Electrical Control of Coherent Spin Rotation of a Single-Spin Qubit
Xiaoche Wang, Yuxuan Xiao, Chuanpu Liu, Eric Lee-Wong, Nathan J. McLaughlin, Hanfeng Wang, Mingzhong Wu, Hailong Wang, Eric E. Fullerton, Chunhui Rita Du
Nitrogen vacancy (NV) centers, optically-active atomic defects in diamond, have attracted tremendous interest for quantum sensing, network, and computing applications due to their excellent quantum coherence and remarkable versatility in a real, ambient environment. One of the critical challenges to develop NV-based quantum operation platforms results from the difficulty to locally address the quantum spin states of individual NV spins in a scalable, energy-efficient manner. Here, we report electrical control of the coherent spin rotation rate of a single-spin qubit in NV-magnet based hybrid quantum systems. By utilizing electrically generated spin currents, we are able to achieve efficient tuning of magnetic damping and the amplitude of the dipole fields generated by a micrometer-sized resonant magnet, enabling electrical control of the Rabi oscillation frequency of NV spins. Our results highlight the potential of NV centers in designing functional hybrid solid-state systems for next-generation quantum-information technologies. The demonstrated coupling between the NV centers and the propagating spin waves harbored by a magnetic insulator further points to the possibility to establish macroscale entanglement between distant spin qubits.
We present a modulated microwave approach for quantum computing with qubits comprising three spins in a triple quantum dot. This approach includes single- and two-qubit gates that are protected against low-frequency electrical noise, due to an operating point with a narrowband response to high frequency electric fields. Furthermore, existing double quantum dot advances, including robust preparation and measurement via spin-to-charge conversion, are immediately applicable to the new qubit. Finally, the electric dipole terms implicit in the high frequency coupling enable strong coupling with sup…
Spin qubits offer one of the most promising routes to the implementation of quantum computers. Very recent results in semiconductor quantum dots show that electrically-controlled gating schemes are particularly well-suited for the realization of a universal set of quantum logical gates. Scalability to a larger number of qubits, however, remains an issue for such semiconductor quantum dots. In contrast, a chemical bottom-up approach allows one to produce identical units in which localized spins represent the qubits. Molecular magnetism has produced a wide range of systems with tailored properti…
Enhanced coherence in HoW$_{10}$ molecular spin qubits has been demonstrated by use of Clock Transitions (CTs). More recently it was shown that, while operating at the CTs, it was possible to use an electrical field to selectively address HoW$_{10}$ molecules pointing in a given direction, within a crystal that contains two kinds of identical but inversion-related molecules. Herein we theoretically explore the possibility of employing the electric field to effect entangling two-qubit quantum gates among two neighbouring CT-protected HoW$_{10}$ qubits within a diluted crystal. We estimate the t…
We investigate the influence of electrical charge noise on a resonant exchange (RX) qubit in a triple quantum dot. This RX qubit is a variation of the exchange-only spin qubit which responds to a narrow-band resonant frequency. Our noise model includes uncorrelated charge noise in each quantum dot giving rise to two independent (noisy) bias parameters $\varepsilon$ and $Δ$. We calculate the energy splitting of the two qubit states as a function of these two bias detuning parameters to find "sweet spots", where the qubit is least susceptible to noise. Our investigation shows that such sweet spo…
We analyze the reading and initialization of a topological qubit encoded by Majorana fermions in one-dimensional semiconducting nanowires, weakly coupled to a single level quantum dot (QD). It is shown that when the Majorana fermions are fused by tuning gate voltage, the topological qubit can be read out directly through the occupation of the QD in an energy window. The initialization of the qubit can also be realized via adjusting the gate voltage on the QD, with the total fermion parity conserved. As a result, both reading and initialization processes can be achieved in an all-electrical way…
All-electrical dephasing-protected spin qubits in altermagnets
