In this study, the magnetic reversal process of exchange-coupled bilayer systems, consisting of a ferrimagnetic TbFeCo alloy layer and a ferromagnetic [Co/Ni/Pt]N multilayer, was investigated. In particular, minor loop studies, probing solely the reversal characteristics of the softer ferromagnetic layer, reveal two distinct reversal mechanisms, which depend strongly on the thickness of the ferromagnetic layer. For thick layers, irreversible switching of the macroscopic minor loop is observed. The underlying microscopic origin of this reversal process was studied in detail by high-resolution magnetic force microscopy, showing that the reversal is triggered by in-plane domain walls propagating through the ferromagnetic layer. In contrast, thin ferromagnetic layers show a hysteresis-free reversal, which is nucleation-dominated due to grain-to-grain variations in magnetic anisotropy of the Co/Ni/Pt multilayer and an inhomogeneous exchange coupling with the magnetically hard TbFeCo layer, as confirmed by micromagnetic simulations.
Electrical detection of topological magnetic textures such as skyrmions is currently limited to conducting materials. While magnetic insulators offer key advantages for skyrmion technologies with high speed and low loss, they have not yet been explored electrically. Here, we report a prominent topological Hall effect in Pt/Tm$_3$Fe$_5$O$_{12}$ bilayers, where the pristine Tm$_3$Fe$_5$O$_{12}$ epitaxial films down to 1.25 unit cell thickness allow for tuning of topological Hall stability over a broad range from 200 to 465 K through atomic-scale thickness control. Although Tm$_3$Fe$_5$O$_{12}$ i…
Dynamic magnetic features of a mixed ferro-ferrimagnetic ternary alloy in the form of AB$_p$C$_{1-p}$, especially. The effect of Hamiltonian parameters on the dynamic magnetic features of the system are investigated. For this aim, an AB$_p$C$_{1-p}$ ternary alloy system was simulated within the mean-field approximation based on a Glauber type stochastic dynamic and for simplicity, A, B and C ions as SA = 1/2, SB = 1 and SC = 3/2, were chosen respectively. It was found that in our dynamic system the critical temperature was always dependent on the concentration ratio of the ternary alloy.
It has been shown that W in its resistive form possesses the largest spin-Hall ratio among all heavy transition metals, which makes it a good candidate for generating efficient dampinglike spin-orbit torque (DL-SOT) acting upon adjacent ferromagnetic or ferrimagnetic (FM) layer. Here we provide a systematic study on the spin transport properties of W/FM magnetic heterostructures with the FM layer being ferromagnetic Co$_{20}$Fe$_{60}$B$_{20}$ or ferrimagnetic Co$_{63}$Tb$_{37}$ with perpendicular magnetic anisotropy. The DL-SOT efficiency $|ξ_{DL}|$, which is characterized by a current-induced…
Multiferroic materials, in which ferroelectric and magnetic ordering coexist, are of fundamental interest for the development of novel memory devices that allow for electrical writing and non-destructive magnetic readout operation. The great challenge is to create room temperature multiferroic materials with strongly coupled ferroelectric and ferromagnetic (or ferrimagnetic) orderings. BiFeO3 has been the most heavily investigated single-phase multiferroic to date due to the coexistence of its magnetic order and ferroelectric order at room temperature. However, there is no net magnetic moment …
The paper presents a computational study of the ground-state magnetic phases of a selected bilayer graphene nanoflake in external electric field and magnetic field. The electric field has parallel and perpendicular component while the magnetic field is oriented in plane. The system consists of two rectangular layers having armchair edges and zigzag terminations with Bernal stacking. The theoretical model is based on a tight binding Hamiltonian with Hubbard term. The magnetic phase diagram involving the total spin is constructed, showing the stability areas of phases with total spin values equa…
Element-resolved x-ray ferrimagnetic and ferromagnetic resonance spectroscopy
我们报告使用X射线磁圆二色性（XMCD）在千兆赫频率的元素特定的磁共振谱的测量。我们研究了Gd取代钇铁石榴石中Gd和Fe离子的亚铁磁旋进，表明Gd的共振场和线宽与Fe精确一致，直到参数激发的非线性区域。相对于Fe的Gd X射线磁共振信号的相反符号与两种离子物种的动态反铁磁对准一致。此外，我们研究了双层金属膜，Ni $_{80}$ Fe $_{20}$（5 nm）/Ni（50 nm），其中Ni和Ni $_{80}$ Fe $_{20}$的耦合共振模式分别解决，揭示了在各个层的共振场的位移，但没有相互驱动的效果。能量依赖的动态XMCD测量，结合X射线吸收和磁共振光谱。
