In this article, we introduce a quantum key distribution protocol for the line of sight channels based on coincidence measurements. We present a proof-of-concept implementation of our protocol. We show that using coincidence measurements to monitor multi-photon pulses results in a higher secure key rate over longer distances for such channels. This key rate is higher than popular implementations of quantum key distribution protocol based on BB84, for example, the GLLP analysis [Quant. Info. Comput. \textbf{4}, 325 (2004)]. In the experiment, we could generate around $74 \%$ more key bits per signal pulse as compared to the GLLP analysis of BB84 protocol with similar parameters and equal value of mean photon number.
The technological possibilities of a realistic eavesdropper are discussed. Two eavesdropping strategies taking profit of multiphoton pulses in faint laser QKD are presented. We conclude that, as long as storage of Qubits is technically impossible, faint laser QKD is not limited by this security issue, but mostly by the detector noise.
We derive a generalized master equation for multiphoton pulses interacting with multiple emitters in a waveguide-quantum electrodynamics system where the emitter frequency can be modulated and the effects of non-guided modes can also be considered. Based on this theory, we can calculate the real-time dynamics of an array of interacting emitters driven by an incident photon pulse which can be vacuum, a coherent state, a Fock state or their superpositions. Moreover, we also derive generalized input-output relations to calculate the reflectivity and transmissivity of this system. We can also calc…
The dynamics of waveguide-QED systems involving coherent time-delayed feedback give rise to a hierarchy of multi-time correlations within the Heisenberg picture due to the induced non-Markovianity. We propose to perform a projection onto a complete set of states in the Hilbert space to decompose the multi-time correlations into single-time matrix elements. To illustrate the procedure, we consider the paradigmatic example of a two-level system that couples to a semi-infinite waveguide and interacts with quantum light pulses. Our approach complements the range of available methods as it allows c…
Within the matrix product state framework, we study the non-Markovian feedback dynamics of a two-level system interacting with the electromagnetic field inside a semi-infinite waveguide where the excitation of an atom-photon bound state is possible. Taking the steady-state excitation of the emitter as a figure of merit, we compare the trapped excitation for an initially excited quantum emitter and an emitter prepared via quantized pulses containing up to four photons. In the latter case, we find that for large feedback delay times, multi-photon pulses can yield a significantly higher steady-st…
Mistrustful cryptography includes important tasks like bit commitment, oblivious transfer, coin flipping, secure computations, position authentication, digital signatures and secure unforgeable tokens. Practical quantum implementations presently use photonic setups. In many such implementations, Alice sends photon pulses encoding quantum states and Bob chooses measurements on these states. In practice, Bob generally uses single photon threshold detectors, which cannot distinguish the number of photons in detected pulses. Also, losses and other imperfections require Bob to report the detected p…
We investigate the electron-positron pair production process in an oscillating field with modulated amplitude in quantum kinetic formalism. By comparing the number density in field with and without modulation, we find that the pair production rate can be enhanced by several orders when the photon energy just reach the threshold with the help of shifted frequency due to modulation. We also detect the same effect in a pulse train with subcycle structure. We demonstrate that the frequency threshold can be lowered by frequency of pulse-train due to modulation effect. We also find that the momentum…
We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate virtual states are absent within our laser pulse timescales. Under these conditions, the multiphoton results are similar to the single photon and that it is possible to extend the single photon coherent control ideas to develop multiphoton coherent control.
