Recent studies have demonstrated that the polarization states of high harmonics from solids can differ from those of the driving pulses. To gain insights on the microscopic origin of this behavior, we perform one-particle intraband-only calculations and reproduce some of the most striking observations. For instance, our calculations yield circularly polarized harmonics from elliptically polarized pulses that sensitively depend on the driving conditions. Furthermore, we perform experiments on ZnS and find partly similar characteristics as reported from silicon. Comparison to our intraband-only calculations shows reasonable qualitative agreement for a below-band-gap harmonic. We show that intraband dynamics predict depolarization effects for higher field strengths. For harmonics above the band gap, interband dynamics become important and the high-harmonic response to elliptical excitation looks systematically different. Our work proposes a method to distinguish between different high-harmonic generation mechanisms and it could pave the way to compact solid-state high-harmonic sources with controllable polarization states.
We experimentally demonstrate the efficient generation of circularly polarized pulses tunable from the vacuum to deep ultraviolet (160-380 nm) through resonant dispersive wave emission from optical solitons in a gas-filled hollow capillary fiber. In the deep ultraviolet we measure up to 13 microjoule of pulse energy, and from numerical simulations, we estimate the shortest output pulse duration to be 8.5 fs. We also experimentally verify that simply scaling the pulse energy by 3/2 between linearly and circularly polarized pumping closely reproduces the soliton and dispersive wave dynamics. Bas…
We derive expressions for the energy, linear momentum, and angular momentum content of circularly polarized Laguerre-Gaussian wave-packets propagating in free space. The vectorial nature of the electromagnetic field is taken into account, and the various consequences of paraxial approximation, which is typically invoked in theoretical treatments of the Laguerre-Gaussian beams, are examined.
We demonstrate an efficient scheme for the generation of broadband, high-energy, circularly polarized femtosecond laser pulses in the deep ultraviolet through seeded degenerate four-wave mixing in stretched gas-filled hollow capillary fibers. Pumping and seeding with circularly polarized 35 fs pulses centered at 400 nm and 800 nm, respectively, we generate idler pulses centered at 266 nm with more than 25 microjoule of energy and over 95% spectrally averaged ellipticity. Even higher idler energies and broad spectra (27 nm bandwidth) can be obtained at the cost of reduced ellipticity. Our syste…
Organic circularly polarized (CP) lasers have received increasing attention due to their future photoelectric applications. Here, we demonstrate a CP laser from a pure organic crystal-filled microcavity without any chiral molecules or chiral structures. Benefited from the giant anisotropy and excellent laser gain of organic crystals, optical Rashba-Dresselhaus spin-orbit coupling effect can be induced and is conductive to the CP laser in such microcavities. The maximum dissymmetry factor of the CP lasing with opposite helicities reached, is as high as 1.2. Our strategy may provide a new idea f…
Monte Carlo simulation of scattered circularly polarized light in biological tissues for detection technique of abnormal tissues using spin-polarized light emitting diodes
Chiral structures have reported radiation of circular polarized electromagnetic waves (CPs) in a specific direction. Here we report a class of torus knot radiators that is not only chiral but also three-dimensional (3-D) rotational symmetric along X, Y and Z axes. Because of this exotic chirality and symmetry, the knot radiator presented is able to demonstrate omnidirectional circular polarized radiation, which has never been reported in any known structures.
Propagation features of circularly polarized (CP) electromagnetic waves in magnetized plasmas are determined by the plasma density and the magnetic field strength. This property can be applied to design a unique plasma photonic device for intense short-pulse lasers. We have demonstrated by numerical simulations that a thin plasma foil under an external magnetic field works as a polarizing plate to separate a linearly polarized laser into two CP waves traveling in the opposite direction. This plasma photonic device has an advantage for generating intense CP waves even with a relativistic amplit…
A scheme for generating intense high-harmonic optical vortices is proposed. It relies on spin-orbit interaction of light when a relativistically-strong circularly polarized laser pulse irradiates a micro-plasma-waveguide. The intense laser field drives a strong surface wave at the inner boundary of the waveguide, which leads to high-order harmonic generation as the laser traveling inside. For a circularly polarized drive laser, the optical chirality is imprinted to the surface wave, which facilitates conversion of spin angular momentum of the fundamental light into orbital angular momenta of t…
Depolarization of circularly polarized light scattered from biological tissues depends on structural changes in cell nuclei, which can provide valuable information for differentiating cancer tissues concealed in healthy tissues. In this study, we experimentally verified the possibility of cancer identification using scattering of circularly polarized light. We investigated the polarization of light scattered from a sliced biological tissue with various optical configurations. A significant difference between circular polarizations of light scattered from cancerous and healthy tissues is observ…
Chiral four-wave-mixing signals are calculated using the irreducible tensor formalism. Different polarization and crossing angle configurations allow to single out the magnetic dipole and the electric quadrupole interactions. Other configurations can reveal that the chiral interaction occurs at a given step within the nonlinear interaction pathways contributing to the signal. Applications are made to the study of valence excitations of S-ibuprofen by chiral Stimulated X-ray Raman signals at the Carbon K-edge and by chiral visible 2D Electronic Spectroscopy.teraction pathways contributing to th…
Planar chiral nanoantenna for excitation-chirality-controlled hot spot modulation and emitter-coupled circularly polarized emission
Friedrich Schiller University Jena（耶拿弗里德里希·席勒大学）；Abbe Center of Photonics, Friedrich Schiller University Jena（耶拿弗里德里希·席勒大学阿贝光学中心）；Leibniz Institute of Photonic Technology（莱布尼茨光子技术研究所）；University of Würzburg（维尔茨堡大学）；The Australian National University（澳大利亚国立大学）；Academia Sinica（中央研究院）；National Yang Ming Chiao Tung University（国立阳明交通大学）