We study the heat-induced magnetization dynamics in a toy model of a ferrimagnetic alloy, which includes localized spins antiferromagnetically coupled to an itinerant carrier system with a Stoner gap. We determine the one-particle spin-density matrix including exchange scattering between localized and itinerant bands as well as scattering with phonons. While a transient ferromagnetic-like state can always be achieved by a sufficiently strong excitation, this transient ferromagnetic-like state only leads to magnetization switching for model parameters that also yield a compensation point in the…
Ferromagnetic spintronics has been a main focus as it offers non-volatile memory and logic applications through current-induced spin-transfer torques. Enabling wider applications of such magnetic devices requires a lower switching current for a smaller cell while keeping the thermal stability of magnetic cells for non-volatility. As the cell size reduces, however, it becomes extremely difficult to meet this requirement with ferromagnets because spin-transfer torque for ferromagnets is a surface torque due to rapid spin dephasing, leading to the 1/ferromagnet-thickness dependence of the spin-to…
Magnetic topological quantum materials have attracted great attention due to their exotic topological quantum physics induced by the interplay among crystalology, magnetism, and topology, which is of profound importance to fundamental research and technology applications. However, limited materials are experimentally available, most of whom are realized by magnetic impurity doping or heterostructural constructions. In this work, based on the first-principles calculations, we predict that double perovskite Ba2CdReO6 is an intrinsic ferromagnetic topological semi-half-metal, while the ferrimagne…
Ferromagnetic materials dominate as the magnetically active element in spintronic devices, but come with drawbacks such as large stray fields, and low operational frequencies. Compensated ferrimagnets provide an alternative as they combine the ultrafast magnetization dynamics of antiferromagnets with a ferromagnet-like spin-orbit-torque (SOT) behavior. However to use ferrimagnets in spintronic devices their advantageous properties must be retained also in ultrathin films (t < 10 nm). In this study, ferrimagnetic Gdx(Fe87.5Co12.5)1-x thin films in the thickness range t = 2-20 nm were grown on h…
Trirutile-type LiFe$_2$F$_6$ is a charge-ordered material with Fe$^{2+}$/Fe$^{3+}$ configuration. Here its physical properties, including magnetism, electronic structure, phase transition, and charge ordering, are studied theoretically. On one hand, the charge ordering leads to improper ferroelectricity with a large polarization. On the other hand, its magnetic ground state can be tuned from the antiferromagnetic to ferrimagnetic by moderate compressive strain. Thus, LiFe$_2$F$_6$ can be a rare multiferroic with both large magnetization and polarization. Most importantly, since the charge orde…
We use micro-focus Brillouin light scattering spectroscopy to study the effects of spin-orbit torque on thermal spin waves in almost angular-momentum compensated ferrimagnetic CoGd alloy films. The spin-orbit torque is produced by the electric current flowing in the Pt layer adjacent to CoGd. Both the ferromagnetic and the exchange modes are detected in our measurements. The intensity and the linewidth of the ferromagnetic mode are modified by the spin-orbit torque. In contrast, the properties of the exchange mode are unaffected by the spin-orbit torque. We also find that the frequencies and t…
We report ferroelectric ordering in Ni substituted CaBaCo4O7. Magnetization showed ferrimagnetic transition at 60 K and an additional transition is found ~ 82 K, further, enhanced antiferromagnetic interactions and decrease in saturation magnetization are noticed with Ni substitution. The dielectric and pyroelectric measurements illustrate a strong coupling between spin and charge degrees of freedom; ferroelectric behavior is confirmed with enhanced ordering temperature (~82 K) and saturation polarization (250 muC/m2. Neutron diffraction has revealed an increase in c-lattice parameter in Ni sa…
In the increasing interests on spin-orbit torque (SOT) with various magnetic materials, we investigated SOT in rare earth-transition metal ferrimagnetic alloys. The harmonic Hall measurements were performed in Pt/GdFeCo bilayers to quantify the effective fields resulting from the SOT. It is found that the damping-like torque rapidly increases near the magnetization compensation temperature TM of the GdFeCo, which is attributed to the reduction of the net magnetic moment.