Consejo Superior de Investigaciones Científicas (CSIC)（西班牙高等科学研究委员会）；Quantum Advanced Research Center (QuARC)（量子先进研究中心）；Instituto de Ciencia de Materiales de Madrid (ICMM)（马德里材料科学研究所）；Nordita（北欧理论天体物理学研究所）；KTH Royal Institute of Technology（瑞典皇家理工学院）；Stockholm University（斯德哥尔摩大学）
The electrical control of single spin qubits based on semiconductor quantum dots is of great interest for scalable quantum computing since electric fields provide an alternative mechanism for qubit control compared with magnetic fields and can also be easier to produce. Here we outline the mechanism for a drastic enhancement in the electrically-driven spin rotation frequency for silicon quantum dot qubits in the presence of a step at a hetero-interface. The enhancement is due to the strong coupling between the ground and excited states which occurs when the electron wave-function overcomes the…
We describe and discuss a solid state proposal for quantum computation with mobile spin qubits in one-dimensional systems, based on recent advances in spintronics. Static electric fields are used to implement a universal set of quantum gates, via the spin-orbit and exchange couplings. Initialization and measurement can be performed either by spin injection from/to ferromagnets, or by using spin filters and mesoscopic spin polarizing beam-splitters. The vulnerability of this proposal to various sources of error is estimated by numerical simulations. We also assess the suitability of various mat…
We study the effect of the spin-orbit interaction on heavy holes confined in a double quantum dot in the presence of a magnetic field of arbitrary direction. Rich physics arise as the two hole states of different spin are not only coupled by the spin-orbit interaction but additionally by the effect of site-dependent anisotropic $g$ tensors. It is demonstrated that these effects may counteract in such a way as to cancel the coupling at certain detunings and tilting angles of the magnetic field. This feature may be used in singlet-triplet qubits to avoid leakage errors and implement an electrica…
Large-scale quantum computers must be built upon quantum bits that are both highly coherent and locally controllable. We demonstrate the quantum control of the electron and the nuclear spin of a single 31P atom in silicon, using a continuous microwave magnetic field together with nanoscale electrostatic gates. The qubits are tuned into resonance with the microwave field by a local change in electric field, which induces a Stark shift of the qubit energies. This method, known as A-gate control, preserves the excellent coherence times and gate fidelities of isolated spins, and can be extended to…
The spins of atoms and atom-like systems are among the most coherent objects in which to store quantum information. However, the need to address them using oscillating magnetic fields hinders their integration with quantum electronic devices. Here we circumvent this hurdle by operating a single-atom `flip-flop' qubit in silicon, where quantum information is encoded in the electron-nuclear states of a phosphorus donor. The qubit is controlled using local electric fields at microwave frequencies, produced within a metal-oxide-semiconductor device. The electrical drive is mediated by the modulati…
Electrons confined in Si quantum dots possess orbital, spin, and valley degrees of freedom (d.o.f.). We perform Landau-Zener-Stuckelberg-Majorana (LZSM) interferometry on a Si double quantum dot that is strongly coupled to a microwave cavity to probe the valley d.o.f. The resulting LZSM interference pattern is asymmetric as a function of level detuning and persists for drive periods that are much longer than typical charge decoherence times. By correlating the LZSM interference pattern with charge noise measurements, we show that valley-orbit hybridization provides some protection from the del…
Exchange-coupled singlet-triplet spin qubits in two gate-defined double quantum dots are considered theoretically. Using charge density operators to describe the double-dot orbital states, we calculate the Coulomb couplings between the qubits, and identify optimal bias points for single- and two-qubit operations, as well as convenient idle positions. The same intuitive formulation is used to derive dephasing rates of these qubits due to the fluctuating charge environment, thereby providing the main considerations for a quantum computation architecture that is within current experimental capabi…
We show that the mixing between spin and valley degrees of freedom in a silicon quantum bit (qubit) can be controlled by a static electric field acting on the valley splitting $Δ$. Thanks to spin-orbit coupling, the qubit can be continuously switched between a spin mode (where the quantum information is encoded into the spin) and a valley mode (where the the quantum information is encoded into the valley). In the spin mode, the qubit is more robust with respect to inelastic relaxation and decoherence, but is hardly addressable electrically. It can however be brought into the valley mode then b…
