The question of classicality is addressed in relation with the shape of the nuclear skeleton of molecular systems. As the most natural environment, the electrons of the molecule are considered as continuously monitoring agents for the nuclei. For this picture, an elementary formalism of decoherence theory is developed and numerical results are presented for few-particle systems. The numerical examples suggest that the electron-nucleus Coulomb interaction is sufficient for inducing a blurred shape with strong quantum coherences in compounds of the lightest elements, H$_2$, D$_2$, T$_2$, and HeH$^+$.
Motivated by trapping and cooling experiments with non-spherical nanoparticles, we discuss how their combined rotational and translational quantum state is affected by the interaction with a gaseous environment. Based on the quantum master equation in terms of orientation-dependent scattering amplitudes, we evaluate the localization rate for gas collisions off an anisotropic van der Waals-type potential and for photon scattering off an anisotropic dielectric. We also show how pure angular momentum diffusion arises from these open quantum dynamics in the limit of weak anisotropies.
The quantum state of motion of a large and rotating polar molecule can lose coherence through the collisions with gas atoms. We show how the associated quantum master equation for the center of mass can be expressed in terms of the orientationally averaged differential and total scattering cross sections, for which we provide approximate analytic expressions. The master equation is then utilized to quantify collisional decoherence in a interference experiment with polar molecules.
It has been claimed that decoherence of open quantum systems explains the tendency of macroscopic systems to exhibit quasiclassical behavior. We show that quasiclassicality is in fact an unremarkable property, characterizing generic subsystems of environments even in the absence of dynamical decoherence. It is suggested that decoherence is best regarded as explaining the persistence of true classicality, rather than the emergence, rather than the emergence of quasiclassicality.
We investigate the influence of environmental noise on polarization entangled light generated by parametric emission in a cavity. By adopting a recently developed separability criterion, we show that: i) self-stimulation may suppress the detrimental influence of noise on entanglement; ii) when self-stimulation becomes effective, a classical model of parametric emission incorporating noise provides the same results of quantum theory for the expectation values involved in the separability criterion. Moreover we show that, in the macroscopic limit, it is impossible to observe violations of local …
We consider the claim that decoherence explains the emergence of classicality in quantum systems, and conclude that it does not. We show that, given a randomly chosen universe composed of a variety of subsystems, some of which are macroscopic and subject to decoherence-inducing interactions, and some of which are microscopic, the macroscopic subsystems will not display any distinctively classical behavior. Therefore, a universe in which macroscopic and microscopic do display distinct behavior must be in a very special, highly nongeneric quantum state.
Maximally predictive states, as defined in recent work by Zurek, Habib and Paz, are studied for more elaborate environment models than a linear coupling. An environment model which includes spatial correlations in the noise is considered in the non-dissipative regime. The Caldeira-Leggett model is also reconsidered in the context of an averaging procedure which produces a completely positive form for the quantum master equation. In both cases, the maximally predictive states for the harmonic oscillator are the coherent states, which is the same result found by Zurek,Habib and Paz for the Calde…
In this article I aim to provide an intuitive and non-technical introduction to decoherence and quantum Darwinism. Together these theories explain how our classical reality emerges from an underlying quantum mechanical description. Here I focus on two aspects of this and explain, firstly, how decoherence can tell us why we never see macroscopic superpositions, such as dead-and-alive cats, in our classical surroundings; and secondly I describe and then provide a resolution to the so-called preferred basis problem. I then introduce recent results demonstrating that certain aspects of classicalit…
Zurek, Habib and Paz [W. H. Zurek, S. Habib and J. P. Paz, Phys. Rev. Lett. {\bf 70} (1993)\ 1187] have characterized the set of states of maximal stability defined as the set of states having minimum entropy increase due to interaction with an environment, and shown that coherent states are maximal for the particular environment model examined. To generalize these results, I consider entropy production within the Lindblad theory of open systems, treating environment effects perturbatively. I characterize the maximally predicitive states which emerge from several forms of effective dynamics, i…
Decoherence shows how the openness of quantum systems -- interaction with their environment -- suppresses flagrant manifestations of quantumness. Einselection accounts for the emergence of preferred quasi-classical pointer states. Quantum Darwinism goes beyond decoherence. It posits that the information acquired by the monitoring environment responsible for decoherence is disseminated, in many copies, in the environment, and thus becomes accessible to observers. This indirect nature of the acquisition of information by observers who use the environment as a communication channel is the mechani…
In this study, we apply the monitoring master equation describing decoherence of internal states to an optically active molecule prepared in a coherent superposition of nondegenerate internal states interacting with thermal photons at low temperatures. We use vibrational Raman scattering theory up to the first chiral-sensitive contribution, i.e., the mixed electric-magnetic interaction, to obtain scattering amplitudes in terms of molecular polarizability tensors. The resulting density matrix is used to obtain elastic decoherence rates.