The light propagation of a probe field pulse in a four-level double-lambda type system driven by laser fields that form a closed interaction loop is studied. Due to the finite frequency width of the probe pulse, a time-independent analysis relying on the multiphoton resonance assumption is insufficient. Thus we apply a Floquet decomposition of the equations of motion to solve the time-dependent problem beyond the multiphoton resonance condition. We find that the various Floquet components can be interpreted in terms of different scattering processes, and that the medium response oscillating in…
This Letter demonstrates control over multiphoton absorption processes in driven two-level systems, which include for example superconducting qubits or laser-irradiated graphene, through spectral shaping of the driving pulse. Starting from calculations based on Floquet theory, we use differential evolution, a general purpose optimization algorithm, to find the Fourier coefficients of the driving function that suppress a given multiphoton resonance in the strong field-regime. We show that the suppression of the transition probability is due to the coherent superposition of high-order Fourier ha…
We present an experimental demonstration of a modified version of the entanglement-assisted "Guess my Number" protocol for the reduction of communication complexity among three separated parties. The results of experimental measurements imply that the separated parties can compute a function of distributed inputs by exchanging less classical information than by using any classical strategy. And the results also demonstrate the advantages of entanglement-enhanced communication, which is very close to quantum communication. The advantages are based on the properties of Greenberger-Horne-Zeilinge…
In this paper, a photon-number-resolving decoy state quantum key distribution scheme is presented based on recent experimental advancements. A new upper bound on the fraction of counts caused by multiphoton pulses is given. This upper bound is independent of intensity of the decoy source, so that both the signal pulses and the decoy pulses can be used to generate the raw key after verified the security of the communication. This upper bound is also the lower bound on the fraction of counts caused by multiphoton pulses as long as faint coherent sources and high lossy channels are used. We show …
The generation of quantum entangled states of many particles is a central goal of quantum information science. Characterizing such states is a complex task that demands exponentially large resources as particles are being added. Previously, we demonstrated a resource efficient source that can generate, in principal, entanglement between any number of photons. This source recursively fuse photon pairs generated by a pulsed laser into a multiphoton entangled state. In the current work, we perform quantum state tomography on the photon pair source and quantum process tomography on the fusion oper…
It is the first scheme which allows the detection apparatus to achieve both the photon number of arriving signals and quantum bit error rate of the multiphoton pulses precisely. We show that the upper bound of the fraction of the tagged multiphoton pulses counts is $μ$, which is independent of the channel loss and the intensity of the decoy source. Such upper bound is $inherent$ and cannot be reduced any longer as long as the weak coherent scouces and high lossy channel are used. We show that our scheme can be implemented even if the channel loss is very high. A stronger intensity of the pulse…
We present a multichannel photoelectron interferometry technique based on trichromatic pulse shaping for unambiguous determination of quantum phases in multiphoton ionization (MPI) of potassium atoms. The colors of the laser field are chosen to produce three energetically separated photoelectron interferograms in the continuum. While the red pulse is two-photon resonant with the $3d$-state resulting in a (2+1) resonance-enhanced MPI (REMPI), a (1+2) REMPI occurs via the non-resonant intermediate $4p$-state with an initial green or blue pulse. We show that ionization via a non-resonant intermed…
Two-color multiphoton emission from polycrystalline tungsten nanotips has been demonstrated using two-color laser fields. The two-color photoemission is assisted by a three-photon multicolor quantum channel, which leads to a twofold increase in quantum efficiency. Weak-field control of two-color multiphoton emission was achieved by changing the efficiency of the quantum channel with pulse delay. The result of this study complements two-color tunneling photoemission in strong fields, and has potential applications for nanowire-based photonic devices. Moreover, the demonstrated two-color multiph…
The multiphoton Jaynes-Cummings model is investigated and applications in quantum information science are explored. Considering the strong atom-field coupling regime and an $N$-photon interaction, a nonlinear driving field can perform an arbitrary rotation in the Fock space of the cavity mode involving the vacuum and an $M$-Fock state, with $M<N$. Besides, driving the cavity mode with a linear coherent field (superposition of many Fock states), only the cavity states within the Fock subspace {$|0\rangle,|1\rangle,..., |N-1\rangle$} can be populated, i.e., we show how to implement a Fock state …
We propose a Bell measurement scheme by employing a logical qubit in Greenberger-Horne-Zeilinger (GHZ) entanglement with an arbitrary number of photons. Remarkably, the success probability of the Bell measurement as well as teleportation of the GHZ entanglement can be made arbitrarily high using only linear optics elements and photon on-off measurements as the number of photons increases. Our scheme outperforms previous proposals using single photon qubits when comparing the success probabilities in terms of the average photon usages. It has another important advantage for experimental feasibi…
We explore applications of nonlinear circuit QED with a charge qubit inductively coupled to a microwave LC resonator in the photonic engineering and ultrastrong-coupling multiphoton quantum optics. Simply sweeping the gate-voltage bias achieves arbitrary Fock-state pulsed maser, where the single qubit plays the role of artificial gain medium. Resonantly pumping the parametric qubit-resonator interface leads to the squeezing of resonator field, which is utilizable to the quantum-limited microwave amplification. Moreover, upwards and downwards multiphoton quantum jumps may be observed in the ste…
The existing decoy-state quantum key distribution (QKD) beating photon-number-splitting (PNS) attack provides a more accurate method to estimate secure key rate, while it still considers that only single-photon pulses can generate secure keys in any case. However, multiphoton pulses can also generate secure keys if we can confirm that there is no attack. In this paper, under the null hypothesis of no PNS attack, we first determine whether there is an attack or not by retrieving the missing information of the existing decoy-state protocols, extract a Cauchy distribution statistic, and further p…
A bipartite multiphoton entangled state is created through stimulated parametric down-conversion of strong laser pulses in a nonlinear crystal. It is shown how detectors that do not resolve photon number can be used to analyze such multiphoton states. Entanglement of up to 12 photons is detected using both the positivity of the partially transposed density matrix and a newly derived criteria. Furthermore, evidence is provided for entanglement of up to 100 photons. The multi-particle quantum state is such that even in the case of an overall photon collection and detection efficiency as low as a…
Multiphoton detachment of F$^-$ by strong few-cycle laser pulses was studied by Shearer and Monteith using a Keldysh-type approach [Phys. Rev. A 88, 033415 (2013)]. We believe that this work contained errors in the calculation of the detachment amplitude and photoelectron spectra. We describe the necessary corrections to the theory and show that the results, in particular, the interference features of the photoelectron spectra, appear noticeably different.