We propose a method to electrically control electron spins in donor-based qubits in silicon. By taking advantage of the hyperfine coupling difference between a single-donor and a two-donor quantum dot, spin rotation can be driven by inducing an electric dipole between them and applying an alternating electric field generated by in-plane gates. These qubits can be coupled with exchange interaction controlled by top detuning gates. The qubit device can be fabricated deep in the silicon lattice with atomic precision by scanning tunneling probe technique. We have combined a large-scale full band a…
A Degenerate Singlet-Triplet Qubit with All-Electrical Orthogonal Control
Harvard University（哈佛大学）；QuTech and Kavli Institute of Nanoscience, Delft University of Technology（代尔夫特理工大学量子纳米科学卡弗里研究所与QuTech）；QuTech and Netherlands Organisation for Applied Scientific Research (TNO)（荷兰应用科学研究组织（TNO）与QuTech）
We propose a realizable architecture using one-dimensional transmission line resonators to reach the strong coupling limit of cavity quantum electrodynamics in superconducting electrical circuits. The vacuum Rabi frequency for the coupling of cavity photons to quantized excitations of an adjacent electrical circuit (qubit) can easily exceed the damping rates of both the cavity and the qubit. This architecture is attractive both as a macroscopic analog of atomic physics experiments and for quantum computing and control, since it provides strong inhibition of spontaneous emission, potentially le…
In this paper, we investigate the impact of gating potential and magnetic field on phonon induced spin relaxation rate and the speed of the electrically driven single-qubit operations inside the InSb nanowire spin qubit. We show that a strong $g$ factor and high magnetic field strength lead to the prevailing influence of electron-phonon scattering due to deformation potential, considered irrelevant for materials with a weak $g$ factor, like GaAs or Si/SiGe. In this regime, we find that spin relaxation between qubit states is significantly suppressed due to the confinement perpendicular to the …
Any single-qubit unitary operation or quantum gate can be considered a rotation. Typical experimental implementations of single-qubit gates involve two or three fixed rotation axes, and up to three rotation steps. Here we show that, if the rotation axes can be tuned arbitrarily in a fixed plane, then two rotation steps are sufficient for implementing a single-qubit gate, and one rotation step is sufficient for implementing a state transformation. The results are relevant for "exchange-only" logical qubits encoded in three-spin blocks, which are important for universal quantum computation in de…
We discuss the modeling of the electrical manipulation of spin qubits in the linear-response regime where the Rabi frequency is proportional to the magnetic field and to the radio-frequency electric field excitation. We show that the Rabi frequency can be obtained from a generalized g-tensor magnetic resonance formula featuring a g-matrix and its derivative g' with respect to the electric field (or gate voltage) as inputs. These matrices can be easily calculated from the wave functions of the qubit at zero magnetic field. The g-matrix formalism therefore provides the complete dependence of the…
Full electrical control of quantum bits could enable fast, low-power, scalable quantum computation. Although electric dipoles are highly attractive to couple spin qubits electrically over long distances, mechanisms identified to control two-qubit couplings do not permit single-qubit operations while two-qubit couplings are off. Here we identify a mechanism to modulate electrical coupling of spin qubits that overcomes this drawback for hole spin qubits in acceptors,that is based on the electrical tuning of the direction of the spin-dependent electric dipole by a gate. In this way, inter-qubit c…
Qubits based on transistor-like Si MOS nanodevices are promising for quantum computing. In this work, we demonstrate a double quantum dot spin qubit that is all-electrically controlled without the need for any external components, like micromagnets, that could complicate integration. Universal control of the qubit is achieved through spin-orbit-like and exchange interactions. Using single shot readout, we show both DC- and AC-control techniques. The fabrication technology used is completely compatible with CMOS.