Spinel Li$_x$Mn$_2$O$_4$ is a key cathode material that is used extensively in commercial Li-ion batteries. A challenge with this material has been that the capacity of the battery fades with cycling, an effect that can be traced to the presence of an anti-ferromagnetic insulator phase in the fully lithiated LiMn$_2$O$_4$ (LMO) and the associated charge disproportionation that drives distortions of the MnO$_6$ octahedra. Here, by combining x-ray magnetic Compton scattering experiments with parallel first-principles computations, we show that the anti-ferromagnetic phase of LMO is surrounded by…
Nowdays, multiferroic materials with magnetoelectric coupling have many real-world applications in the fields of novel memory devices. It is challenging is to create multiferroic materials with strongly coupled ferroelectric and ferrimagnetic orderings at room temperature. The single crystal of ferric selenide (Fe3Se4) shows type-II multiferroic due to the coexistence of ferroelectric as well as magnetic ordering at room temperature. We have investigated the lattice instability, electronic structure, ferroelectric, ferrimagnetic ordering and transport properties of ferroelectric metal Fe3Se4. …
Magnetic skyrmions are swirling magnetic textures with novel characteristics suitable for future spintronic and topological applications. Recent studies confirmed the room-temperature stabilization of skyrmions in ultrathin ferromagnets. However, such ferromagnetic skyrmions show undesirable topological effect, the skyrmion Hall effect, which leads to their current-driven motion towards device edges, where skyrmions could easily be annihilated by topographic defects. Recent theoretical studies have predicted enhanced current-driven behaviour for antiferromagnetically exchange-coupled skyrmions…
In the quantum Hall regime of graphene, antiferromagnetic and spin-polarized ferromagnetic states at the zeroth Landau level compete, leading to a canted antiferromagnetic state depending on the direction and magnitude of an applied magnetic field. Here, we investigate this transition at 2.7 K in graphene Hall bars that are proximity coupled to the ferrimagnetic insulator Y$_{3}$Fe$_{5}$O$_{12}$. From nonlocal transport measurements, we demonstrate an induced magnetic exchange field in graphene, which lowers the magnetic field required to modulate the magnetic state in graphene. These results …
Lithium and Vanadium Intercalation into Bilayer V2Se2O: Ferrimagnetic-Ferroelastic Multiferroics and Anomalous and Spin Transport
Huazhong University of Science and Technology（华中科技大学）；Shandong Normal University（山东师范大学）；Chongqing University of Posts and Telecommunications（重庆邮电大学）；University of Wollongong（伍伦贡大学）；Florida State University（佛罗里达州立大学）；National High Magnetic Field Laboratory（国家强磁场实验室）
We provide a macroscopic theory and experimental results for magnetic resonances of antiferromagnetically-coupled ferrimagnets. Our theory, which interpolates the dynamics of antiferromagnets and ferromagnets smoothly, can describe ferrimagnetic resonances across the angular momentum compensation point. We also present experimental results for spin-torque induced ferrimagnetic resonance at several temperatures. The spectral analysis based on our theory reveals that the Gilbert damping parameter, which has been considered to be strongly temperature dependent, is insensitive to temperature. We e…
Although several multiferroic materials/heterostructures have been extensively studied, finding strong magnetoelectric couplings for the electric field control of the magnetization remains challenging. Here, a novel interfacial magnetoelectric coupling based on three components (ferroelectric dipole, magnetic moment, and antiferromagnetic order) is analytically formulated. As an extension of carrier-mediated magnetoelectricity, the new coupling is shown to induce an electric-magnetic hysteresis loop. Realizations employing BiFeO$_3$ bilayers grown along the [$111$] axis are proposed. Without i…
Two-dimensional (2D) ferromagnets with high Curie temperature have long been the pursuit for electronic and spintronic applications. CrI3 is a rising star of intrinsic 2D ferromagnets, however, it suffers from weak exchange coupling. Here we propose a general strategy of self-intercalation to achieve enhanced ferromagnetism in bilayer CrI3. We showed that filling either Cr or I atoms into the van der Waals gap of stacked and twisted CrI3 bilayers can induce the double exchange effect and significantly strengthen the interlayer ferromagnetic coupling. According to our first-principles calculati…
We carefully investigated the ferromagnetic coupling in the as-grown and annealed ferromagnetic semiconductor GaMnAs/AlGaMnAs bilayer devices. We observed that the magnetic interaction between the two layers strongly affects the magnetoresistance of the GaMnAs layer with applying out of plane magnetic field. After low temperature annealing, the magnetic easy axis of the AlGaMnAs layer switches from out of plane into in-plane and the interlayer coupling efficiency is reduced from up to 0.6 to less than 0.4. However, the magnetic coupling penetration depth for the annealed device is twice that o…
