The absolute mass value of $^{168}$Yb has been directly determined with the JYFLTRAP Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line (IGISOL) facility. A more precise value of the mass of $^{168}$Yb is needed to extract possible signatures of beyond standard model physics from high-precision isotope shift measurements of Yb atomic transition frequencies. The measured mass-excess value, ME($^{168}$Yb) = $-$61579.846(94) keV, is 12 times more precise and deviates from the Atomic Mass Evaluation 2016 value by 1.7$σ$. The impact on precision isotope shift studies of the stable Yb isotopes is discussed.
The photo-neutron cross sections of $^{162,163}\rm{Dy}$ have been measured for the first time in an energy region from the neutron threshold ($S_n$) up to $\approx$ $13$~MeV. The ($γ$,n) reaction was induced with quasi-monochromatic laser Compton-scattered $γ$ rays, produced at the NewSUBARU laboratory. The corresponding $γ$-ray strength functions ($γ$SF) have been calculated from the photo-neutron cross sections. The data are compared to reanalyzed $γ$SFs of $^{160-164}\rm{Dy}$, which are measured below $S_n$. The excellent agreement with the photo-neutron data at $S_n$ confirms the principle…
Nuclear mass measurements of isotopes are key to improving our understanding of nuclear structure across the chart of nuclides, in particular for the determination of the appearance or disappearance of nuclear shell closures. We present high-precision mass measurements of neutron-rich Ca, Ti and V isotopes performed at the TITAN and LEBIT facilities. These measurements were made using the TITAN multiple-reflection time-of-flight mass spectrometer (MR-ToF-MS) and the LEBIT 9.4T Penning trap mass spectrometer. In total, 13 masses were measured, eight of which represent increases in precision ove…
We present the results of precision mass measurements of neutron-rich cadmium isotopes. These nuclei approach the $N=82$ closed neutron shell and are important to nuclear structure as they lie near doubly-magic $^{132}$Sn on the chart of nuclides. Of particular note is the clear identification of the ground state mass in $^{127}$Cd along with the isomeric state. We show that the ground state identified in a previous mass measurement which dominates the mass value in the Atomic Mass Evaluation is an isomeric state. In addition to $^{127/m}$Cd, we present other cadmium masses measured ($^{125/m}…
We report high-precision mass measurements of $^{50-55}$Sc isotopes performed at the LEBIT facility at NSCL and at the TITAN facility at TRIUMF. Our results provide a substantial reduction of their uncertainties and indicate significant deviations, up to 0.7 MeV, from the previously recommended mass values for $^{53-55}$Sc. The results of this work provide an important update to the description of emerging closed-shell phenomena at neutron numbers $N=32$ and $N=34$ above proton-magic $Z=20$. In particular, they finally enable a complete and precise characterization of the trends in ground stat…
The region near Z=28, N=40 is a subject of great interest for nuclear structure studies due to spectroscopic signatures in $^{68}$Ni suggesting a subshell closure at N=40. Trends in nuclear masses and their derivatives provide a complementary approach to shell structure investigations via separation energies. Penning trap mass spectrometry has provided precise measurements for a number of nuclei in this region, however a complete picture of the mass surfaces has so far been limited by the large uncertainty remaining for nuclei with N > 40 along the iron and cobalt chains. Here we present the f…
Probing the N=104 midshell region for the r process via precision mass spectrometry of neutron-rich rare-earth isotopes with the JYFLTRAP double Penning trap
We present a robust analysis code developed in the Python language and incorporating libraries of the ROOT data analysis framework for the state-of-the-art mass spectrometry method called phase-imaging ion-cyclotron-resonance (PI-ICR). A step-by-step description of the dataset construction and analysis algorithm is given. The code features a new phase-determination approach that offers up to 10 times smaller statistical uncertainties. This improvement in statistical uncertainty is confirmed using extensive Monte-Carlo simulations and allows for very high-precision studies of exotic nuclear mas…