A fundamental design challenge for quantum dot spin qubits is to extend the strength and range of qubit interactions while suppressing their coupling to the environment, since both effects have electrical origins. Key tools include the ability to retune the qubits, to take advantage of physical resources in different operating regimes, and to access optimal working points, or "sweet spots," where dephasing is minimized. Here, we explore an important, new resource for singlet-triplet qubits: a transverse sweet spot (TSS) that enables (i) direct transitions between qubit states, (ii) a strong, c…
Nuclear spin qubits have the longest coherence times in the solid state, but their quantum read-out and initialization is a great challenge. We present a theory for the interaction of an electric current with the nuclear spins of donor impurities in semiconductors. The theory yields a sensitivity criterion for quantum detection of nuclear spin states using electrically detected magnetic resonance, as well as an all electrical method for fast nuclear spin qubit initialization.
Coherent rotations of single spin-based qubits may be accomplished electrically at fixed Zeeman energy with a qubit defined solely within a single electrostatically-defined quantum dot; the $g$-factor and the external magnetic field are kept constant. All that is required to be varied are the voltages on metallic gates which effectively change the shape of the elliptic quantum dot. The pseudospin-1/2 qubit is constructed from the two-dimensional $S=1/2$, $S_z=-1/2$ subspace of three interacting electrons in a two-dimensional potential well. Rotations are created by altering the direction of th…
We consider a model of two interacting always-on, exchange-only qubits for which controlled phase ($CPHASE$), controlled NOT ($CNOT$), quantum Fourier transform ($QFT$) and $SWAP$ operations can be implemented only in a few electrical pulses in a nanosecond time scale. Each qubit is built of three quantum dots (TQD) in a triangular geometry with three electron spins which are always kept coupled by exchange interactions only. The qubit states are encoded in a doublet subspace and are fully electrically controlled by a voltage applied to gate electrodes. The two qubit quantum gates are realized…
We describe an approach to electrically control the strong interaction between a single electron spin and the vibrational motion of a suspended carbon nanotube resonator. The strength of the deflection-induced spin-phonon coupling is dependent on the wavefunction of the electron confined in a lateral carbon nanotube quantum dot. An electrical field along the nanotube shifts the effective center of the quantum dot, leading to the corresponding modification of the spin-phonon strength. Numerical simulations with experimentally reachable parameters show that high fidelity quantum state transfer b…
We propose a quadrupolar exchange-only spin (QUEX) qubit that is highly robust against charge noise and nuclear spin dephasing, the dominant decoherence mechanisms in quantum dots. The qubit consists of four electrons trapped in three quantum dots, and operates in a decoherence-free subspace to mitigate dephasing due to nuclear spins. To reduce sensitivity to charge noise, the qubit can be completely operated at an extended charge noise sweet spot that is first-order insensitive to electrical fluctuations. Due to on-site exchange mediated by the Coulomb interaction, the qubit energy splitting …
We investigate the effects of the orientation of the magnetic field and the orientation of a quantum dot, with respect to crystallographic coordinates, on the quality of an electrically controlled qubit realized in a gated semiconductor quantum dot. We find that, due to the anisotropy of the spin-orbit interactions, varying the two orientations it is possible to tune the qubit in the sense of optimizing the ratio of its couplings to phonons and to a control electric field. We find conditions under which such optimal setup can be reached by solely reorienting the magnetic field, and when a spec…
