation light si…
Searching for neutrinoless double-beta decay (0$ν$2$β$) is one of the main experimental challenges of modern physics. One experimental technique is given by cryogenic detectors named bolometers that are really promising for this purpose. The current generation tonne-scale experiment CUORE using this technology is putting the best limit on $^{130}$Te 0$ν$2$β$ half-life with TeO$_2$ crystals but its sensitivity is limited by its background. Therefore, it will be followed by the next generation experiment CUPID (CUORE Upgrade with Particle IDentification) that will study $^{100}$Mo embedded insid…
We have developed and tested a new way of coupling bolometric light detectors to scintillating crystal bolometers based upon simply resting the light detector on the crystal surface, held in position only by gravity. This straightforward mounting results in three important improvements: (1) it decreases the amount of non-active materials needed to assemble the detector, (2) it substantially increases the light collection efficiency by minimizing the light losses induced by the mounting structure, and (3) it enhances the thermal signal induced in the light detector thanks to the extremely weak …
Test of $^{116}$CdWO$_4$ and Li$_2$MoO$_4$ scintillating bolometers in the CROSS underground facility with upgraded detector suspension
Univ. Grenoble Alpes, CNRS, Grenoble INP (Institute of Engineering Univ. Grenoble Alpes), SIMAP（格勒诺布尔阿尔卑斯大学、法国国家科学研究中心、格勒诺布尔理工学院（格勒诺布尔大学工程学院）、SIMAP）；National Research Center Kurchatov Institute, Kurchatov Complex of Theoretical and Experimental Physics（库尔恰托夫研究所国家研究中心、理论与实验物理库尔恰托夫综合体）；Institute for Nuclear Research of NASU（乌克兰国家科学院核物理研究所）；INFN Laboratori Nazionali del Gran Sasso（意大利国家核物理研究院格兰萨索国家实验室）；Gran Sasso Science Institute（格兰萨索科学研究所）
AMoRE is an international project to search for the neutrinoless double beta decay of $^{100}$Mo using a detection technology consisting of magnetic microcalorimeters (MMCs) and molybdenum-based scintillating crystals. Data collection has begun for the current AMORE-I phase of the project, an upgrade from the previous pilot phase. AMoRE-I employs thirteen $^\mathrm{48depl.}$Ca$^{100}$MoO$_4$ crystals and five Li$_2$$^{100}$MoO$_4$ crystals for a total crystal mass of 6.2 kg. Each detector module contains a scintillating crystal with two MMC channels for heat and light detection. We report the …
Cryogenic light detectors with thermal signal amplification for $0νββ$ search experiments
Institut de Physique des 2 Infinis（双无穷大物理研究所）；IRFU, CEA, Université Paris-Saclay（巴黎萨克雷大学CEA IRFU）；National Research Center Kurchatov Institute（库尔恰托夫国家研究中心）；University of Milano-Bicocca（米兰比可卡大学）；INFN Sezione di Milano-Bicocca（意大利国家核物理研究所米兰比可卡分部）；University of California, Berkeley（加州大学伯克利分校）；Université Paris-Saclay, CNRS/IN2P3, IJCLab（巴黎萨克雷大学CNRS/IN2P3 IJCLab）；Laboratorio Subterráneo de Canfranc（坎弗兰克地下实验室）；Escuela Superior de Ingeniería y Tecnología, Universidad Internacional de La Rioja（拉里奥哈国际大学高等工程与技术学院）；Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）；Physik-Institut, University of Zürich（苏黎世大学物理研究所）
ZnMoO$_4$ scintillators with a mass of $\sim$ 0.3 kg, as well as Zn$^{100}$MoO$_4$ crystals enriched in the isotope $^{100}$Mo were produced for the first time by using the low-thermal-gradient Czochralski technique. The optical and luminescent properties of the produced crystals were studied to estimate the progress in crystal growth quality. The low-temperature tests with a 313 g ZnMoO$_4$ and two enriched Zn$^{100}$MoO$_4$ crystals were performed aboveground in the Centre de Sciences Nucléaires et de Sciences de la Matière. The low background measurements with a three ZnMoO$_4$ and two enri…
The AMoRE (Advanced Mo-based Rare process Experiment) project is a series of experiments that use advanced cryogenic techniques to search for the neutrinoless double-beta decay of \mohundred. The work is being carried out by an international collaboration of researchers from eight countries. These searches involve high precision measurements of radiation-induced temperature changes and scintillation light produced in ultra-pure \Mo[100]-enriched and \Ca[48]-depleted calcium molybdate ($\mathrm{^{48depl}Ca^{100}MoO_4}$) crystals that are located in a deep underground laboratory in Korea. The \m…