Mass measurements continue to provide invaluable information for elucidating nuclear structure and scenarios of astrophysical interest. The transition region between the $Z = 20$ and $28$ proton shell closures is particularly interesting due to the onset and evolution of nuclear deformation as nuclei become more neutron rich. This provides a critical testing ground for emerging ab-initio nuclear structure models. Here, we present high-precision mass measurements of neutron-rich chromium isotopes using the sensitive electrostatic Multiple-Reflection Time-Of-Flight Mass Spectrometer (MR-TOF-MS) …
Atomic isotope shifts (ISs) are the isotope-dependent energy differences in the atomic electron energy levels. These shifts serve an important role in atomic and nuclear physics, and particularly in the latter as signatures of nuclear structure. Recently ISs have been suggested as unique probes of beyond Standard Model (SM) physics, under the condition that they be determined significantly more precisely than current state of the art. In this work we present a simple and robust method for measuring ISs with ions in a Paul trap, by taking advantage of Hilbert subspaces that are insensitive to c…
High-precision ab initio calculations of nuclear binding energies: Tin isotopes from dripline to dripline
Technische Universität Darmstadt（达姆施塔特工业大学）；ExtreMe Matter Institute EMMI, GSI Helmholtzzentrum für Schwerionenforschung GmbH（GSI重离子研究中心极端物质研究所EMMI）；KU Leuven, Instituut voor Kern- en Stralingsfysica（荷语鲁汶大学核与辐射物理研究所）；Institut d’Astronomie et d’Astrophysique, Université Libre de Bruxelles（布鲁塞尔自由大学天体物理学与天文学研究所）；Brussels Laboratory of the Universe – BLU-ULB（布鲁塞尔宇宙实验室）；IRFU, CEA, Université Paris-Saclay（巴黎萨克雷大学CEA IRFU）；Max-Planck-Institut für Kernphysik（马克斯·普朗克核物理研究所）
If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$σ$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both…
Nuclear properties across the chart of nuclides are key to improving and validating our understanding of the strong interaction in nuclear physics. We present high-precision mass measurements of neutron-rich Fe isotopes performed at the TITAN facility. The multiple-reflection time-of-flight mass spectrometer (MR-ToF-MS), achieving a resolving power greater than $600\,000$ for the first time, enabled the measurement of $^{63-70}$Fe, including first-time high-precision direct measurements ($δm/m \sim 10^{-7}$) of $^{68-70}$Fe, as well as the discovery of a long-lived isomeric state in $^{69}$Fe.…
We report on the mass measurements of several neutron-rich $\mathrm{Rb}$ and $\mathrm{Sr}$ isotopes in the $A \approx 100$ region with the TITAN Penning-trap mass spectrometer. Using highly charged ions in the charge state $q=10+$, the masses of $^{98,99}\mathrm{Rb}$ and $^{98-100}\mathrm{Sr}$ have been determined with a precision of $6 - 12\ \mathrm{keV}$, making their uncertainty negligible for r-process nucleosynthesis network calculations. The mass of $^{101}\mathrm{Sr}$ has been determined directly for the first time with a precision eight times higher than the previous indirect measureme…
A precision mass investigation of the neutron-rich titanium isotopes $^{51-55}$Ti was performed at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The range of the measurements covers the $N=32$ shell closure and the overall uncertainties of the $^{52-55}$Ti mass values were significantly reduced. Our results confirm the existence of a weak shell effect at $N=32$, establishing the abrupt onset of this shell closure. Our data were compared with state-of-the-art \textit{ab-initio} shell model calculations which, despite very successfully describing where the $N=32$ shell gap is strong,…
A new beamline for Resonant Excitation of Beams with Electromagnetic fields and Lasers (REBEL) and Stopping and Trapping of Radioactive Isotopes for Precision Experiments (STRIPE)