Semiconductor quantum dots in silicon are promising qubits because of long spin coherence times and their potential for scalability. However, such qubits with complete electrical control and fidelities above the threshold for quantum error correction have not yet been achieved. We show theoretically that the threshold fidelity can be achieved with ac gate operation of the quantum dot hybrid qubit. Formed by three electrons in a double dot, this qubit is electrically controlled, does not require magnetic fields, and runs at GHz gate speeds. We analyze the decoherence caused by 1/f charge noise …
Multi-donor quantum dots have been at the forefront of recent progress in Si-based quantum computation. Among them, $2P:1P$ qubits have a built-in dipole moment, enabling all-electrical spin operation via hyperfine mediated electron dipole spin resonance (EDSR). The development of all-electrical multi-donor dot qubits requires a full understanding of their EDSR and coherence properties, incorporating multi-valley nature of their ground state. Here, by introducing a variational effective mass wave-function, we examine the impact of qubit geometry and nearby charge defects on the electrical oper…
Electrically driven spin resonance (EDSR) is an established tool for controlling semiconductor spin qubits. Here, we theoretically study a frequency-mixing variant of EDSR, where two driving tones with different drive frequencies are applied, and the resonance condition connects the spin Larmor frequency with the sum of the two drive frequencies. Focusing on flopping-mode operation, we calculate the parameter dependence of the Rabi frequency and the Bloch-Siegert shift. A shared-control spin qubit architecture could benefit from this bichromatic EDSR scheme, as it enables simultaneous single-q…
We study a voltage-controlled version of the superconducting flux qubit [Chiorescu et al., Science 299, 1869 (2003)] and show that full control of qubit rotations on the entire Bloch sphere can be achieved. Circuit graph theory is used to study a setup where voltage sources are attached to the two superconducting islands formed between the three Josephson junctions in the flux qubit. Applying a voltage allows qubit rotations about the y axis, in addition to pure x and z rotations obtained in the absence of applied voltages. The orientation and magnitude of the rotation axis on the Bloch sphere…
Strong, direct Rashba spin-orbit coupling in Si, Ge, and the Ge/Si core/shell nanowire quantum dot (QD) allows for all electrical manipulation of the hole spin qubit. Motivated by this fact, we analyze different fabrication-dependent properties of nanowires, such as orientation, cross section, and the presence of strain, with the goal being to find the material and geometry that enables the fastest qubit manipulation, whose speed can be identified using the Rabi frequency. We show that QD in nanowires with a circular cross section (cNWs) enables much weaker driving of the hole spin qubit than …
High fidelity entanglement of an on-chip array of spin qubits poses many challenges. Spin-orbit coupling (SOC) can ease some of these challenges by enabling long-ranged entanglement via electric dipole-dipole interactions, microwave photons, or phonons. However, SOC exposes conventional spin qubits to decoherence from electrical noise. Here we propose an acceptor-based spin-orbit qubit in silicon offering long-range entanglement at a sweet spot where the qubit is protected from electrical noise. The qubit relies on quadrupolar SOC with the interface and gate potentials. As required for surface…
Resonant manipulation of carbon nanotube valley-spin qubits by an electric field is investigated theoretically. We develop a new analysis of electrically driven spin resonance exploiting fixed physical characteristics of the nanotube: a bend and inhomogeneous disorder. The spectrum is simulated for an electron valley-spin qubit coupled to a hole valley-spin qubit and an impurity electron spin, and features that coincide with a recent measurement are identified. We show that the same mechanism allows resonant control of the full four-dimensional spin-valley space.