A typical structure of an auto-compensation system for quantum key distribution is given. The principle of operation of a fiber-optic system for the distribution of quantum keys with phase coding of photon states is described. The operation of the system in the synchronization mode and the formation of quantum keys was investigated. The process of detecting a time interval with an optical synchronization pulse is analyzed. The structural scheme of the experimental stand of the quantum-cryptographic network is given. Data are obtained that attest to the presence of a multiphoton signal during t…
The measurement of the tunneling time in attosecond experiments, termed attoclock, triggered a hot debate about the tunneling time, the role of time in quantum mechanics, where the interaction with the laser pulse involves two regimes of a different character, the multiphoton and the tunneling (field-) ionization. In the adiabatic field calibration, one of us (O. K.) developed in earlier works a real tunneling time model and showed that the model fits well to the experimental data of Landsmann et al. (Optica {\bf 1}, 343 2014). In the present work, it is shown that the model explains the exper…
Two-photon excitation (TPE) proceeds via a "virtual" pathway, which depends on the accessibility of one or more intermediate states, and, in the case of non-centrosymmetric molecules, an additional "dipole" pathway involving the off-resonance dipole-allowed one-photon transitions and the change in the permanent dipole moment between the initial and final states. Here, we control the quantum interference between these two optical excitation pathways by using phase-shaped femtosecond laser pulses. We find enhancements by a factor of up to 1.75 in the two-photon-excited fluorescence of the photob…
We present a detailed analysis of the Bell measurement scheme proposed in [Phys. Rev. Lett. 114, 113603 (2015)] based on a logical qubit using Greenberger-Horne-Zeilinger (GHZ) entanglement of photons. The success probability of the proposed Bell measurement can be made arbitrarily high using only linear optics as the number of photons in a logical qubit increases. We compare our scheme with all the other proposals, using single-photon qubits, coherent-state qubits or hybrid qubits, suggested to enhance the efficiency of the Bell measurement. As a remarkable advantage, our scheme requires only…
The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform. Optical photons passing through linear networks may be configured to perform quantum simulation tasks, but the efficient preparation and detection of multiphoton quantum states of light in linear optical systems are challenging. Here, we experimentally implement a boson sampling protocol for simulating molecular vibronic spectra [Nature Photonics $\textbf{9}$…
The phenomenon of quantum revivals resulting from the self-interference of wave packets has been observed in several quantum systems and utilized widely in spectroscopic applications. Here, we present a combined analytical and numerical study on the generation of orientational quantum revivals (OQRs) exclusively using a single-cycle THz pulse. As a proof of principle, we examine the scheme in the linear polar molecule HCN with experimentally accessible pulse parameters and obtain strong field-free OQR without requiring the condition of the sudden-impact limit. To visualize the involved quantum…
In practical quantum key distribution (QKD), weak coherent states as the photon sources have a limit in secure key rate and transmission distance because of the existence of multiphoton pulses and heavy loss in transmission line. Decoy states method and nonorthogonal encoding protocol are two important weapons to combat these effects. Here, we combine these two methods and propose a efficient method that can substantially improve the performance of QKD. We find a 79 km increase in transmission distance over the prior record using decoy states method.
Selective control of decoherence is demonstrated for a multilevel system by generalizing the instantaneous phase of any chirped pulse as individual terms of a Taylor series expansion. In the case of a simple two-level system, all odd terms in the series lead to population inversion while the even terms lead to self-induced transparency. These results also hold for multiphoton transitions that do not have any lower-order photon resonance or any intermediate virtual state dynamics within the laser pulse-width. Such results form the basis of a robustly implementable CNOT gate.
The smallest spot in optical lithography and microscopy is generally limited by diffraction. Quantum lithography, which utilizes interference between groups of N entangled photons, was recently proposed to beat the diffraction limit by a factor N. Here we propose a simple method to obtain N photons interference with classical pulses that excite a narrow multiphoton transition, thus shifting the "quantum weight" from the electromagnetic field to the lithographic material. We show how a practical complete lithographic scheme can be developed and demonstrate the underlying principles experimental…