We report measurements of the isotope shifts of two transitions ($4f^46s\rightarrow [25044.7]^{\circ}_{7/2}$ and $4f^46s\rightarrow [25138.6]^{\circ}_{7/2}$) in neodymium ions (Nd$^+$) with hundredfold improved accuracy, using laser spectroscopy of a cryogenically-cooled neutral plasma. The isotope shifts were measured across a set of five spin-zero isotopes that spans a nuclear shape transition. We discuss the prospects for further improvements to the accuracy of Nd$^+$ isotope shifts using optical clock transitions, which could enable higher precision tests of King plot linearity for new phy…
High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis
The University of Hong Kong（香港大学）；Sino-French Institute of Nuclear Engineering and Technology, Sun Yat-Sen University（中山大学中法核工程与技术学院）；RIKEN Nishina Center for Accelerator-Based Science, RIKEN（理化学研究所仁科加速器科学研究中心）；Advanced Energy Science And Technology GuangDong Laboratory（广东省先进能源科学与技术实验室）；State Key Laboratory of Heavy Ion Science and Technology, Institute of Modern Physics, Chinese Academy of Sciences（中国科学院近代物理研究所重离子物理国家重点实验室）；Wako Nuclear Science Center (WNSC), Institute of Particle and Nuclear Studies (IPNS), High Energy Accelerator Research Organization (KEK)（高能加速器研究机构粒子与核研究所在职和核科学中心）；Department of Physics, Kyushu University（九州大学物理学系）；School of Physics, Peking University（北京大学物理学院）
The JYFLTRAP double Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility has been used to measure the atomic masses of 13 neutron-rich rare-earth isotopes. Eight of the nuclides, $^{161}$Pm, $^{163}$Sm, $^{164,165}$Eu, $^{167}$Gd, and $^{165,167,168}$Tb, were measured for the first time. The systematics of the mass surface has been studied via one- and two-neutron separation energies as well as neutron pairing-gap and shell-gap energies. The proton-neutron pairing strength has also been investigated. The impact of the new mass values on the astrophysical rapid neutron capt…
Precision Isotope-Shift Measurement of the ${}^1S_0 \leftrightarrow {}^3P_2$ Transition and a Multi-Transition King-Plot Consistency Test
Kyoto University（京都大学）；HIKARI-COOL Kyoto（HIKARI-COOL 京都）；The Hakubi Center for Advanced Research, Kyoto University（京都大学博雅研究高级研究中心）；ELTE, Eötvös Loránd University（罗兰大学）；High Energy Accelerator Research Organization (KEK)（高能加速器研究机构）；The University of Osaka（大阪大学）
Direct mass measurements of the low-spin $3/2^{(-)}$ and high-spin $13/2^{(+)}$ states in the neutron-deficient isotopes $^{195}$Po, $^{197}$Po, and high-spin $13/2^{(+)}$ state in $^{199}$Po were performed with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE-CERN. These measurements allow the determination of the excitation energy of the isomeric state arising from the $ν$i$_{13/2}$ orbital in $^{195,197}$Po. Additionally, the excitation energy of isomeric states of lead, radon, and radium isotopes in this region were obtained from $α$-decay chains. The new excitation energies complete …
The rare-earth peak in the $r$-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in $r$-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. $^{158}$Nd, $^{160}$Pm, $^{162}$Sm, and $^{164-166}$Gd have been measured for the first time and the precisions for $^{156}$Nd, $^{158}$Pm, $^{162,163}$Eu, $^{163}$Gd, and $^{164}$Tb have been improved considerably. Nuclear struct…
Precision mass measurements of neutron-rich rhodium isotopes have been performed at the JYFLTRAP Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line (IGISOL) facility. We report results on ground- and isomeric-state masses in $^{110,112,114,116,118}$Rh and the very first mass measurement of $^{120}$Rh. The isomeric states were separated and measured for the first time using the phase-imaging ion-cyclotron-resonance (PI-ICR) technique. For $^{112}$Rh, we also report new half-lives for both the ground state and the isomer. The results are compared to theoretical predictions…
Magneto-optical trapping of bosonic and fermionic neon isotopes and their mixtures: isotope shift of the ^3P_2 to ^3D_3 transition and hyperfine constants of the ^3D_3 state of Ne-21
A high-voltage MR-ToF mass spectrometer and separator for the study of exotic isotopes at FRIB
Facility for Rare Isotope Beams（稀有同位素束设施）；Michigan State University（密歇根州立大学）；University of Edinburgh（爱丁堡大学）；Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）
