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arXiv 2008.11124cond-mat.mes-hall
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高相干电子脉冲探测的结构动力学

Structural dynamics probed by high-coherence electron pulses

Armin Feist, Gero Storeck, Sascha Schäfer, Claus Ropers

摘要:

超快测量技术为我们对固体和纳米结构的性质和功能的微观理解做出了重要贡献。基于X射线和电子的短脉冲的方法提供了具有不断增长的空间和时间分辨率的原子级前景。时间分辨电子衍射和显微镜是研究激发态物质非平衡结构动力学的最有力的方法之一。在这篇文章中,我们讨论了在超快电子成像的脉冲电子束的相干性显着改善启用的最新进展。具体而言,我们回顾了超快低能电子衍射(ULEED)的发展和首次应用于表面结构动力学的研究,并讨论了激光触发场发射源促进超快透射电子显微镜(UTEM)的新机会。这些和进一步的发展将使相干电子束成为未来超快纳米成像的重要组成部分。

英文摘要:

Ultrafast measurement technology provides essential contributions to our microscopic understanding of the properties and functions of solids and nanostructures. Atomic-scale vistas with ever-growing spatial and temporal resolution are offered by methods based on short pulses of x-rays and electrons. Time-resolved electron diffraction and microscopy are among the most powerful approaches to investigate non-equilibrium structural dynamics in excited matter. In this article, we discuss recent advances in ultrafast electron imaging enabled by significant improvements in the coherence of pulsed electron beams. Specifically, we review the development and first application of Ultrafast Low-Energy Electron Diffraction (ULEED) for the study of structural dynamics at surfaces, and discuss novel opportunities of Ultrafast Transmission Electron Microscopy (UTEM) facilitated by laser-triggered field emission sources. These and further developments will render coherent electron beams an essential component in the future of ultrafast nanoscale imaging.

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