arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2005.14486cond-mat.mtrl-scicond-mat.mes-hall
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用于电子泵浦紫外光源的AlGaN/AlN量子点超晶格的内量子效率

Internal quantum efficiency of AlGaN/AlN quantum dot superlattices for electron-pumped ultraviolet sources

A. Harikumar, F. Donatini, C. Bougerol, E. Bellet-Amalric, Q. -M. Thai, C. Dujardin, I. Dimkou, S. T. Purcell, E. Monroy

摘要:

在本文中,我们描述了530 nm厚的超晶格(100个周期)的AlxGa 1-xN/AlN(x = 0,0.1)的Stranski-Krastanov量子点的应用程序作为电子束泵浦紫外灯的有源区的生长和表征。采用分子束外延技术制备了高密度(> 10 e11 cm-2)的量子点层,并研究了生长过程中III/V比对其光学性能的影响。该研究考虑了在室温下在244-335 nm范围内发射的结构,相对线宽在6-11%范围内,主要是由于自组装生长中固有的QD直径分散。在电子泵浦下,对于低于9 kV的加速电压,发射效率保持恒定。该阈值与超晶格的总厚度和电子束的穿透深度的相关性证实了纳米结构沿生长轴的均匀性。在阈值以下,发射强度与注入电流成线性比例。内量子效率的特点是在低注入,这揭示了在非辐射过程方面的材料特性,和高注入,这模仿载流子注入的操作条件。在III/V比< 0.75的量子点中,从低注入到高达200 kW/cm 2的泵浦功率密度,内量子效率保持在50%左右,是第一种呈现这种稳定行为的纳米结构。

英文摘要:

In this paper, we describe the growth and characterization of 530-nm-thick superlattices (100 periods) of AlxGa1-xN/AlN (x = 0, 0.1) Stranski-Krastanov quantum dots for application as the active region of electron-beam pumped ultraviolet lamps. Highly dense (>10e11 cm-2) quantum dot layers are deposited by molecular beam epitaxy, and we explore the effect of the III/V ratio during the growth process on their optical performance. The study considers structures emitting in the 244-335 nm range at room temperature, with a relative linewidth in the 6-11% range, mainly due to the QD diameter dispersion inherent in self-assembled growth. Under electron pumping, the emission efficiency remains constant for acceleration voltages below 9 kV. The correlation of this threshold with the total thickness of the superlattice and the penetration depth of the electron beam confirms the homogeneity of the nanostructures along the growth axis. Below the threshold, the emission intensity scales linearly with the injected current. The internal quantum efficiency is characterized at low injection, which reveals the material properties in terms of non-radiative processes, and high injection, which emulates carrier injection in operation conditions. In quantum dots synthesized with III/V ratio < 0.75, the internal quantum efficiency remains around 50% from low injection to pumping power densities as high as 200 kW/cm2, being the first kind of nanostructures that present such stable behaviour.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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