A large experimental program is being mounted to search for neutrinoless double-beta decay over the next decade. Multiple experiments using different target isotopes are being prepared to explore the whole parameter space allowed for inverted-ordered light neutrinos, and have the potential to make discoveries in several other scenarios, including normal-ordered light neutrinos and other exotic mechanisms. We investigate to what extent long-range and exotic short-range contributions may be distinguished by combining measurements of the decay half-life across isotopes. We demonstrate how measure…
The neutron-rich isotopes $^{58-63}$Cr were produced for the first time at the ISOLDE facility and their masses were measured with the ISOLTRAP spectrometer. The new values are up to 300 times more precise than those in the literature and indicate significantly different nuclear structure from the new mass-surface trend. A gradual onset of deformation is found in this proton and neutron mid-shell region, which is a gateway to the second island of inversion around \emph{N}=40. In addition to comparisons with density-functional theory and large-scale shell-model calculations, we present predicti…
We report on the design, installation, and test of an experimental facility for the production of ultra-cold atomic isotopes and isomers of cesium. The setup covers a broad span of mass numbers and nuclear isomers, allowing one to directly compare chains of isotopes and isotope/isomer pairs. Cesium nuclei are produced by fission or fusion-evaporation reactions using primary proton beams from a 130 MeV cyclotron impinging upon a suitable target. The species of interest is ejected from the target in ionic form, electrostatically accelerated, mass separated, and routed to a science chamber. Here,…
With increasing demand for accurate calculation of isotope shifts of atomic systems for fundamental and nuclear structure research, an analytic energy derivative approach is presented in the relativistic coupled-cluster theory framework to determine the atomic field shift and mass shift factors. This approach allows the determination of expectation values of atomic operators, overcoming fundamental problems that are present in existing atomic physics methods, i.e. it satisfies the Hellmann-Feynman theorem, does not involve any non-terminating series, and is free from choice of any perturbative…
Reactor neutrino experiments have seen major improvements in precision in recent years. With the experimental uncertainties becoming lower than those from theory, carefully considering all sources of $\overlineν_{e}$ is important when making theoretical predictions. One source of $\overlineν_{e}$ that is often neglected arises from the irradiation of the nonfuel materials in reactors. The $\overlineν_{e}$ rates and energies from these sources vary widely based on the reactor type, configuration, and sampling stage during the reactor cycle and have to be carefully considered for each experiment…
An investigation of the α-decay of $^{147}$Sm was performed using an ultra low-background Twin Frisch-Grid Ionisation Chamber (TF-GIC). Four natural samarium samples were produced using pulsed laser deposition in ultra high vacuum. The abundance of the $^{147}$Sm isotope was mea- sured using inductively coupled plasma mass spectrometry. A combined half-life value for 147Sm of $1.079(26)\times{}10^{11}$ years was measured. A search for the α-decay into the first excited state of $^{143}$Nd has been performed using $γ$-spectroscopy, resulting in a lower half-life limit of $T_{1/2} > 3.1 \times{}…
Radioactivity is understood to be described by a Poisson process, yet some measurements of nuclear decays appear to exhibit unexpected variations. Generally, the isotopes reporting these variations have long half lives, which are plagued by large measurement uncertainties. In addition to these inherent problems, there are some reports of time-dependent decay rates and even claims of exotic neutrino-induced variations. We present a dedicated experiment for the stable long-term measurement of gamma emissions resulting from $β$ decays, which will provide high-quality data and allow for the identi…