Superselection rules induced by the interaction with the environment are a basis to understand the emergence of classical observables within quantum theory. The aim of this article is to investigate the decoherence effects, which lead to superselection sectors, with the help of exactly soluble Hamiltonian models. Starting from the examples of Araki and of Zurek more general models with scattering are presented for which the projection operators onto the induced superselection sectors do no longer commute with the Hamiltonian. The example of an environment given by a free quantum field indicate…
Macroscopic systems are described most completely by local densities (particle number, momentum and energy) yet the superposition states of such physical variables, indicated by the Everett interpretation, are not observed. In order to explain this, it is argued that histories of local number, momentum and energy density are approximately decoherent when coarse-grained over sufficiently large volumes. Decoherence arises directly from the proximity of these variables to exactly conserved quantities (which are exactly decoherent), and not from environmentally-induced decoherence. We discuss the …
Decoherence of a quantum state coupled to an exterior environment is at the foundation of our understanding of the emergence of classical behavior from the quantum world, but how does it emerge in a finite closed quantum system? Here this is studied by modeling an isolated quantum system of a handful of ultracold atoms confined to a double well potential and coupled to a single atom of a different type. The ultracold atoms thermalize and serve as an environmental bath for the single atom. We observe accelerated decoherence of the single atom when ultracold atoms have thermalized. This is expla…
The idea that decoherence in a unitary-only quantum theory suffices to explain emergence of classical phenomena has been shown in the peer-reviewed literature to be seriously flawed due to circularity. However, claims continue to be made that this approach, also known as "Quantum Darwinism," is the correct way to understand classical emergence. This Letter reviews the basic problem and points out an additional logical flaw in the argument. It is concluded that the "Quantum Darwinism" program fails.
We use a master equation to study the dynamics of two coupled macroscopic quantum systems (e.g.\ a Josephson junction made of two Bose-Einstein condensates or two spin states of an ensemble of trapped ions) subject to a weak continuous measurement. If the coupling between the two systems is suddenly switched on the resulting dynamics leads to caustics (fold and cusp catastrophes) in the number-difference probability distribution, and at the same time the measurement gradually induces a quantum-to-classical transition. Decoherence is often invoked to help resolve paradoxes associated with macro…
Practical implementations of quantum technology are limited by unavoidable effects of decoherence and dissipation. With achieved experimental control for individual atoms and photons, more complex platforms composed by several units can be assembled enabling distinctive forms of dissipation and decoherence, in independent heat baths or collectively into a common bath, with dramatic consequences for the preservation of quantum coherence. The cross-over between these two regimes has been widely attributed in the literature to the system units being farther apart than the bath's correlation lengt…
We study the emergence and dynamics of pointer states in the motion of a quantum test particle affected by collisional decoherence. These environmentally distinguished states are shown to be exponentially localized solitonic wave functions which evolve according to the classical equations of motion. We explain their formation using the orthogonal unraveling of the master equation, and we demonstrate that the statistical weights of the arising mixture are given by projections of the initial state onto the pointer basis.
We have studied the emergence of classical states in the perturbative interaction model. The states which interact with many other degrees of freedom, such as the center of mass of a macro-object, play important role. Although the random phase mechanism is effective as same as Zurek's strong correlation model, there are enormous states, each of which independently developes due to the orthogonality of the environmental states. In these privileged states, the subsystem picture with the separability is stable.
The inherent difficulty in talking about quantum decoherence in the context of quantum cosmology is that decoherence requires subsystems, and cosmology is the study of the whole Universe. Consistent histories gave a possible answer to this conundrum, by phrasing decoherence as loss of interference between alternative histories of closed systems. When one can apply Boolean logic to a set of histories, it is deemed 'consistent'. However, the vast majority of the sets of histories that are merely consistent are blatantly nonclassical in other respects, and further constraints than just consistenc…
We give a pedagogical introduction to the process of decoherence - the irreversible emergence of classical properties through interaction with the environment. After discussing the general concepts, we present the following examples: Localisation of objects, quantum Zeno effect, classicality of fields and charges in QED, and decoherence in gravity theory. We finally emphasise the important interpretational features of decoherence.