We investigate capacitively coupled two-qubit quantum gates based on quantum dots. For exchange-only coded qubits electron spin $S$ and its projection $S_z$ are exact quantum numbers. Capacitive coupling between qubits, as distinct from interqubit exchange, preserves these quantum numbers. We prove, both analytically and numerically, that conservation of the spins of individual qubits has dramatic effect on performance of two-qubit gates. By varying the level splittings of individual qubits, $J_a$ and $J_b$, and the interqubit coupling time $t$, we can find an infinite number of triples $(J_a,…
Nanofabricated quantum bits permit large-scale integration but usually suffer from short coherence times due to interactions with their solid-state environment. The outstanding challenge is to engineer the environment so that it minimally affects the qubit, but still allows qubit control and scalability. Here we demonstrate a long-lived single-electron spin qubit in a Si/SiGe quantum dot with all-electrical two-axis control. The spin is driven by resonant microwave electric fields in a transverse magnetic field gradient from a local micromagnet, and the spin state is read out in single-shot mo…
Once called a "classically non-describable two-valuedness" by Pauli , the electron spin is a natural resource for long-lived quantum information since it is mostly impervious to electric fluctuations and can be replicated in large arrays using silicon quantum dots, which offer high-fidelity control. Paradoxically, one of the most convenient control strategies is the integration of nanoscale magnets to artificially enhance the coupling between spins and electric field, which in turn hampers the spin's noise immunity and adds architectural complexity. Here we demonstrate a technique that enables…
In this paper, several nanodevices which realize basic single heavy hole qubit operations are proposed and supported by time dependent self consistent Poisson-Schrödinger calculations using a four band heavy hole-light hole model. In particular we propose a set of nanodevices which can act as Pauli X, Y, Z quantum gates and as a gate that acts similar as a Hadamard gate (i.e. it creates a balanced superposition of basis states but with an additional phase factor) on the heavy hole spin qubit. We also present the design and simulation of a gated semiconductor nanodevice which can realize an arb…
Strong `spin'-orbit coupled one-dimensional hole gas is achievable in a Ge nanowire in the presence of a strong magnetic field. The strong magnetic field lifts the two-fold degeneracy in the hole subband dispersions, so that the effective low-energy subband dispersion exhibits strong `spin'-orbit coupling. Here, we study the electrical `spin' manipulation in a Ge nanowire quantum dot for both the lowest and second lowest hole subband dispersions. Using a finite square well to model the quantum dot confining potential, we calculate exactly the level splitting of the `spin'-orbit qubit and the R…
Nuclear spins in semiconductors are leading candidates for quantum technologies, including quantum computation, communication, and sensing. Nuclear spins in diamond are particularly attractive due to their extremely long coherence lifetime. With the nitrogen-vacancy (NV) centre, such nuclear qubits benefit from an auxiliary electronic qubit, which has enabled entanglement mediated by photonic links. The transport of quantum information by the electron itself, via controlled transfer to an adjacent centre or via the dipolar interaction, would enable even faster and smaller processors, but optic…
In a semiconductor spin qubit with sizable spin-orbit coupling, coherent spin rotations can be driven by a resonant gate-voltage modulation. Recently, we have exploited this opportunity in the experimental demonstration of a hole spin qubit in a silicon device. Here we investigate the underlying physical mechanisms by measuring the full angular dependence of the Rabi frequency as well as the gate-voltage dependence and anisotropy of the hole $g$-factors. We show that a $g$-matrix formalism can simultaneously capture and discriminate the contributions of two mechanisms so far independently disc…
Cryogen-free low-temperature setups are becoming more prominent in experimental science due to their convenience and reliability, and concern about the increasing scarcity of helium as a natural resource. Despite not having any moving parts at the cold end, pulse tube cryocoolers introduce vibrations that can be detrimental to the experiments. We characterize the coupling of these vibrations to the electrical signal observed on cables installed in a cryogen-free dilution refrigerator. The dominant electrical noise is in the 5 to 10 kHz range and its magnitude is found to be strongly temperatur…
Electron spins confined in quantum dots are an attractive system to realize high-fidelity qubits owing to their long coherence time. With the prolonged spin coherence time, however, the control fidelity can be limited by systematic errors rather than decoherence, making characterization and suppression of their influence crucial for further improvement. Here we report that the control fidelity of Si/SiGe spin qubits can be limited by the microwave-induced frequency shift of electric dipole spin resonance and it can be improved by optimization of control pulses. As we increase the control micro…
Solid-state approaches to quantum information technology are attractive because they are scalable. The coherent transport of quantum information over large distances, as required for a practical quantum computer, has been demonstrated by coupling solid-state qubits to photons1. As an alternative approach for a spin-based quantum computer, single electrons have also been transferred between distant quantum dots in times faster than their coherence time2, 3. However, there have been no demonstrations to date of techniques that can coherently transfer scalable qubits and perform quantum operation…