Strong ferromagnetic interlayer exchange couplings $J$ in perpendicularly magnetized systems are becoming increasingly desirable for applications. We study whether ferromagnetic interlayer exchange couplings can be measured by a combination of broadband ferromagnetic resonance methods and magnetometry hysteresis loops. For this we model the switching and the eigenexcitations in bilayer systems comprising a soft layer coupled to a thicker harder layer that possesses higher perpendicular magnetic anisotropy. For large $J >0$ the switching fields are essentially independent of $J$ but the frequen…
Recently intrinsic ferromagnetism in two-dimensional(2D) van der Waals materials was discovered [1, 2, 3]. A monolayer of Chromiun triiodide(CrI3) is ferromagnetic while a bilayer structure was reported to be anti-ferro magnetic, moreover an external electric field changes its magnetic phase [4]. We have studied the two found in nature stackings of CrI3 bilayers and found that indeed the magnetic phase of one of them can be tuned by an external electric field while the other remains ferromagnetic. We simulate those results with ab initio calculations and explain them with a simple model based …
Heterostructures of two-dimensional (2D) layered materials with selective compositions play an important role in creating novel functionalities. Effective interface coupling between 2D ferromagnet and electronic materials would enable the generation of exotic physical phenomena caused by intrinsic symmetry breaking and proximity effect at interfaces. Here, epitaxial growth of bilayer Bi(110) on 2D ferromagnetic Fe3GeTe2 (FGT) with large magnetic anisotropy has been reported. Bilayer Bi(110) islands are found to extend along fixed lattice directions of FGT. The six preferred orientations could …
We present the Co-Gd composition dependence of the spin-Hall magnetoresistance (SMR) and anisotropic magnetoresistance (AMR) for ferrimagnetic Co100-xGdx / Pt bilayers. With Gd concentration x, its magnetic moment increasingly competes with the Co moment in the net magnetization. We find a nearly compensated ferrimagnetic state at x = 24. The AMR changes sign from positive to negative with increasing x, vanishing near the magnetization compensation. On the other hand, the SMR does not vary significantly even where the AMR vanishes. These experimental results indicate that very different scatte…
We utilize anisotropic magnetoresistance to study temporal evolution of the magnetization state in epitaxial Ni$_{80}$Fe$_{20}$/Fe$_{50}$Mn$_{50}$ ferromagnet/antiferromagnet bilayers. The resistance exhibits power-law evolution over a wide range of temperatures and magnetic fields, indicating that aging is characterized by a wide range of activation time scales. We show that aging is a cooperative process, i.e. the magnetic system is not a superposition of weakly interacting subsystems characterized by simple Arrhenius activation. The observed effects are reminiscent of avalanches in granular…
Spin-orbit torque (SOT)-induced magnetization switching shows promise for realizing ultrafast and reliable spintronics devices. Bipolar switching of perpendicular magnetization via SOT is achieved under an in-plane magnetic field collinear with an applied current. Typical structures studied so far comprise a nonmagnet/ferromagnet (NM/FM) bilayer, where the spin Hall effect in the NM is responsible for the switching. Here we show that an antiferromagnet/ferromagnet (AFM/FM) bilayer system also exhibits a SOT large enough to switch the magnetization of FM. In this material system, thanks to the …
Extraordinary electronic phases can form in artificial oxide heterostructures, which will provide a fertile ground for new physics and also give rise to novel device functions. Based on a systematic first-principles density functional theory study of the magnetic and electronic properties of the (111) superlattices (ABO3)2/(AB'O3)10 of 4d and 5d transition metal perovskite (B = Ru, Rh, Ag, Re, Os, Ir, Au; AB'O3 = LaAlO3, SrTiO3), we demonstrate that due to quantum confinement, bilayers (LaBO3)2 (B = Ru, Re, Os) and (SrBO3)2 (B = Rh, Os, Ir) are ferromagnetic with ordering temperatures up to ro…
Many technologically useful magnetic oxides are ferrimagnetic insulators, which consist of chemically distinct cations. Here, we examine the spin dynamics of different magnetic cations in ferrimagnetic NiZnAl-ferrite (Ni$_{0.65}$Zn$_{0.35}$Al$_{0.8}$Fe$_{1.2}$O$_4$) under continuous microwave excitation. Specifically, we employ time-resolved x-ray ferromagnetic resonance to separately probe Fe$^{2+/3+}$ and Ni$^{2+}$ cations on different sublattice sites. Our results show that the precessing cation moments retain a rigid, collinear configuration to within $\approx$2$^\circ$. Moreover, the effe…