A recent debate has ensued over the claim by Pikovski et al. [Nat. Phys. 11, 668 (2015)] that systems with internal degrees of freedom undergo a universal, gravity-induced, type of decoherence that explains their quantum-to-classical transition. This decoherence is supposed to arise from the different gravitational redshifts experienced by such systems when placed in a superposition of two wave packets at different heights in a gravitational field. Here we investigate some aspects of the discussion with the aid of simple examples. In particular, we first resolve an apparent conflict between th…
We give a short, critical review of the issue of decoherence. We establish the most general framework in which decoherence can be discussed, how it can be quantified and how it can be measured. We focus on environment induced decoherence and its degree of usefulness for the interpretation of quantum theory. We finally discuss the emergence of a classical world. An overall emphasis is given in pointing at common fallacies and misconceptions.
Niels Bohr famously insisted on the indispensability of what he termed "classical concepts." In the context of the decoherence program, on the other hand, it has become fashionable to talk about the "dynamical emergence of classicality" from the quantum formalism alone. Does this mean that decoherence challenges Bohr's dictum -- for example, that classical concepts do not need to be assumed but can be derived? In this paper, we'll try to shed some light down the murky waters where formalism and philosophy mingle. To begin, we'll clarify the notion of classicality in the decoherence description…
Can the computational complexity theory of computer science and mathematics say something new about unresolved problems in quantum physics? Particularly, can the P versus NP question in the computational complexity theory be a factor in the elucidation of the emergency of classicality in quantum mechanics? The paper compares two different ways of deriving classicality from the quantum formalism resulted from two differing hypotheses regarding the P versus NP question -- the approach of the quantum decoherence theory implying that P = NP and the computational complexity approach which assumes t…
We study the role of the information deposited in the environment of an open quantum system in course of the decoherence process. Redundant spreading of information -- the fact that some observables of the system can be independently ``read-off'' from many distinct fragments of the environment -- is investigated as the key to effective objectivity, the essential ingredient of ``classical reality''. This focus on the environment as a communication channel through which observers learn about physical systems underscores importance of quantum Darwinism -- selective proliferation of information ab…
We show that the pointer basis distinguished by collisional decoherence consists of exponentially localized, solitonic wave packets. Based on the orthogonal unraveling of the quantum master equation, we characterize their formation and dynamics, and we demonstrate that the statistical weights arising from an initial superposition state are given by the required projection. Since the spatial width of the pointer states can be obtained by accounting for the gas environment in a microscopically realistic fashion, one may thus calculate the coherence length of a strongly interacting gas.
Emergence of classicality from quantum mechanics, a hotly debated topic, has had no satisfactory resolution so far. Various approaches including decoherence and gravitational interactions have been suggested. In the present work, the Schrödinger-Newton model is used to study the role of semi-classical self-gravity in the evolution of massive spin-1/2 particles in a Stern-Gerlach experiment. For small mass, evolution of the initial wavepacket in a spin superposition shows a splitting in the magnetic field gradient into two trajectories as in the standard Stern-Gerlach experiment. For larger mas…
Entanglement within a given device provides a potential resource for quantum information processing. Entanglement between system and environment leads to decoherence (thus suppressing non-classical features within the system) but also opens up a route to robust and universal control. The latter is related to thermodynamic equilibrium, a generic behavior of bi-partite quantum systems. Fingerprints of this equilibrium behavior (including relaxation and stability) show up already far from the thermodynamic limit, where a complete solution of the underlying Schroedinger dynamics of the total syste…
The interaction of quantum emitters with one-dimensional photon-like reservoirs induces strong and long-range dissipative couplings that give rise to the emergence of so-called Decoherence Free Subspaces (DFS) which are decoupled from dissipation. When introducing weak perturbations on the emitters, e.g., driving, the strong collective dissipation enforces an effective coherent evolution within the DFS. In this work, we show explicitly how by introducing single-site resolved drivings, we can use the effective dynamics within the DFS to design a universal set of one and two-qubit gates within t…
The Diosi-Penrose model of quantum-classical boundary postulates gravity-related spontaneous wave function collapse of massive degrees of freedom. The decoherence effects of the collapses are in principle detectable if not masked by the overwhelming environmental decoherence. But the DP (or any other, like GRW, CSL) spontaneous collapses are not detectable themselves, they are merely the redundant formalism of spontaneous decoherence. To let DP collapses become testable physics, recently we extended the DP model and proposed that DP collapses are responsible for the emergence of the Newton gra…
It is now widely accepted that environmental entanglement and the resulting decoherence processes play a crucial role in the quantum-to-classical transition and the emergence of "classicality" from quantum mechanics. To this extent, decoherence is often understood as signifying a break with the Copenhagen interpretation, and in particular with Bohr's view of the indispensability of classical concepts. This paper analyzes the relationship between Bohr's understanding of the quantum-classical divide and his doctrine of classical concepts and the decoherence-based program of emergent classicality…
We study the process of observation (measurement), within the framework of a `perspectival' (`relational', `relative state') version of the modal interpretation of quantum mechanics. We show that if we assume certain features of discreteness and determinism in the operation of the measuring device (which could be a part of the observer's nerve system), this gives rise to classical characteristics of the observed properties, in the first place to spatial localization. We investigate to what extent semi-classical behavior of the object system itself (as opposed to the observational system) is ne…
An example is presented when decoherence and quantum interference gives rise to narrow eigenstates (in coordinate representation) for the reduced density matrix of macroscopic quantum systems. On the basis of modal interpretations this means the emergence of classical properties.
In a series of comments, Bonder et al. criticized our work on decoherence due to time dilation [Nature Physics 11, 668-672 (2015)]. First the authors erroneously claimed that our results contradict the equivalence principle, only to "resolve" the alleged conflict in a second note. The resolution - relativity of simultaneity - was already explained in our reply [arXiv:1508.03296], which Bonder et al. now essentially reiterate. The newly raised points were also already extensively clarified in our note. The physical prediction of our work remains valid: systems with internal dynamics decohere if…
Wave-particle duality is an essential character of quantum systems. In the last few years, much progress has being made towards formally quantifying these quantum features. The properties of the quantum density matrix were shown to lead to duality inequalities for single-quanton mixed states and to triality identities, also known as complete complementarity relations (CCRs), for two-quanton pure states. In this article, we establish connections between CCRs and EPR (ir)realism, as formalized by Bilobran and Angelo in [Europhys. Lett. 112, 40005 (2015)]. Besides, we show that, for tripartite pu…
We clarify the way in which cosmological perturbations of quantum origin, produced during inflation, assume classical properties. Two features play an important role in this process: First, the dynamics of fluctuations which are presently on large cosmological scales leads to a very peculiar state (highly squeezed) that is indistinguishable, in a precise sense, from a classical stochastic process. This holds for almost all initial quantum states. Second, the process of decoherence by interaction with the environment distinguishes the field amplitude basis as a robust pointer basis. We discuss …
The origin of classical reality in our quantum world is a long-standing mystery. Here, we examine a nitrogen vacancy center evolving naturally in the presence of its environment to study quantum Darwinism - the proliferation of information about preferred quantum states throughout the world via the environment. This redundantly imprinted information accounts for the perception of objective reality, as it is independently accessible by many without perturbing the system of interest. To observe the emergence of redundant information, we implement a novel dynamical decoupling scheme that enables …
We explore the interplay between tunneling process and chiral interactions in the discrimination of chiral states for an ensemble of molecules in a biological environment. Each molecule is described by an asymmetric double-well potential and the environment is modeled as a bath of harmonic oscillators. We carefully analyze different time-scales appearing in the resulting master equation at both weak- and strong-coupling limits. The corresponding results are accompanied by a set of coupled differential equations characterizing optical activity of the molecules. We show that, at the weak-couplin…
Two-electron quantum walks can probe entanglement and decoherence in an electron microscope
Solid State Institute, Technion – Israel Institute of Technology（固体研究所，以色列理工学院）；Fachbereich Physik, Universität Konstanz（康斯坦茨大学物理系）；E. L. Ginzton Laboratories, Stanford University（斯坦福大学Ginz顿实验室）
This review summarizes and amplifies on recent investigations of coupled quantum dynamical systems in the short wavelength limit. We formulate and attempt to answer three fundamental questions: (i) What drives a dynamical quantum system to behave classically ? (ii) What determines the rate at which two coupled quantum--mechanical systems become entangled ? (iii) How does irreversibility occur in quantum systems with few degrees of freedom ? We embed these three questions in the broader context of the quantum--classical correspondence, which motivates the use of short--wavelength approximations…
